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Praseodymium (Pr$^{3+}$) ions doped in the site 1 of yttrium orthosilicate (Y$_2$SiO$_5$) has been widely employed as the photonic quantum memory due to their excellent optical coherence and spin coherence. While praseodymium ions occupying…

Quantum Physics · Physics 2020-05-26 Yi-Xin Xiao , Zong-Quan Zhou , Yu Ma , Tian-Shu Yang , You-Zhi Ma , Chuan-Feng Li , Guang-Can Guo

The spin coherence time of $^{151}$Eu$^{3+}$ which substitutes the yttrium at site 1 in Y$_2$SiO$_5$ crystal has been extended to 6 hours in a recent work [\textit{Nature} \textbf{517}, 177 (2015)]. To make this long-lived spin coherence…

Rare-earth ions doped in crystals with low nuclear-spin densities are highly promising candidates for quantum technology applications. In this study, we investigated the spectroscopic properties of the 7F0 - 5 D0 optical and the hyperfine…

Materials Science · Physics 2025-04-15 Xiantong An , Weiye Sun , Zhehao Xu , Wanting Xiao , Miaomiao Ren , Mucheng Guo , Shuping Liu , Fudong Wang , Manjin Zhong

In this letter we present a method for increasing the coherence time of praseodymium hyperfine ground state transitions in Pr^3+:Y_2SiO_5 by the application of a specific external magnetic field. The magnitude and angle of the external…

Quantum Physics · Physics 2009-11-10 E. Fraval , M. J. Sellars , J. J. Longdell

In many important situations the dominant dephasing mechanism in cryogenic rare-earth-ion doped systems is due to magnetic field fluctuations from spins in the host crystal. Operating at a magnetic field where a transition has a zero…

Atomic Physics · Physics 2015-06-03 D. L. McAuslan , J. G. Bartholomew , M. J. Sellars , J. J. Longdell

Optically addressable spins are actively investigated in quantum communication, processing and sensing. Optical and spin coherence lifetimes, which determine quantum operation fidelity and storage time, are often limited by spin-spin…

We report the measurement of the inhomogeneous linewidth, homogeneous linewidth and spin state lifetime of Pr3+ ions in a novel waveguide architecture. The TeO2 slab waveguide deposited on a bulk Pr3+:Y2SiO5 crystal allows the 3H4 - 1D2…

Quantum Physics · Physics 2015-07-17 Sara Marzban , John G. Bartholomew , Stephen Madden , Khu Vu , Matthew J. Sellars

Rare-earth-doped crystals are excellent hardware for quantum storage of optical information. Additional functionality of these materials is added by their waveguiding properties allowing for on-chip photonic networks. However, detection and…

Quantum Physics · Physics 2014-05-22 P. Siyushev , K. Xia , R. Reuter , M. Jamali , N. Zhao , N. Yang , C. Duan , N. Kukharchyk , A. D. Wieck , R. Kolesov , J. Wrachtrup

A thulium-doped crystal is experimentally shown to be an excellent candidate for broadband quantum storage in a solid-state medium. For the first time, nuclear spin coherence is optically excited, detected and characterized in such a…

We characterize the Europium (Eu$^{3+}$) hyperfine interaction of the excited state ($^5$D$_0$) and determine its effective spin Hamiltonian parameters for the Zeeman and quadrupole tensors. An optical free induction decay method is used to…

We experimentally investigate the coherence properties of a qubit stored in the Zeeman substates of the 5S1/2, F=1 hyperfine ground level of a single optically trapped Rb-87 atom. Larmor precession of a single atomic spin-1 system is…

Quantum Physics · Physics 2015-05-28 Wenjamin Rosenfeld , Jürgen Volz , Markus Weber , Harald Weinfurter

Rare-earth ion doped crystals are promising systems for quantum communication and quantum information processing. In particular, paramagnetic rare-earth centres can be utilized to realize quantum coherent interfaces simultaneously for…

Efficient and reversible optical to microwave coherent transducers are required to enable entanglement transfer between superconducting qubits and light for quantum networks. Rare-earth-doped crystals that possess narrow optical and spin…

Erbium ions doped into crystals have unique properties for quantum information processing, because of their optical transition at 1.5 $\mu$m and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most…

Optically addressable solid-state spins have been extensively studied for quantum technologies, offering unique advantages for quantum computing, communication, and sensing. Advancing these applications is generally limited by finding…

Rare earth ions (REI) in solid materials are among the leading systems for quantum technology applications. However, developing practical REI quantum devices with long-lived coherent states remains challenging due to great growth…

We present a comprehensive study of spin relaxation dynamics at cryogenic temperatures in a rare-earth-doped crystal used for quantum memory applications: $^{171}$Yb:Y$_2$SiO$_5$. Spin relaxation is indeed a major limiting factor for both…

We characterize the optical coherence and energy-level properties of the 795 nm $^3$H$_6$ to $^3$H$_4$ transition of Tm$^{3+}$ in a Ti$^{4+}$:LiNbO$_{3}$ waveguide at temperatures as low as 0.65 K. Coherence properties are measured with…

Rare-earth ions are characterised by transitions with very narrow linewidths even in solid state crystals. Exceedingly long coherence times have been shown on both spin and optical transitions of rare-earth-ion doped crystals. A key factor,…

An experimental platform of ultralow-temperature pulsed ENDOR (electron-nuclear double resonance) spectroscopy is constructed for the bulk materials. Coherent property of the coupled electron and nuclear spins of the rare-earth (RE) dopants…

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