Attosecond Inner-Shell Lasing at Angstrom Wavelengths
Abstract
Since the invention of the laser nonlinear effects such as filamentation, Rabi-cycling and collective emission have been explored in the optical regime leading to a wide range of scientific and industrial applications. X-ray free electron lasers (XFELs) have led to the extension of many optical techniques to X-rays for their advantages of angstrom scale spatial resolution and elemental specificity. One such example is XFEL driven population inversion of 1s core hole states resulting in inner-shell K (2p to 1s) X-ray lasing in elements ranging from neon to copper, which has been utilized for nonlinear spectroscopy and development of next generation X-ray laser sources. Here we show that strong lasing effects, similar to those observed in the optical regime, can occur at 1.5 to 2.1 angstrom wavelengths during high intensity (> W/cm) XFEL driven inner-shell lasing and superfluorescence of copper and manganese. Depending on the temporal substructure of the XFEL pump pulses(containing - photons) i, the resulting inner-shell X-ray laser pulses can exhibit strong spatial inhomogeneities as well as spectral splitting, inhomogeneities and broadening. Through 3D Maxwell Bloch theory we show that the observed spatial inhomogeneities result from X-ray filamentation, and that the spectral splitting and broadening is driven by Rabi cycling with sub-femtosecond periods. Our simulations indicate that these X-ray pulses can have pulse lengths of less than 100 attoseconds and coherence properties that open the door for quantum X-ray optics applications.
Cite
@article{arxiv.2409.06914,
title = {Attosecond Inner-Shell Lasing at Angstrom Wavelengths},
author = {Thomas M. Linker and Aliaksei Halavanau and Thomas Kroll and Andrei Benediktovitch and Yu Zhang and Yurina Michine and Stasis Chuchurka and Zain Abhari and Daniele Ronchetti and Thomas Fransson and Clemens Weninger and Franklin D. Fuller and Andy Aquila and Roberto Alonso-Mori and Sebastien Boutet and Marc W. Guetg and Agostino Marinelli and Alberto A. Lutman and Makina Yabashi and Ichiro Inoue and Taito Osaka and Jumpei Yamada and Yuichi Inubushi and Gota Yamaguchi and Toru Hara and Ganguli Babu and Devashish Salpekar and Farheen N. Sayed and Pulickel M. Ajayan and Jan Kern and Junko Yano and Vittal K. Yachandra and Matthias F. Kling and Claudio Pellegrini and Hitoki Yoneda and Nina Rohringer and Uwe Bergmann},
journal= {arXiv preprint arXiv:2409.06914},
year = {2025}
}