Related papers: Quantum dynamics of molecules in 4He nano-droplets…
Much of our knowledge about dynamics and functionality of molecular systems has been achieved with femtosecond time-resolved spectroscopy. Despite extensive technical developments over the past decades, some classes of systems have eluded…
Besides the use as cold matrix for spectroscopic studies, superfluid helium droplets have served as a cold environment for the synthesis of molecules and clusters. Since vibrational frequencies of molecules in helium droplets exhibit almost…
Using density functional theory, we investigate the structure of mixed $^3$He$_{N_3}$-$^4$He$_{N_4}$ droplets with an embedded impurity (Xe atom or HCN molecule) which pins a quantized vortex line. We find that the…
We have theoretically investigated the structure of spinning self-bound droplets made of $^{41}$K-$^{87}$Rb Bose mixture by solving the Gross-Pitaevskii equation including beyond-mean-field correction in the Lee-Huang-Yang form. The…
The superfluid transition in liquid 4He filled in Gelsil glass observed in recent experiments is discussed in the framework of quantum critical phenomena. We show that quantum fluctuations of phase are indeed important at the experimentally…
Rapid new developments have occurred in superfluid hydrodynamics since the discovery of a host of unusual phenomena which arise from the diverse structure and dynamics of quantized vortices in 3He superfluids. These have been studied in…
A semi-phenomenological model of a many-particle system of 4He atoms is proposed, in which a helium atom is considered as a complex consisting of a nucleus and a bound pair of electrons in the singlet state. At zero temperature, there are…
We address the collision of two superfluid 4 He droplets at non-zero initial relative velocities and impact parameters within the framework of liquid 4 He time-dependent density functional theory at zero temperature. In spite of the small…
We have explored the light induced dynamics in superfluid helium nanodroplets with wide-angle scattering in a pump-probe measurement scheme. The droplets are doped with xenon atoms to facilitate the ignition of a nanoplasma through…
We present a novel density functional for liquid 4He, properly accounting for the static response function and the phonon-roton dispersion in the uniform liquid. The functional is used to study both structural and dynamical properties of…
The experimental investigation of superfluid turbulence in 3He-B is generally not possible with the techniques which have been developed for 4He-II. We describe a new method by which a transient burst of turbulent vortex expansion can be…
We have developed a nanomechanical resonator, for which the motional degree of freedom is a superfluid 4He oscillating flow confined to precisely defined nanofluidic channels. It is composed of an in-cavity capacitor measuring the…
Two-dimensional superfluidity and quantum turbulence are directly connected to the microscopic dynamics of quantized vortices. However, surface effects have prevented direct observations of coherent vortex dynamics in strongly-interacting…
Alignment of OCS, CS$_2$ and I$_2$ molecules embedded in helium nanodroplets is measured as a function of time following rotational excitation by a non-resonant, comparatively weak ps laser pulse. The distinct peaks in the power spectra,…
We propose a new theoretical approach to the excitation spectrum of superfluid ${^4}He$. It is based on the assumption that, in addition to the usual Feynman density fluctuations, there exist localized modes which describe the short range…
The paper is concerned with the interpretation of many experiments that have been reported recently on the production of quantum turbulence by oscillating spheres, wires and grids in both 4He and 3He-B at temperatures so low that there is a…
We study quantum droplets emerging in a quasi-one-dimensional asymmetric mixture of two atomic species with different intra-component coupling constants. We find that such mixtures support a rich variety of multipole quantum droplets, where…
We study a polar molecule immersed into a superfluid environment, such as a helium nanodroplet or a Bose-Einstein condensate, in the presence of an intense electrostatic field. We show that coupling of the molecular pendular motion, induced…
For future quantum technologies the combination of a long quantum state lifetime and an efficient interface with external optical excitation are required. In solids, the former is for example achieved by individual spins, while the latter…
In several settings of physics and chemistry one has to deal with molecules interacting with some kind of an external environment, be it a gas, a solution, or a crystal surface. Understanding molecular processes in the presence of such a…