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Electrostatic interactions in polymeric systems are responsible for a wide range of liquid-liquid phase transitions that are of importance for biology and materials science. Such transitions are referred to as complex coacervation, and…

Soft Condensed Matter · Physics 2023-09-29 Boyuan Yu , Heyi Liang , Paul F. Nealey , Matthew Tirrell , Artem M. Rumyantsev , Juan J. de Pablo

We review recent experimental, numerical, and analytical results on active suspensions of self-propelled colloidal beads moving in (quasi) two dimensions. Active colloids form part of the larger theme of active matter, which is noted for…

Soft Condensed Matter · Physics 2014-09-03 Julian Bialké , Thomas Speck , Hartmut Löwen

We studied formation of vortex with four-fold symmetry in a minimal model of self-propelled particles, confined inside a squared box, using computer simulations and also theoretical analysis. In addition to the vortex pattern, we observed…

Statistical Mechanics · Physics 2016-03-23 Hamid Seyed-Allaei , Mohammad Reza Ejtehadi

Colloidal particles that are confined to an interface such as the air-water interface are an example of a two-dimensional fluid. Such dispersions have been observed to spontaneously form cluster and stripe morphologies in certain systems…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer

Gels in soft-matter systems are an important nonergodic state of matter. We study a colloid-polymer mixture which is quenched by increasing the polymer concentration, from a fluid to a gel. Using confocal microscopy, we study both the…

Soft Condensed Matter · Physics 2009-04-20 Takehiro Ohtsuka , C. Patrick Royall , Hajime Tanaka

The "melting" of self-formed rigid structures made of a small number of interacting classical particles confined in an irregular two-dimensional space is investigated using Monte Carlo simulations. It is shown that the interplay of…

Disordered Systems and Neural Networks · Physics 2013-06-13 Dyuti Bhattacharya , Amit Ghosal

We report a computer-simulation study of the equilibrium phase diagram of a three-dimensional system of particles with a repulsive step potential. Using free-energy calculations, we have determined the equilibrium phase diagram of this…

Soft Condensed Matter · Physics 2009-11-13 Yu. D. Fomin , Daan Frenkel , N. V. Gribova , V. N. Ryzhov , S. M. Stishov

We study the formation of a colloidal gel by means of Molecular Dynamics simulations of a model for colloidal suspensions. A slowing down with gel-like features is observed at low temperatures and low volume fractions, due to the formation…

Soft Condensed Matter · Physics 2009-11-13 A. Fierro , E. Del Gado , A. de Candia , A. Coniglio

All liquids (except helium due to quantum effects) crystallize at low temperatures, forming ordered structures. The competition between disorder, which stabilizes the liquid phase, and energy, which favors the ordered crystalline structure,…

Soft Condensed Matter · Physics 2013-07-09 Frank Smallenburg , Francesco Sciortino

The equilibrium phase diagram of a 1:1 symmetrical mixture composed of oppositely charged colloids is calculated using Monte Carlo simulations. We model the system by the DLVO effective interaction potential. The phase diagram is similar to…

Soft Condensed Matter · Physics 2007-05-23 José B. Caballero , Antonio M. Puertas

We describe a series of experiments involving the creation of cylindrical packings of star-shaped particles, and an exploration of the stability of these packings. The stars cover a broad range of arm sizes and frictional properties. We…

Soft Condensed Matter · Physics 2020-02-25 Yuchen Zhao , Kevin Liu , Matthew Zheng , Jonathan Barés , Karola Dierichs , Achim Menges , Robert P. Behringer

We perform extensive Monte Carlo simulations to investigate the phase behaviour of colloidal suspensions of hard board-like particles (HBPs). While theories restricting particle orientation or ignoring higher ordered phases suggest the…

Soft Condensed Matter · Physics 2020-06-23 Alessandro Patti , Alejandro Cuetos

When a fluid that undergoes a vapor to liquid transition in the bulk is confined to a long cylindrical pore, the phase transition is shifted (mostly due to surface effects at the walls of the pore) and rounded (due to finite size effects).…

Statistical Mechanics · Physics 2015-05-19 Alexander Winkler , Dorothea Wilms , Peter Virnau , Kurt Binder

Patchy colloidal model with three and four equivalent patches, confined in the attractive random porous media, undergo re-entrant gas-liquid phase separation with the possibility for the liquid phase density to approach zero. This unusual…

Soft Condensed Matter · Physics 2022-05-11 Taras Hvozd , Yurij V. Kalyuzhnyi , Vojko Vlachy , Peter T. Cummings

In this work the well-known Frenkel-Mulder phase diagram of hard ellipsoids of revolution [Mol. Phys. 55, 1171 (1985)] is revisited by means of replica exchange Monte Carlo simulations. The method provides good sampling of dense systems and…

Statistical Mechanics · Physics 2015-06-04 Gerardo Odriozola

Colloidal particles trapped at an interface between two fluids can form a wide range of different structures. Replacing one of the fluid with a liquid crystal increases the complexity of interactions and results in a greater range of…

Soft Condensed Matter · Physics 2014-03-20 Anne Claire Pawsey , Juho Lintuvuori

We systematically study the relationship between equilibrium and non-equilibrium phase diagrams of a system of short-ranged attractive colloids. Using Monte Carlo and Brownian dynamics simulations we find a window of enhanced…

Soft Condensed Matter · Physics 2009-11-13 Andrea Fortini , Eduardo Sanz , Marjolein Dijkstra

Block copolymer melts self-assemble in the bulk into a variety of nanostructures, making them perfect candidates to template the position of nanoparticles. The morphological changes of block copolymers are studied in the presence of a…

Soft Condensed Matter · Physics 2019-10-31 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

X-shaped liquid crystalline molecules (XLCMs) are obtained by tethering two flexible end A-blocks and two flexible side B-blocks to a rigid backbone (R). A rich array of ordered structures can be formed from XLCMs, driven by the competition…

Soft Condensed Matter · Physics 2024-10-25 Dan Wei , Zhijuan He , Yunqing Huang , An-Chang Shi , Kai Jiang

We study a chemically active binary mixture undergoing phase separation and show that under non-equilibrium conditions, stable liquid spherical shells can form via a spinodal instability in the droplet center. A single liquid shell tends to…

Soft Condensed Matter · Physics 2023-06-21 Jonathan Bauermann , Giacomo Bartolucci , Job Boekhoven , Christoph A. Weber , Frank Jülicher