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We present the results of a muon-spin relaxation (muSR) investigation into magnetic ordering in several families of layered quasi-two-dimensional molecular antiferromagnets based on transition metal ions such as S=1/2 Cu2+ bridged with…

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

muSR experiments on the geometrically frustrated spinel oxide, Li2Mn2O4, show the development of spin correlations over a range of length scales with decreasing temperature. Increased relaxation below 150 K is consistent with the onset of…

Strongly Correlated Electrons · Physics 2009-11-11 C. R. Wiebe , P. L. Russo , A. T. Savici , Y. J. Uemura , G. J. MacDougall , G. M. Luke , S. Kuchta , J. E. Greedan

We report muon spin relaxation measurements on two Ti3+ containing perovskites, LaTiO3 and YTiO3, which display long range magnetic order at low temperature. For both materials, oscillations in the time-dependence of the muon polarization…

Strongly Correlated Electrons · Physics 2009-11-13 P. J. Baker , T. Lancaster , S. J. Blundell , W. Hayes , F. L. Pratt , M. Itoh , S. Kuroiwa , J. Akimitsu

Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility \chi_ ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements on…

We present an experimental study of the pyrochlore coumpound Nd2Zr2O7 by means of neutron scattering and magnetization measurements down to 90 mK. The Nd$^{3+}$ magnetic moments exhibit a strong local $\langle$111$\rangle$ Ising anisotropy…

Strongly Correlated Electrons · Physics 2016-01-05 E. Lhotel , S. Petit , S. Guitteny , O. Florea , M. Ciomaga Hatnean , C. Colin , E. Ressouche , M. R. Lees , G. Balakrishnan

We report results of magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements on the polycrystalline Ba$_6$Nd$_2$Ti$_4$O$_{17}$, a disorder-free triangular-lattice antiferromagnet. The absence of long-range…

Strongly Correlated Electrons · Physics 2024-11-21 C. Y. Jiang , B. L. Chen , K. W. Chen , J. C. Jiao , Y. Wang , Q. Wu , N. Y. Zhang , M. Y. Zou , P. -C. Ho , O. O. Bernal , L. Shu

The magnetic ground state of single crystalline RuO$_2$ was investigated by the muon spin rotation/relaxation ($\mu$SR) experiment. The spin precession signal due to the spontaneous internal magnetic field $B_{\rm loc}$, which is expected…

Strongly Correlated Electrons · Physics 2024-04-19 M. Hiraishi , H. Okabe , A. Koda , R. Kadono , T. Muroi , D. Hirai , Z. Hiroi

We report on the electron spin resonance (ESR), heat capacity, magnetization, nuclear magnetic resonance (NMR), magnetic circular and linear dichroism (XMCD, XMLD), as well as the electrical resistivity of EuMn$_{2}$P$_{2}$ single crystals.…

In this study, we performed powder neutron diffraction and inelastic scattering measurements of frustrated pyrochlore Nd$_2$Ir$_2$O$_7$, which exhibits a metal-insulator transition at a temperature $T_{\rm MI}$ of 33 K. The diffraction…

Strongly Correlated Electrons · Physics 2012-02-29 K. Tomiyasu , K. Matsuhira , K. Iwasa , M. Watahiki , S. Takagi , M. Wakeshima , Y. Hinatsu , M. Yokoyama , K. Ohoyama , K. Yamada

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at…

Strongly Correlated Electrons · Physics 2015-06-11 Songrui Zhao , P. Dalmas de R/'eotier , A. Yaouanc , D. E. MacLaughlin , J. M. Mackie , O. O. Bernal , Y. Nambu , T. Higo , S. Nakatsuji

We have studied the spin liquid Tb$\_2$Sn$\_2$O$\_7$ by neutron diffraction and specific heat measurements. Below about 2 K, the magnetic correlations change from antiferromagnetic to ferromagnetic. Magnetic order settles in two steps, with…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apeteri , J. Rodriguez-Carvajal , P. Bonville , A. Forget , D. Colson , V. Glazkov , J. P. Sanchez , O. Isnard , E. Suard

R$_2$Mo$_2$O$_7$ compounds show a ferromagnetic metal-insulator spin glass transition tuned by the radius of the rare earth ion R$^{3+}$. We have studied Gd$_2$Mo$_2$O$_7$ located on the verge of the transition, by neutron diffraction on a…

Strongly Correlated Electrons · Physics 2007-05-23 I. Mirebeau , A. Apetrei , I. Goncharenko , D. Andreica , P. Bonville , J. P. Sanchez , A. Amato , E. Suard , W. A. Crichton

High resolution X-ray scattering measurements on single crystal Tb2Ti2O7 reveal finite structural correlations at low temperatures. This geometrically frustrated pyrochlore is known to exhibit a spin liquid, or cooperative paramagnetic…

Disordered Systems and Neural Networks · Physics 2009-11-13 J. P. C. Ruff , B. D. Gaulin , J. P. Castellan , K. C. Rule , J. P. Clancy , J. Rodriguez , H. A. Dabkowska

We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $\rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with…

Strongly Correlated Electrons · Physics 2022-08-11 A. Scheie , M. Sanders , Yiming Qiu , T. R. Prisk , R. J. Cava , C. Broholm

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

Non-Fermi liquid behavior in some fermionic systems have attracted significant interest in last few decades. Certain pyrochlore iridates with stronger spin-orbit coupling strength have recently been added to the list. Here, we provide…

Strongly Correlated Electrons · Physics 2022-01-03 Md Salman Khan , Ilaria Carlomagno , Carlo Meneghini , P. K. Biswas , Fabrice Bert , Subham Majumdar , Sugata Ray

We report a resonant inelastic X-ray scattering study on a single crystal of a non-stoichiometric pyrochlore iridate Tb$_{2+x}$Ir$_{2-x}$O$_{7-y}$ ($x \simeq 0.25$) that magnetically orders at $T_{\rm{N}}\simeq 50$ K. We find that the…

Strongly Correlated Electrons · Physics 2024-09-18 Q. Faure , A. Toschi , J. R. Soh , E. Lhotel , B. Detlefs , D. Prabhakaran , D. F. McMorrow , C. J. Sahle

When the transition temperature of a continuous phase transition is tuned to absolute zero, new ordered phases and physical behaviour emerge in the vicinity of the resulting quantum critical point. Sr3Ru2O7 can be tuned through quantum…

Strongly Correlated Electrons · Physics 2021-10-25 C. Lester , S. Ramos , R. S. Perry , T. P. Croft , M. Laver , R. I. Bewley , T. Guidi , A. Hiess , A. Wildes , E. M. Forgan , S. M. Hayden

We present a muon-spin relaxation investigation of the Ising chain magnet Ca_{3}Co_{2-x}Mn_{x}O_{6} (x~0.95). We find dynamic spin fluctuations persisting down to the lowest measured temperature of 1.6 K. The previously observed transition…

Strongly Correlated Electrons · Physics 2009-08-27 T. Lancaster , S. J. Blundell , P. J. Baker , H. J. Lewtas , W. Hayes , F. L. Pratt , H. T. Yi , S. -W. Cheong