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Related papers: Real Space Green's Function Approach to RIXS

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We study resonant inelastic x-ray scattering (RIXS) peaks corresponding to low energy particle-hole excited states of metallic FeTe and semi-metallic TiSe$_2$ for photon incident energy tuned near the $L_{3}$ absorption edge of Fe and Ti…

Materials Science · Physics 2014-07-04 B. Barbiellini , J. N. Hancock , C. Monney , Y. Joly , G. Ghiringhelli , L. Braicovich , T. Schmitt

Recent improvements in instrumentation have established resonant inelastic x-ray scattering (RIXS) as a valuable new probe of the magnetic excitations in the cuprates. This article introduces RIXS, focusing on the Cu $L_3$ resonance, and…

Superconductivity · Physics 2015-02-17 M. P. M. Dean

We study the magnetic excitations in 5d transition-metal oxide Sr$_2$IrO$_4$ on the basis of the Heisenberg model with small anisotropic terms on a square lattice. We calculate the correlation functions by using the Green's functions in the…

Strongly Correlated Electrons · Physics 2015-06-18 Jun-ichi Igarashi , Tatsuya Nagao

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

Generic low-energy spectral features related to $d$-$d$ excitations in nearly cubic vanadium perovskites are predicted for the expected $L$-edge resonant inelastic X-ray scattering (RIXS) measurements. Model Hamiltonian describing local…

Strongly Correlated Electrons · Physics 2013-01-22 V. Yushankhai , L. Siurakshina

We theoretically demonstrate that a resonant inelastic x-ray scattering (RIXS) with a sizable momentum transfer can be utilized to study valence band dispersion for broad band materials. We take RIXS at the Si K edge of 3C-SiC as a typical…

Materials Science · Physics 2009-09-21 Yunori Nisikawa , Muneharu Ibuki , Manabu Usuda

We present a computational study of $L$-edge resonant inelastic x-ray scattering (RIXS) in correlated 3$d$ transition-metal oxides using an $ab$ $initio$ method based on local density approximation + dynamical mean-field theory (DMFT). The…

Strongly Correlated Electrons · Physics 2020-03-25 Atsushi Hariki , Mathias Winder , Takayuki Uozumi , Jan Kuneš

Closed expressions are derived for resonant multidimensional X-ray spectroscopy using the quasiparticle nonlinear exciton representation of optical response. This formalism is applied to predict coherent four wave mixing signals which probe…

Strongly Correlated Electrons · Physics 2015-05-13 U. Harbola , S. Mukamel

A two-dimensional resonant inelastic x-ray scattering (2D-RIXS) microscopy system has been developed at the beamline BL02U of NanoTerasu. The instrument combines a Wolter type-I mirror for spatial imaging with a varied-line-spacing grating…

Materials Science · Physics 2026-05-07 Kohei Yamamoto , Hakuto Suzuki , Jun Miyawaki

A Green's function approach to the inclusive quasielastic ($e,e'$) scattering is presented. The components of the nuclear response are written in terms of the single-particle optical model Green's function. The explicit calculation of the…

Nuclear Theory · Physics 2007-05-23 F. Capuzzi , C. Giusti , A. Meucci , F. D. Pacati

Inelastic losses in core level x-ray spectra arise from many-body excitations, leading to broadening and damping as well as satellite peaks in x-ray photoemission (XPS) and x-ray absorption (XAS) spectra. Here we present a practical…

Materials Science · Physics 2016-08-17 J. J. Kas , J. J. Rehr , J. B. Curtis

Intrinsic inelastic losses in x-ray spectra originate from excitations in an interacting electron system due to a suddenly created core-hole. These losses characterize the features observed in x-ray photoemission spectra (XPS), as well Here…

Other Condensed Matter · Physics 2023-03-08 J. J. Kas , J. J. Rehr

We present an ab initio study of neutral core and valence electronic excitations in {\alpha}-Al2O3 by solving the Bethe-Salpeter equation (BSE) of many-body perturbation theory within an all-electron framework. Calculated spectra at the Al…

Materials Science · Physics 2024-01-26 M. Laura Urquiza , Matteo Gatti , Francesco Sottile

Using a model Hamiltonian, we discuss how we could interpret data obtained from transition metal $K$-edge resonant inelastic x-ray scattering (RIXS) experiments. By analyzing the creation of valence excitations from the screening of the…

Materials Science · Physics 2008-08-08 K. H. Ahn , A. J. Fedro , Michel van Veenendaal

We investigate resonant inelastic X-ray scattering (RIXS) at the O $K$-edge in insulating cuprates by means of three methods: cluster perturbation theory (CPT), Hartree--Fock approximation (HFA) and exact diagonalization (ED) method. We…

Strongly Correlated Electrons · Physics 2023-02-22 Yukihiro Matsubayashi , Sumio Ishihara

We present a theoretical investigation of the origin of Raman-like and fluorescencelike (FL) features of resonant inelastic x-ray scattering (RIXS) spectra. Using a combination of local-density approximation + dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2018-09-26 Atsushi Hariki , Mathias Winder , Jan Kuneš

We analyze resonant inelastic x-ray scattering (RIXS) at the Cu K edge in a typical orbital-ordered compound KCuF3 on the basis of a microscopic theory. Spectral shape and its dependence on polarization direction and momentum transfer of…

Strongly Correlated Electrons · Physics 2014-06-20 Takuji Nomura

We present an implementation of a damped response framework for calculating resonant inelastic X-ray scattering (RIXS) at the equation-of-motion coupled cluster singles and doubles (CCSD) and second-order approximate coupled cluster singles…

We derive general expressions for resonant inelastic x-ray scattering (RIXS) operators for $t_{2g}$ orbital systems, which exhibit a rich array of unconventional magnetism arising from unquenched orbital moments. Within the fast collision…

Strongly Correlated Electrons · Physics 2017-08-16 B. J. Kim , Giniyat Khaliullin

We develop a formalism to study indirect resonant inelastic x-ray scattering (RIXS) in systems with itinerant electrons, accounting for the attraction between valence electrons and the positively-charged core hole exactly, and apply this…

Strongly Correlated Electrons · Physics 2014-07-16 David Benjamin , Israel Klich , Eugene Demler