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Atomic nuclei can be spontaneously deformed into non-spherical shapes as many-nucleon systems. We discuss to what extent a similar deformation takes place in many-electron systems. To this end, we employ several many-body methods, such as…

Atomic Physics · Physics 2021-09-24 Tomoya Naito , Shimpei Endo , Kouichi Hagino , Yusuke Tanimura

We present detailed results of Unrestricted Hartree-Fock (UHF) calculations for up to eight electrons in a parabolic quantum dot. The UHF energies are shown to provide rather accurate estimates of the ground-state energy in the entire range…

Strongly Correlated Electrons · Physics 2009-11-10 Boris Reusch , Hermann Grabert

In this article, we consider the extended Kohn-Sham model for atoms subjected to cylindrically-symmetric external potentials. The variational approximation of the model and the construction of appropriate discretization spaces are detailed…

Mathematical Physics · Physics 2018-07-04 Eric Cancès , Nahia Mourad

We describe the code HFODD which solves the nuclear Skyrme-Hartree-Fock problem by using the deformed Cartesian harmonic oscillator basis. The user has a possibility of choosing among various symmetries of the nuclear HF problem for…

Nuclear Theory · Physics 2009-10-30 J. Dobaczewski , J. Dudek

We study atomic ground state energies for neutral atoms as the nuclear charge $Z$ is large in the no-pair formalism. We show that for a large class of projections defining the underlying Dirac sea -- covering not only the physical…

Mathematical Physics · Physics 2025-07-01 Long Meng , Heinz Siedentop

The ground and some excited states of the Li atom in external uniform magnetic fields are calculated by means of our 2D mesh Hartree-Fock method for field strengths ranging from zero up to 2.35 10^8 T. With increasing field strength the…

Atomic Physics · Physics 2009-10-31 M. V. Ivanov , P. Schmelcher

Starting from the relativistic form of the Bonn potential as a bare nucleon-nucleon interaction, the full Relativistic Brueckner-Hartree-Fock (RBHF) equations are solved for finite nuclei in a fully self-consistent basis. This provides a…

Nuclear Theory · Physics 2017-08-03 Shihang Shen , Haozhao Liang , Jie Meng , Peter Ring , Shuangquan Zhang

The Hartree-Fock equation admits homogeneous states that model infinitely many particles at equilibrium. We prove their asymptotic stability in large dimensions, under assumptions on the linearised operator. Perturbations are moreover…

Analysis of PDEs · Mathematics 2025-02-26 Charles Collot , Elena Danesi , Anne-Sophie de Suzzoni , Cyril Malézé

We study the Hartree-Fock model for pseudorelativistic atoms, that is, atoms where the kinetic energy of the electrons is given by the pseudorelativistic operator \sqrt{(pc)^2+(mc^2)^2}-mc^2. We prove the existence of a Hartree-Fock…

Mathematical Physics · Physics 2013-10-30 Anna Dall'Acqua , Thomas Østergaard Sørensen , Edgardo Stockmeyer

The Hartree-Fock states of the many-electron atomic system can be unstable with respect to a static or dynamic shift of the electron shells. An appropriate non-rigid shell model for atomic clusters is developed. It permits to formulate a…

Strongly Correlated Electrons · Physics 2009-10-30 A. S. Moskvin , V. A. Korotaev , Yu. D. Panov , M. A. Sidorov

We present a general scheme for treating the integrable singular terms within exact exchange (EXX) Kohn-Sham or Hartree-Fock (HF) methods for periodic solids. We show that the singularity corrections for treating these divergencies depend…

Materials Science · Physics 2009-11-11 Pierre Carrier , Stefan Rohra , Andreas Goerling

We compute the ground state energy of atoms and quantum dots with a large number N of electrons. Both systems are described by a non-relativistic Hamiltonian of electrons in a d-dimensional space. The electrons interact via the Coulomb…

Quantum Physics · Physics 2015-05-14 Hervé Kunz , Rico Rueedi

We study the behavior of Hartree-Fock (HF) solutions in the vicinity of conical intersections. These are here understood as regions of a molecular potential energy surface characterized by degenerate or nearly-degenerate eigenfunctions with…

Chemical Physics · Physics 2018-04-10 Lena C. Jake , Thomas M. Henderson , Gustavo E. Scuseria

We prove that the Hartree--Fock orbitals of pseudorelativistic atoms, that is, atoms where the kinetic energy of the electrons is given by the pseudorelativistic operator sqrt{-Delta+1}-1, are real analytic away from the origin. As a…

Mathematical Physics · Physics 2013-10-30 Anna Dall'Acqua , Søren Fournais , Thomas Østergaard Sørensen , Edgardo Stockmeyer

In this paper we study the Hartree-Fock type system as follows: \begin{equation*} \left\{ \begin{array}{ll} -\Delta u+u+\lambda \phi _{u,v}u=\left\vert u\right\vert ^{p-2}u+\beta \left\vert v\right\vert ^{\frac{p}{2}}\left\vert u\right\vert…

Analysis of PDEs · Mathematics 2023-09-28 Juntao Sun , Tsung-fang Wu

We prove the ionization conjecture within the Hartree-Fock theory of atoms. More precisely, we prove that, if the nuclear charge is allowed to tend to infinity, the maximal negative ionization charge and the ionization energy of atoms…

Mathematical Physics · Physics 2007-05-23 Jan Philip Solovej

We benchmark three standard approximations for the many-body problem -- the Hartree-Fock, projected Hartree-Fock, and random phase approximations -- against full numerical configuration-interaction calculations of the electronic structure…

Atomic Physics · Physics 2012-08-31 Micah D. Schuster , Calvin W. Johnson , Joshua T. Staker

The multiconfigurational time-dependent Hartree-Fock equations are discussed and solved for a one-dimensional model of the Helium atom. Results for the ground state energy and two-particle density as well as the absorption spectrum are…

Quantum Physics · Physics 2015-03-13 D. Hochstuhl , S. Bauch , M. Bonitz

We consider the ground state of the homogeneous electron gas and we prove that a Hartree-Fock solution, motivated by previous simulations, has lower energy than the Fermi gas in the large density limit. This solution is a metallic phase :…

Strongly Correlated Electrons · Physics 2008-07-08 F. Delyon , M. Duneau , B. Bernu , M. Holzmann

We demonstrate that unrestricted Hartree-Fock theory applied to electrons in a uniform potential has stable Wigner crystal solutions for $r_s \geq 1.44$ in two dimensions and $r_s \geq 4.5$ in three dimensions. The correlation energies of…

Materials Science · Physics 2009-10-01 J. R. Trail , M. D. Towler , R. J. Needs