English

Stability of the Liquid Phase in Colloidal Electrolytes

Soft Condensed Matter 2007-05-23 v1

Abstract

The equilibrium phase diagram of a 1:1 symmetrical mixture composed of oppositely charged colloids is calculated using Monte Carlo simulations. We model the system by the DLVO effective interaction potential. The phase diagram is similar to that of its atomic analog (the ionic fluid), where a liquid-gas first order transition emerges in the low TρT-\rho regions being stable with respect to crystallization. As in the ionic fluids, we have found two different crystals: at high TT the fluid crystallizes in a FCC lattice, whereas at low TT, the liquid coexists with a BCC crystal. The region of gas-liquid stability is observed to be narrower as the interaction range is diminished.

Keywords

Cite

@article{arxiv.cond-mat/0511666,
  title  = {Stability of the Liquid Phase in Colloidal Electrolytes},
  author = {José B. Caballero and Antonio M. Puertas},
  journal= {arXiv preprint arXiv:cond-mat/0511666},
  year   = {2007}
}

Comments

Proceedings of Quitel-2005 (Margarita, Venezuela)