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We describe a spin-resolved electron spectrometer capable of uniquely efficient and high energy resolution measurements. Spin analysis is obtained through polarimetry based on low-energy exchange scattering from a ferromagnetic thin-film…

Materials Science · Physics 2014-11-21 C. Jozwiak , J. Graf , G. Lebedev , N. Andresen , A. K. Schmid , A. V. Fedorov , F. El Gabaly , W. Wan , A. Lanzara , Z. Hussain

We report a novel approach for coherent multi-photon photoemission band mapping of the entire Brillouin zone with infrared light that is readily implemented in a laboratory setting. We excite a solid state material, Ag(110), with intense…

Other Condensed Matter · Physics 2020-08-31 Andi Li , Namitha Ann James , Tianyi Wang , Zehua Wang , Hrvoje Petek , Marcel Reutzel

A system based on commercially available items, such as a laser diode, emitting in the visible range $\sim 400$ nm,and multimode fiber patches, fused fiber splitters and optical switches may be assembled,for time calibration of…

Instrumentation and Detectors · Physics 2016-06-01 M. Bonesini , R. Bertoni , A. deBari , M. Rossella

Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present…

A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond…

Since its inception, velocity map imaging (VMI) has been a powerful tool for measuring the 2D momentum distribution of photoelectrons generated by strong laser fields. There has been continued interest in expanding it into 3D measurements…

A 790-nm-driven high-harmonic generation source with a repetition rate of 6 kHz is combined with a toroidal-grating monochromator and a high-detection-efficiency photoelectron time-of-flight momentum microscope to enable time- and…

Here we present a high repetition rate, narrow band-width, extreme ultraviolet (XUV) photon source for time- and angle-resolved photoemission spectroscopy (tr-ARPES). The narrow band width pulses $\Delta E=9, 14, 18$ meV for photon energies…

We demonstrate the implementation of a simple time-of-flight (ToF) mass spectrometer with medium-mass resolution ($m/\Delta m\sim50$) geared towards the demands of atomic, molecular, and chemical physics experiments. By utilizing a novel…

Angle-resolved photoemission spectroscopy (ARPES) provides a direct access to the electronic band structure of solid and molecular systems. The momentum range accessible by this technique depends directly on the photon energy used, and…

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

Time and angle-resolved photoemission spectroscopy (trARPES) allows direct mapping of the electronic band structure and its dynamic response on femtosecond timescales. Here, we present a new ARPES system, powered by a new fiber-based…

A time-of-flight (ToF) imaging system is proposed and its working principle demonstrated. To realize this system, a new device, a free-space optical mixer, is designed and fabricated. A scene is illuminated (flashed) with a megahertz level…

We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire…

Materials Science · Physics 2025-02-11 Takeshi Suzuki , Yigui Zhong , Kecheng Liu , Teruto Kanai , Jiro Itatani , Kozo Okazaki

We have realized a high-resolution time-of-flight mass spectrometer combined with a magneto-optical trap. The spectrometer enables excellent optical access to the trapped atomic cloud using specifically devised acceleration and deflection…

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced…

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes the electron optics allows imaging of the image plane, momentum plane, or…

We present proof-of-principle experiments of stroboscopic time-of-flight (TOF) neutron diffraction in long pulsed magnetic fields. By utilizing electric double-layer capacitors, we developed a long pulsed magnet for neutron diffraction…

The design and performance of the first vacuum ultra-violet (VUV) laser-based angle-resolved photoemission (ARPES) system are described. The VUV laser with a photon energy of 6.994 eV and bandwidth of 0.26 meV is achieved from the second…