Related papers: Molecular imaging with X-ray free electron lasers:…
Since the invention of the laser nonlinear effects such as filamentation, Rabi-cycling and collective emission have been explored in the optical regime leading to a wide range of scientific and industrial applications. X-ray free electron…
An important goal for any advanced X-ray FEL is an option for providing Fourier-limited X-ray pulses. In this way, no monochromator is needed in the experimental hall. Self-seeding is a promising approach to significantly narrow the SASE…
This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray Free-Electron Laser. We present results of…
Free-electron lasers have demonstrated their capability of generating intense attosecond X-ray pulses, which are the key to studying electron dynamics at their natural time scale and in specifically targeted electronic states, but come at…
We investigate the possibility of non-destructive electron diffraction imaging of a single molecule to determine its structure. The molecular specimen will be held on a free-standing sheet of graphene. Due to the high conductivity of…
The pioneering experiments of linear spectroscopy were performed using flames in the 1800s, but nonlinear optical measurements had to wait until lasers became available in the twentieth century. Because the nonlinear cross section of…
Plasma accelerators can generate ultra high brightness electron beams which open the door to light sources with smaller physical footprint and properties un-achievable with conventional accelerator technology. In this paper we show that…
High-intensity, ultrashort, fully coherent X-ray pulses hold great potential for advancing spectroscopic techniques to unprecedented levels. Here, we propose a novel scheme for generating high-brightness and femtosecond-scale soft X-ray…
This Letter of Intent describes LUXE (Laser Und XFEL Experiment), an experiment that aims to use the high-quality and high-energy electron beam of the European XFEL and a powerful laser. The scientific objective of the experiment is to…
A method is proposed to generate trains of few-cycle x-ray pulses from a Free-Electron Laser (FEL) amplifier via a compact 'afterburner' extension consisting of several few-period undulator sections separated by electron chicane delays.…
Measurements of the spatial and temporal coherence of single, femtosecond x-ray pulses generated by the first hard x-ray free-electron laser (FEL), the Linac Coherent Light Source (LCLS), are presented. Single shot measurements were…
Volume Free Electron Laser (VFEL) was proposed in [1-4]. It can operate in the wide spectral range from microwaves to X-rays. To simulate the processes which take place in VFEL the superradiance from a short electron pulse moving in a…
We discuss the theory and phenomenology of pair annihilation, within an ultra-short laser pulse, to a single photon. The signature of this process is the uni-directional emission of single photons with a fixed energy. We show that the cross…
A well-characterised wavefront is important for many X-ray free-electron laser (XFEL) experiments, especially for single-particle imaging (SPI), where individual bio-molecules randomly sample a nanometer-region of highly-focused femtosecond…
We have investigated multiphoton multiple ionization dynamics of argon and xenon atoms using a new x-ray free electron laser (XFEL) facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that highly charged…
X-ray fluorescence holography (XFH) is a method for obtaining diffraction-limited images of the local atomic structure around a given type of emitter. The reconstructed wave-field represents a distorted image of the scatterer electron…
The quantum mechanical motion of electrons in molecules and solids occurs on the sub-femtosecond timescale. Consequently, the study of ultrafast electronic phenomena requires the generation of laser pulses shorter than 1 fs and of…
To shorten the duration of x-ray pulses, we present a nonlinear optical technique using atoms with core-hole vacancies (core-hole atoms) generated by inner-shell photoionization. The weak Coulomb screening in the core-hole atoms results in…
Structure determination is a key application of XFELs and 4th generation synchrotron sources, particularly using the coherent and pulsed X-ray radiation from X-ray free-electron lasers (XFEL). Scientific interest focuses on understanding…
The all-optical synchronization systems used in various X-ray free-electron lasers (XFEL) such as the European XFEL observe the transient fields of passing electron bunches coupled into one or more pickups in the Bunch Arrival Time Monitors…