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One of the options for increasing longitudinal coherency of X-ray free electron lasers (XFELs) is their seeding with microbunched electron beam. Several schemes leading to significant amplitude of the beam bunching at X-ray wavelengths were…

Accelerator Physics · Physics 2012-07-23 Nikolai A. Yampolsky , Bruce E. Carlsten

The fluctuations of the longitudinal coherence length expected from the world's first hard X-ray Free Electron Laser, the Linac Coherent Light Source, are investigated. We analyze, on a shot-to-shot basis, series of power spectra generated…

Instrumentation and Detectors · Physics 2010-06-07 Sooheyong Lee , Zhirong Huang , Yuantao Ding , Paul Emma , Wojciech Roseker , Gerhard Gruebel , Aymeric Robert

We demonstrate a hard x-ray probe of laser-aligned small molecules. To align small molecules with optical lasers, high intensities at nonresonant wavelengths are necessary. We use 95 ps pulses focused to 40 mum from an 800 nm Ti:sapphire…

Free-electron lasers (FELs) operate at wavelengths from millimeter waves through hard x-rays. At x-ray wavelengths, FELs typically rely on self-amplified spontaneous emission (SASE). Typical SASE emission contains multiple temporal "spikes"…

Here we propose to exploit the low energy bandwidth, small wavelength and penetration power of ultrashort pulses from XFELs for resonant Small Angle Scattering (SAXS) on plasma structures in laser excited plasmas. Small angle scattering…

Plasma Physics · Physics 2016-03-09 Thomas Kluge , M. Bussmann , H. -K. Chung , C. Gutt , L. G. Huang , M. Zacharias , U. Schramm , T. E. Cowan

Modern Flash X-ray diffraction Imaging (FXI) acquires diffraction signals from single biomolecules at a high repetition rate from X-ray Free Electron Lasers (XFELs), easily obtaining millions of 2D diffraction patterns from a single…

Image and Video Processing · Electrical Eng. & Systems 2020-10-28 Jing Liu , Stefan Engblom , Carl Nettelblad

We propose and analyze a novel regenerative amplifier free electron laser (FEL) to produce fully coherent x-ray pulses. The method makes use of narrow-bandwidth Bragg crystals to form an x-ray feedback loop around a relatively short…

Accelerator Physics · Physics 2009-11-11 Zhirong Huang , Ronald D. Ruth

Advanced accelerator-based light sources such as free electron lasers (FEL) accelerate highly relativistic electron beams to generate incredibly short (10s of femtoseconds) coherent flashes of light for dynamic imaging, whose brightness…

Accelerator Physics · Physics 2024-07-19 Alexander Scheinker

Ultrafast electron diffraction and time-resolved serial crystallography are the basis of the ongoing revolution in capturing at the atomic level of detail the structural dynamics of molecules. However, most experiments employ the classical…

Resonant inelastic x-ray scattering (RIXS) is a well-established tool for studying electronic, nuclear and collective dynamics of excited atoms, molecules and solids. An extension of this powerful method to a time-resolved probe technique…

Chemical Physics · Physics 2015-11-03 Victor Kimberg , Nina Rohringer

Electron motion on the (sub-)femtosecond time scale constitutes the fastest response in many natural phenomena such as light-induced phase transitions and chemical reactions. Whereas static electron densities in single molecules can be…

A channel-cut Si(111) crystal with a channel width of 90 $\mu$m was developed for achieving reflection self-seeding in hard X-ray free-electron lasers (XFELs). With the crystal, a monochromatic seed pulse is produced from a broadband XFEL…

Instrumentation and Detectors · Physics 2018-11-06 Taito Osaka , Ichiro Inoue , Ryota Kinjo , Takashi Hirano , Yuki Morioka , Yasuhisa Sano , Kazuto Yamauchi , Makina Yabashi

The importance of investigating magnetized plasmas/solids in extreme conditions has grown over the last decades, particularly in the field of high energy density physics (HEDP), such as laboratory astrophysics and inertial confinement…

We present a theoretical justification for a method of extracting of supplementary information for the phase retrieval procedure taken from diffraction of fs-pulses from X-ray Free Electron Laser facilities. The approach is based on…

Materials Science · Physics 2015-02-18 A. Leonov , D. Ksenzov , A. Benediktovitch , I. Feranchuk , U. Pietsch

A barrier to realizing the potential of molecules for quantum information science applications is a lack of high-fidelity, single-molecule imaging techniques. Here, we present and theoretically analyze a general scheme for dispersive…

The new capacity of X-ray free-electron laser (XFEL) facilities to produce multi-color X-ray femtosecond pulses paves the way to explore ultrafast phenomena in matter induced by X-ray photons. In the present study, we exploit the site…

Chemical Physics · Physics 2020-01-08 S. Oberli , J. González-Vázquez , E. Rodríguez-Perelló , M. Sodupe , F. Martín , A. Picón

The current state of the art in structural biology is led by NMR, X-ray crystallography and TEM investigations. These powerful tools however all rely on averaging over a large ensemble of molecules. Here, we present an alternative concept…

Atomic and Molecular Clusters · Physics 2015-12-15 Tatiana Latychevskaia , Jean-Nicolas Longchamp , Conrad Escher , Hans-Werner Fink

Recent advancements in X-ray light sources at synchrotrons and X-ray free-electron lasers (XFELs) present exciting opportunities to probe molecular chirality using novel nonlinear spectroscopies with element-sensitivity. Circular dichroism…

Chemical Physics · Physics 2025-01-27 Yeonsig Nam , Majed Chergui , Linda Young , Jérémy R. Rouxel

We demonstrate that a common-line method can assemble a 3D oversampled diffracted intensity distribution suitable for high-resolution structure solution from a set of measured 2D diffraction patterns, as proposed in experiments with an…

Biomolecules · Quantitative Biology 2007-10-16 V. L. Shneerson , A. Ourmazd , D. K. Saldin

The last decade has shown the great potential that X-ray Free Electron Lasers (FEL) have to study High Energy Density (HED) physics. Experiments at FELs have made significant breakthroughs in Shock Physics and Dynamic Diffraction, Dense…

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