Related papers: Quantum dynamics of molecules in 4He nano-droplets…
The rotational dynamics of a supercooled molecular liquid is investigated by a molecular-dynamics numerical study. We detect rotational jumps with a waiting-time distribution which is well fitted by a truncated power law. At lower…
Due to its broken spin and orbit rotation symmetries, superfluid $^3$He plays a unique role for testing rotational quantum properties on a macroscopic scale. In this system the orbital momentum forms textures that provide an effective…
We have studied the solubility of molecular hydrogen in bulk liquid $^4$He at zero temperature using the diffusion Monte Carlo method and realistic interatomic potentials between the different species of the mixture. Around the $^4$He…
We review current understanding of the non-equilibrium dynamics of collective quantum systems. We describe an approach based on the Hamiltonian formulation of superfluid hydrodynamics. It is shown that, in the presence of constant energy…
We use molecular dynamics simulations to probe the rotational dynamics of the SPC/E model of water for a range of temperatures down to 200 K, 13 K above to the mode coupling temperature. We find that rotational dynamics is spatially…
We experimentally demonstrate control of molecular rotation in bulk superfluid $^4\mathrm{He}$. Metastable helium dimers, $\mathrm{He}_2^*$, are rotationally excited by a periodic train of linearly polarized femtosecond laser pulses. We…
Superfluidity is a well-characterized quantum phenomenon which entails frictionless-motion of mesoscopic particles through a superfluid, such as $^4$He or dilute atomic-gases at very low temperatures. As shown by Landau, the incompatibility…
Electric deflection measurements on liquid helium nanodroplets doped with individual polar molecules demonstrate that the cold superfluid matrix enables full orientation of the molecular dipole along the external field. This translates into…
We present a microscopic quantum analysis for rotational constants of the OCS-H$_2$ complex in helium droplets using the local two-fluid theory in conjunction with path integral Monte Carlo simulations. Rotational constants are derived from…
The flow of superfluid $^4$He around a translationally oscillating sphere, levitating without mechanical support, can either be laminar or turbulent, depending on the velocity amplitude. Below a critical velocity $v_c$ that scales as…
This article provides a review of recent work in the field of helium nanodroplet spectroscopy with emphasis on the dynamical aspects of the interactions between molecules in helium as well as their interaction with this unique quantum…
We present a study of the dynamics and structural changes for trans-1,2-dichloroethylene between high and low density liquids using neutron scattering techniques (diffraction, small angle neutron scattering and time of flight spectroscopy)…
The observation of a non-classical rotation inertia (NCRI) fraction in bulk solid 4He by M. Chan and E. Kim attracted significant interest as a possible manifestation of supersolid state of matter. Despite numerous experimental and…
Defects are believed to play a fundamental role in the supersolid state of 4He. We report on studies by exact Quantum Monte Carlo (QMC) simulations at zero temperature of the properties of solid 4He in presence of many vacancies, up to 30…
Decoherent quantum equations of motion are derived that yield the trajectory of an open quantum system. The viscosity of superfluid Lennard-Jones helium-4 is obtained with a quantum stochastic molecular dynamics algorithm. The momentum…
In recent torsional oscillator experiments by Kim and Chan (KC), a decrease of rotational inertia has been observed in solid 4He in porous materials and in a bulk annular channel. This observation strongly suggests the existence of…
The dynamic behavior of a partially wetting polymer droplet driven over a nanostructured interface is studied using molecular dynamics simulations. We consider the bead-spring model to represent a polymeric liquid that partially wets a…
Because of their central importance in chemistry and biology, water molecules have been the subject of decades of intense spectroscopic investigations. Rotational spectroscopy of water vapor has yielded detailed information about the…
Within the diffusion Monte Carlo approach, we have determined the structure of isotopically pure and mixed helium droplets doped with one magnesium atom. For pure 4He clusters, our results confirm those of M. Mella et al. [J. Chem. Phys.…
We investigate the ground state and dynamics of one-dimensional spin-orbit coupled (SOC) quantum droplets within the extended Gross-Pitaevskii approach. As the SOC wavenumber increases, stripe droplet patterns emerge, with a flat-top…