Related papers: Quantum dynamics of molecules in 4He nano-droplets…
Accurate computer simulations of the rotational dynamics of linear molecules solvated in He clusters indicate that the large-size (nano-droplet) regime is attained quickly for light rotors (HCN, CO) and slowly for heavy ones (OCS, N$_2$O,…
Within Density Functional Theory, we have studied the interplay between vortex arrays and capillary waves in spinning prolate He-4 droplets made of several thousands of helium atoms. Surface capillary waves are ubiquitous in prolate…
Superfluid 4He, the first superfluid ever discovered, is in some ways the least well understood. Unlike 3He superfluid, or the variety of Bose-Einstein condensates of ultracold gases, superfluid 4He is a very dense liquid of strongly…
We present static and dynamical properties of linear vortices in 4He droplets obtained from Density Functional calculations. By comparing the adsorption properties of different atomic impurities embedded in pure droplets and in droplets…
Superfluidity, liquid flow without friction, is familiar in helium. The first evidence for "supersolidity", its analogue in quantum solids, came from recent torsional oscillator (TO) measurements involving 4-He. At temperatures below 200…
Molecular nanomagnets are among the first examples of spin systems of finite size and have been test-beds for addressing a range of elusive but important phenomena in quantum dynamics. In fact, for short-enough timescales the spin…
We present neutron scattering results for the dynamic response by superfluid and normal-fluid 4He and the results of a simple perturbation-theory analysis which allows us to describe all aspects of the observed behavior by considering only…
Path Integral Monte Carlo calculations of the superfluid density throughout ^4He droplets doped with linear impurities (HCN)_n are presented. After deriving a local estimator for the superfluid density distribution, we find a decreased…
The possibility of a supersolid state of matter, i.e., a crystalline solid exhibiting superfluid properties, first appeared in theoretical studies about forty years ago. After a long period of little interest due to the lack of experimental…
The superfluid response of nanoscale size quasi-2D He-4 droplets adsorbed on a graphite substrate is investigated by computer simulations. It is found that clusters comprising as few as 7 atoms are stable at temperatures lower than < 0.15…
Using Path Integral Monte Carlo we calculate exchange frequencies in bulk hcp 4He as atoms undergo ring exchange. We fit the frequencies to a lattice model and examine whether such atoms could become a supersolid, that is have a…
We investigate the spreading of 4He droplets on alkali surfaces at zero temperature, within the frame of Finite Range Density Functional theory. The equilibrium configurations of several 4He_N clusters and their asymptotic trend with…
Superfluids, such as superfluid $^3\mathrm{He}$ and $^4\mathrm{He}$, exhibit a broad range of quantum phenomena and excitations which are unique to these systems. Nanoscale mechanical resonators are sensitive and versatile force detectors…
We present a superfluid hydrodynamic model for the increase in moment of inertia, $\Delta I$, of molecules rotating in liquid $^4$He. The static inhomogeneous He density around each molecule (calculated using the Orsay-Paris liquid $^4$He…
A significant fraction of superfluid helium nanodroplets produced in a free-jet expansion have been observed to gain high angular momentum resulting in large centrifugal deformation. We measured single-shot diffraction patterns of…
We have studied the appearance of vortex arrays in a rotating helium-4 nanodroplet at zero temperature within density functional theory. Our results are compared with those for classical rotating fluid drops used to analyze the shape and…
A density functional theory is used to investigate the instability arising in superfluid $^4$He as it flows at velocity u just above the Landau critical velocity of rotons v_c. Confirming an early theoretical prediction by one of us [JETP…
$^4$He nanodroplets doped with an alkali ion feature a snowball of crystallized layers surrounded by superfluid helium. For large droplets, we predict that a transitional supersolid layer can form, bridging between the solid core and the…
A superfluid having atomic scale superflow of a hexagonal lattice of vortex and antivortex filaments, described by a single macroscopic wave function is presented as a supersolid. As superfluid \he4 is pressurized, at a first order…
Purely rotational transitions of a molecule, such as HCCCN, embedded in large $^4$He clusters have been detected for the first time. The saturation behavior shows that, in contrast to previous expectations, the microwave line profiles are…