Related papers: Quantum dynamics of molecules in 4He nano-droplets…
Quantum coherence is highly involved in photochemical functioning of complex molecular systems. Co-existence and intermixing of electronic and/or vibrational coherences, while never unambiguously identified experimentally, has been proposed…
To describe long-range behaviour of one particle removed from a few- or a many-body system, a hyperspherical cluster model has been developed. It has been applied to the ground and first excited states of helium drops with five, six, eight…
Surface waves on both superfluid 3He and 4He were examined with the premise, that these inviscid media would represent ideal realizations for this fluid dynamics problem. The work on 3He is one of the first of its kind, but on 4He it was…
We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this hybrid system. Its incoherent part, the one arising…
Ensembles of elongated magnetic droplets in a rotating field are studied experimentally. In a given range of field strength and frequency the droplets form rotating structures with a triangular order - rotating crystals. A model is…
Vortex flow remains laminar up to large Reynolds numbers (Re~1000) in a cylinder filled with 3He-B. This is inferred from NMR measurements and numerical vortex filament calculations where we study the spin up and spin down responses of the…
The dynamics of non-polar diatomic molecules interacting with a far-detuned narrow-band laser field, that only may drive rotational transitions, is studied. The rotation of the molecule is considered both classically and quantum…
We have studied the structure of $^4$He droplets doped with magnesium atoms using density functional theory. We have found that the solvation properties of this system strongly depend on the size of the $^4$He droplet. For small drops, Mg…
Droplet deformations caused by substrate vibrations are ubiquitous in nature and highly relevant for applications such as microreactors and single-cell sorting. The vibrations can induce droplet oscillations, a fundamental process that…
Spin dynamics of nanomolecules and nanoclusters are analyzed. The nanosizes of these objects make it possible to consider them as single-domain magnets with a large total spin, where the motion of the spins of all atoms, composing a…
In a recent study we have reported a new type of trial wave function symmetric under the exchange of particles and which is able to describe a supersolid phase. In this work, we use the diffusion Monte Carlo method and this model wave…
The chemical and physical properties of molecular clusters can heavily depend on their size, which makes them very attractive for the design of new materials with tailored properties. Deriving the structure and dynamics of clusters is…
In recent years, experimental data were published which point to the possibility of the existence of superfluidity in solid helium. To investigate this phenomenon theoretically we employ a hierarchy of equations for reduced density matrices…
The transition between the gas-, supercritical-, and liquid-phase behaviour is a fascinating topic which still lacks molecular-level understanding. Recent ultrafast two-dimensional infrared spectroscopy experiments suggested that the…
We have studied the merging of two $^4$He droplets at zero temperature, caused by their Van der Waals mutual attraction. During the early stages of the merging, density structures appear which closely match the experimental observations by…
The relevance of the point-symmetry group $\mathcal{D}_{4h}$ for the prediction of spectrum and electromagnetic properties of the $^{24}\mathrm{Mg}$ nucleus is discussed in the framework of the geometric $\alpha$-cluster model at leading…
Low temperature structural and superfluid properties of $^4$He confined in cylindrical nanopores are theoretically investigated by means of first principle Quantum Monte Carlo (QMC) simulations. We vary the density of $^4$He inside the…
A frozen, solid helium core, dubbed snowball, is typically observed around cations in liquid helium. Here we discover, using path integral simulations, that around a cationic molecular impurity, protonated methane, the $^4$He atoms are…
We have used nanoelectromechanical resonators to probe superfluid $^4$He at different temperature regimes, spanning over four orders of magnitude in damping. These regimes are characterized by the mechanisms which provide the dominant…
We propose a mechanism of a vortex nucleation in a flow of a superfluid $^4He$. The mechanism is related to the creation by critical fluctuations of a "plasma" of half-vortex rings located near the wall. The "plasma" screens the attraction…