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We report an optical memory in a rare earth doped crystal with long storage times, up to 20 ms, together with an optical bandwidth of 1.5 MHz. This is obtained by transferring optical coherences to nuclear spin coherences, which were then…

Quantum Physics · Physics 2016-07-14 Marko Lovrić , Alban Ferrier , Dieter Suter , Philippe Goldner

Silicon is undoubtedly one of the most promising semiconductor materials for spin-based information processing devices. Its highly advanced fabrication technology facilitates the transition from individual devices to large-scale processors,…

Rare earth doped crystals are promising systems for quantum information processing. In particular paramagnetic rare earths could be used to build coherent interfaces with optical and microwave photons. In addition, isotopes with non zero…

Materials Science · Physics 2016-10-19 Sacha Welinski , Alban Ferrier , Mikael Afzelius , Philippe Goldner

Rare-earth doped crystals have long coherence times and the potential to provide quantum interfaces between microwave and optical photons. Such applications benefit from a high cooperativity between the spin ensemble and a microwave cavity…

Interfacing between various elements of a computer - from memory to processors to long range communication - will be as critical for quantum computers as it is for classical computers today. Paramagnetic rare earth doped crystals, such as…

Mapping the physical dipolar Hamiltonian of a solid-state network of nuclear spins onto a system of nearest-neighbor couplings would be extremely useful for a variety of quantum information processing applications, as well as NMR structural…

We explore spin dynamics of isotopically purified $^{166}$Er:$^{7}$LiYF$_4$ crystal below 1 Kelvin and at weak magnetic fields $<$0.3 T. Crystals grown in our lab demonstrate record-narrow inhomogeneous optical broadening down to 16~MHz.…

We investigate the relevant spectroscopic properties of the 795 nm $^3$H$_6$$\leftrightarrow$$^3$H$_4$ transition in 1% Tm$^{3+}$:Y$_3$Ga$_5$O$_{12}$ at temperatures as low as 1.2 K for optical quantum memories based on persistent spectral…

Quantum Physics · Physics 2014-10-23 Charles W. Thiel , Neil Sinclair , Wolfgang Tittel , Rufus L. Cone

Erbium-doped solids are prime candidates for optical quantum communication networks due to erbium's telecom C-band emission. A long-lived electron spin of erbium with millisecond coherence time is highly desirable for establishing…

Quantum Physics · Physics 2023-10-16 Shobhit Gupta , Xuntao Wu , Haitao Zhang , Jun Yang , Tian Zhong

Rare-earth ion doped crystals are state-of-the-art platforms for processing quantum information, particularly thanks to their excellent optical and spin coherence properties at cryogenic temperatures. Experimental observations have shown…

We characterize the 795 nm $^3$H$_6$ to $^3$H$_4$ transition of Tm$^{3+}$ in a Ti$^{4+}$:LiNbO$_{3}$ waveguide at temperatures as low as 800 mK. Coherence and hyperfine population lifetimes -- up to 117 $\mu$s and 2.5 hours, respectively --…

Quantum Physics · Physics 2017-03-21 Neil Sinclair , Daniel Oblak , Charles W. Thiel , Rufus L. Cone , Wolfgang Tittel

We investigate the potential for optical quantum technologies of Pr3+:Y2O3 in the form of monodisperse spherical nanoparticles. We measured optical inhomogeneous lines of 27 GHz, and optical homogeneous linewidths of 108 kHz and 315 kHz in…

Quantum Physics · Physics 2019-10-09 D. Serrano , C. Deshmukh , S. Liu , A. Tallaire , A. Ferrier , H. de Riedmatten , P. Goldner

We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is…

Elucidating the factors limiting quantum coherence in real materials is essential to the development of quantum technologies. Here we report a strategic approach to determine the effect of lattice dynamics on spin coherence lifetimes using…

Ultracold polar molecules (UPMs) are emerging as a novel and powerful platform for fundamental applications in quantum science. Here, we report characterization of the coherence between nuclear spin levels of ultracold ground-state…

Atomic Physics · Physics 2022-06-15 Junyu Lin , Junyu He , Mucan Jin , Guanghua Chen , Dajun Wang

Quantum memories for light will be essential elements in future long-range quantum communication networks. These memories operate by reversibly mapping the quantum state of light onto the quantum transitions of a material system. For…

Quantum Physics · Physics 2018-04-27 Miloš Rančić , Morgan P. Hedges , Rose L. Ahlefeldt , Matthew J. Sellars

Solid-state impurity spins with optical control are currently investigated for quantum networks and repeaters. Among these, rare-earth-ion doped crystals are promising as quantum memories for light, with potentially long storage time, high…

Er$^{3+}$$:$Y$_2$SiO$_5$ is a material of particular interest due to its suitability for telecom-band quantum memories and quantum transducers interfacing optical communication with quantum computers working in the microwave regime.…

Quantum Physics · Physics 2022-06-28 Jian-Yin Huang , Pei-Yun Li , Zong-Quan Zhou , Chuan-Feng Li , Guang-Can Guo

Spins in silicon that are accessible via a telecom-compatible optical transition are a versatile platform for quantum information processing that can leverage the well-established silicon nanofabrication industry. Key to these applications…

Rovibrational energies, wave functions, and Raman transition moments are reported for the lowest-energy states of the H$_3^+$ molecular ion including the magnetic couplings of the proton spins and molecular rotation in the presence of a…

Chemical Physics · Physics 2024-10-29 Gustavo Avila , Ayaki Sunaga , Stanislav Komorovsky , Edit Matyus