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We use the isoconfigurational (IC) ensemble to show the connection between emerging heterogeneities in the tetrahedral order parameter and the dynamic propensity in a mildly undercooled glass-forming liquid. We observe that spatially…

Soft Condensed Matter · Physics 2021-01-18 M Shajahan G Razul , Gurpreet S Matharoo , Balakrishnan Viswanathan

Collective motion over increasing length scales is a signature of the vitrification process of liquids. We demonstrate the emergence of distinct static and dynamic length scales probed near the free surface in fully equilibrated…

Statistical Mechanics · Physics 2022-11-28 Hailong Peng , Huashan Liu , Thomas Voigtmann

We study hydrogen-bond dynamics in liquid water at low temperatures using molecular dynamics simulations. We find that bond lifetime (``fast dynamics'') has Arrhenius temperature dependence. We also calculate the bond correlation function…

Condensed Matter · Physics 2009-10-31 Francis W. Starr , Johannes K. Nielsen , H. Eugene Stanley

We present numerical results obtained from Time-Dependent Density Functional calculations of the dynamics of liquid He-4 in different environments characterized by geometrical confinement. The time-dependent density profile and velocity…

Condensed Matter · Physics 2009-11-07 Luigi Giacomazzi , Flavio Toigo , Francesco Ancilotto

Dynamic heterogeneity, believed to be one of the hallmarks of the dynamics of supercooled liquids, is expected to affect the diffusion of the particles comprising the liquid. We have carried out extensive molecular dynamics simulations of…

Soft Condensed Matter · Physics 2019-12-23 Rajsekhar Das , Chandan Dasgupta , Smarajit Karmakar

The spatial correlation function of the momentum density in the three-dimensional dilute sheared granular fluids is theoretically investigated. The existence of the long-range correlation is verified through both the analytic calculation…

Statistical Mechanics · Physics 2009-11-13 Michio Otsuki , Hisao Hayakawa

The super-cooled $N3$ model exhibits an increasingly slow dynamics as density approaches the model's random closest packing density. Here, we present a direct measurement of the dynamical correlation function $G_4(r,t)$, showing the…

Statistical Mechanics · Physics 2010-12-21 Ziv Rotman , Eli Eisenberg

We study the temporal and spatial correlations in a one-dimensional model of a heterogeneous fault zone, in the presence of visco-elastic effects. As a function of dynamical weakening and of dissipation, the system exhibits three different…

Statistical Mechanics · Physics 2015-06-24 Bora Orcal , Ayse Erzan

Glass formers exhibit a viscoelastic behavior: at the laboratory timescale, they behave like (glassy) solids at low temperatures, and like liquids at high temperatures. Based on this observation, elastic models relate the long time…

Chemical Physics · Physics 2017-08-01 Emmanuel Guillaud , Laurent Joly , Dominique De Ligny , Samy Merabia

One of the most controversial hypotheses for explaining the heterogeneous dynamics of glasses postulates the temporary coexistence of two phases characterized by a high and by a low diffusivity. In this scenario, two phases with different…

Soft Condensed Matter · Physics 2015-07-16 R. Pastore , A. Coniglio , M. Pica Ciamarra

A static correlation function of concentration fluctuations in a (dilute) binary liquid mixture subjected to both a concentration gradient and uniform shear flow is investigated within the framework of fluctuating hydrodynamics. It is shown…

Statistical Mechanics · Physics 2009-11-10 Hirofumi Wada

In a preceding paper, Mukhopadhyay and I studied the diffusive motion of a tagged molecule in a heterogeneous glass-forming liquid at temperatures just above a glass transition. Among other features of this system, we postulated a relation…

Statistical Mechanics · Physics 2009-11-13 J. S. Langer

We study nonequilibrium dynamical properties of inhomogeneous systems, in particular at a free surface or at a defect plane. Thereby we consider nonconserved (model-A) dynamics of a system which is prepared in the high-temperature phase and…

Statistical Mechanics · Physics 2009-11-10 Michel Pleimling , Ferenc Igloi

Relaxation processes in supercooled liquids are known to exhibit interesting as well as complex behavior. One of the hallmarks of this relaxation process observed in the measured auto correlation function is occurrence of multiple steps of…

Soft Condensed Matter · Physics 2018-08-01 Rajsekhar Das , Indrajit Tah , Smarajit Karmakar

This paper is the fourth in a series exploring the physical consequences of the solidity of highly viscous liquids. It is argued that the two basic characteristics of a flow event (a jump between two energy minima in configuration space)…

Soft Condensed Matter · Physics 2007-05-23 Jeppe C. Dyre

Despite the use of glasses for thousands of years, the nature of the glass transition is still mysterious. On approaching the glass transition, the growth of dynamic heterogeneity has long been thought to play a key role in explaining the…

Soft Condensed Matter · Physics 2018-03-23 Lijin Wang , Ning Xu , W. H. Wang , Pengfei Guan

Particle suspensions, present in many natural and industrial settings, typically contain aggregates or other microstructures that can complicate macroscopic flow behaviors and damage processing equipment. Recent work found that applying…

Soft Condensed Matter · Physics 2018-07-31 Jikai Wang , J. M. Schwarz , Joseph D. Paulsen

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, $T_{MCT}$. Specifically, we follow the evolution of…

Soft Condensed Matter · Physics 2009-11-10 M. Vogel , S. C. Glotzer

We investigate the relaxation mechanism of a supercooled tetrahedral liquid at its limit of stability using isothermal isobaric ($NPT$) Monte Carlo (MC) simulations. In similarity with systems which are far from equilibrium but near the…

Statistical Mechanics · Physics 2017-09-06 Arvind Kumar Gautam , Nandlal Pingua , Aashish Goyal , Pankaj A. Apte

We have gone through the detailed microscopic calculation of the shear viscosity of a 2-dimensional graphene system in the relaxation time approximation-based kinetic theory framework. After getting its final expressions, we compared it…

Nuclear Theory · Physics 2024-03-27 Cho Win Aung , Thandar Zaw Win , Gaurav Khandal , Sabyasachi Ghosh
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