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We present a setup for highly polarized proton beams using two parallel propagating laser pulses that have a carrier envelope phase difference of $\pi$. This mechanism is examined utilizing particle-in-cell simulations and compared to a…

Plasma Physics · Physics 2022-08-19 Lars Reichwein , Markus Büscher , Alexander Pukhov

A theoretical study of the rotational dynamics of a linear polar molecule in a two-color non-resonant cw laser field is presented. By systematically considering the interactions of this field with the electric dipole moment, polarizability…

Quantum Physics · Physics 2020-08-26 David Mellado-Alcedo , Niurka R. Quintero , Rosario González-Férez

Linear and nonlinear optical response of WSe$_{2}$ monolayer is investigated by two-dimensional Maxwell plus time-dependent density functional theory with spin-orbit interaction. By applying the chiral resonant pulses, the electron dynamics…

Materials Science · Physics 2022-02-04 Arqum Hashmi , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Tomohito Otobe

Natively, atomic and molecular processes develop in a sub-femtosecond time scale. In order to, for instance, track and capture the electron motion in that scale we need suitable `probes'. Attosecond pulses configure the most appropriate…

We study the dynamics of an array of nearest-neighbor coupled spatially distributed systems each generating a periodic sequence of short pulses. We demonstrate that unlike a solitary system generating a train of equidistant pulses, an array…

Pattern Formation and Solitons · Physics 2017-10-25 D. Puzyrev , A. G. Vladimirov , A. Pimenov , S. V. Gurevich , S. Yanchuk

We show that the decays with pressure of the alignment echoes induced in N2O-He gas mixtures by two laser pulses with various delays bring detailed information on collision-induced changes of the rotational speed. Measurements and…

We present theoretical calculations for polarization and ellipticity of high-order harmonics from aligned N$_2$, CO$_2$, and O$_2$ molecules generated by linearly polarized lasers. Within the rescattering model, the two polarization…

Atomic Physics · Physics 2010-12-13 Anh-Thu Le , R. R. Lucchese , C. D. Lin

We theoretically demonstrate a scheme for tomographic reconstruction of asymmetric molecular orbitals based on high-order harmonic generation with a two-color multicycle laser field. It is shown that by adjusting the relative phase of the…

Atomic Physics · Physics 2013-12-30 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Peixiang Lu

In atoms spin-orbit coupling (SOC) cannot raise the angular momentum above a maximum value or lower it below a minimum. Here we show that this need not be the case in materials built from nanoscale structures including multi-nuclear…

Strongly Correlated Electrons · Physics 2017-03-15 A. L. Khosla , A. C. Jacko , J. Merino , B. J. Powell

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

Atomic Physics · Physics 2009-10-30 D. Bauer

Several laser techniques have been suggested and demonstrated recently for preparing polarizable molecules in rapidly spinning states with a disc-like angular distribution. We consider motion of these spinning discs in inhomogeneous fields,…

Chemical Physics · Physics 2015-05-20 Johannes Floss , Erez Gershnabel , Ilya Sh. Averbukh

Recently, it was predicted theoretically and verified experimentally that a pair of delayed and cross-polarized short laser pulses can create molecular ensembles with a well defined sense of rotation (clockwise or counterclockwise). Here we…

A strong inhomogeneous static electric field is used to spatially disperse a rotationally cold supersonic beam of 2,6-difluoroiodobenzene molecules according to their rotational quantum state. The molecules in the lowest lying rotational…

Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…

We show that multiple filamentation patterns in high-power laser beams, can be described by means of two statistical physics concepts, namely self-similarity of the patterns over two nested scales, and nearest-neighbor interactions of…

Statistical Mechanics · Physics 2015-05-27 Wahb Ettoumi , Jérôme Kasparian , Jean-Pierre Wolf

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

Control of molecular rotations by laser fields is an active area of research focusing on the alignment/orientation of otherwise isotropic molecular samples. Oriented molecules are useful in many applications, such as molecular orbital…

Chemical Physics · Physics 2020-07-03 Long Xu , Ilia Tutunnikov , Erez Gershnabel , Yehiam Prior , Ilya Sh. Averbukh

We present a novel method for probing the alignment of the molecular axis of an ultracold, nonpolar dimer. These results are obtained using diatomic $^{87}\textrm{Rb}_2$ molecules in the vibrational ground state of the lowest triplet…

Atomic Physics · Physics 2015-01-15 Markus Deiß , Björn Drews , Benjamin Deissler , Johannes Hecker Denschlag

The mixed-field orientation of an asymmetric-rotor molecule with its permanent dipole moment non-parallel to the principal axes of polarizability is investigated experimentally and theoretically. We find that for the typical case of a…

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh