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We report the design of an angular array of electron Time-of-Flight (eToF) spectrometers intended for non-invasive spectral, temporal, and polarization characterization of single shots of high-repetition rate, quasi-continuous,…

The quest for mapping the femtosecond dynamics of the electronic band structure of complex materials via Time- and Angle-Resolved Photoelectron Spectroscopy (TR-ARPES) over their full First Brillouin Zone is pushing the development of…

The paper describes a time- and angle-resolved photoemission apparatus consisting of a hemispherical analyzer and a pulsed laser source. We demonstrate 1.48-eV pump and 5.90-eV probe measurements at the >10.5-meV and >240-fs resolutions by…

Materials Science · Physics 2016-12-16 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Kiss , T. Otsu , Y. Kobayashi , S. Shin

A laser-based angle resolved photoemission (APRES) system utilizing 6 eV photons from the fourth harmonic of a mode-locked Ti:sapphire oscillator is described. This light source greatly increases the momentum resolution and photoelectron…

Other Condensed Matter · Physics 2007-06-08 J. D. Koralek , J. F. Douglas , N. C. Plumb , J. D. Griffith , S. T. Cundiff , H. C. Kapteyn , M. M. Murnane , D. S. Dessau

We describe a setup of time-, spin-, and angle-resolved photoemission spectroscopy (tr-SARPES) employing a 10.7-eV ($\lambda$=115.6 nm) pulse laser at 1-MHz repetition rate as a probe photon source. This equipment effectively combines…

Time- and angle-resolved photoelectron spectroscopy (trARPES) employing a 500 kHz extreme-ultravioled (XUV) light source operating at 21.7 eV probe photon energy is reported. Based on a high-power ytterbium laser, optical parametric chirped…

Instrumentation and Detectors · Physics 2019-02-14 M. Puppin , Y. Deng , C. W. Nicholson , J. Feldl , N. B. M. Schroeter , H. Vita , P. S. Kirchmann , C. Monney , L. Rettig , M. Wolf , R. Ernstorfer

We present the development of a time- and angle-resolved photoemission spectroscopy based on a Yb-based femtosecond laser and a hemispherical electron analyzer. The energy of the pump photon is tunable between 1.4 and 1.9 eV, and the pulse…

Strongly Correlated Electrons · Physics 2020-03-03 Yuanyuan Yang , Tianwei Tang , Shaofeng Duan , Chaocheng Zhou , Duxing Hao , Wentao Zhang

We developed a table-top vacuum ultraviolet (VUV) laser with $113.778$nm wavelength (10.897eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond…

Efforts to push the spatiotemporal imaging-resolution limits of femtosecond (fs) laser-driven ultrafast electron microscopes (UEMs) to the combined angstrom-fs range will benefit from stable sources capable of generating high bunch charges.…

Materials Science · Physics 2024-09-25 Jialiang Chen , Simon A. Willis , David J. Flannigan

The Time-of-Flight (ToF) technique coupled with semiconductor-like detectors, as silicon carbide and diamond, is one of the most promising diagnostic methods for high-energy, high repetition rate, laser-accelerated ions allowing a full…

Performing time and angle resolved photoemission spectroscopy (tr-ARPES) at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite recent advances, HHG-based…

Photoelectron momentum microscopy is an emerging powerful method for angle-resolved photoelectron spectroscopy (ARPES), especially in combination with imaging spin filters. These instruments record kx-ky images, typically exceeding a full…

Applied Physics · Physics 2021-02-03 G. Schoenhense , S. Babenkov , D. Vasilyev , H. -J. Elmers , K. Medjanik

The development of extreme ultraviolet sources is critical for advancing angleresolved photoemission spectroscopy (ARPES), a powerful technique for probing the electronic structure of materials. Here, we report the construction of a…

The small time gap of synchrotron radiation in conventional multi-bunch mode (100-500MHz) is prohibitive for time-of-flight (ToF) based electron spectroscopy. Even the new generation of delay-line detectors with improved time resolution…

Time-Of-Flight (TOF) methods are very effective to detect particles accelerated in laser-plasma interactions, but they shows significant limitations when used in experiments with high energy and intensity lasers, where both high-energy ions…

We report on spectroscopy and time-of-flight measurements using an 18 keV fast-pulsed photoelectron source of adjustable intensity, ranging from single photoelectrons per pulse to 5 photoelectrons per microsecond at pulse repetition rates…

Instrumentation and Detectors · Physics 2009-06-19 K. Valerius , M. Beck , H. Arlinghaus , J. Bonn , V. M. Hannen , H. Hein , B. Ostrick , S. Streubel , Ch. Weinheimer , M. Zboril

We present a detailed exposition of the design for time- and angle-resolved photoemission spectroscopy using a UV probe laser source that combines the nonlinear effects of \b{eta}-BaB2O4 and KBe2BO3F2 optical crystals. The photon energy of…

Mesoscale and Nanoscale Physics · Physics 2023-10-13 Mojun Pan , Junde Liu , Famin Chen , Ji Wang , ChenXia Yun , Tian Qian

In photoelectron spectroscopy, the measured electron momentum range is intrinsically related to the excitation photon energy. Low photon energies $<10$ eV are commonly encountered in laser-based photoemission and lead to a momentum range…

A novel detector based on a polycrystalline diamond sensor is here employed in an advanced Time-Of-Flight scheme for the characterization of energetic ions accelerated during laser-matter interactions. The optimization of the detector and…

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