Related papers: Alignment of asymmetric-top molecules using multip…
We demonstrate a novel experimental implementation to strongly align molecules at full repetition rates of free-electron lasers. We utilized the available in-house laser system at the coherent x-ray imaging beamline at the Linac Coherent…
It is shown that well collimated mono-energetic ion beams with a large particle number can be generated in the hole-boring radiation pressure acceleration regime by using an elliptically polarized laser pulse with appropriate theoretically…
We present a theoretical study of the time-dependent laser alignment of molecules taking into account the hyperfine coupling due to nuclear-quadrupole interactions. The coupling of nuclear spins to the overall angular momentum of molecules…
Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…
We propose a mechanism to produce a superposition of atomic and molecular states by a train of ultrashort laser pulses combined with weak control fields. By adjusting the repetition rate of the pump pulses and the intensity of the coupling…
We computationally demonstrate a new method for coherently controlling the rotation-axis direction in asymmetric top molecules with an optical centrifuge. Appropriately chosen electric-field strengths and the centrifuge's acceleration rate…
We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…
Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…
Interaction of axisymmetrically-polarized (radially or azimuthally-polarized), relativistically intense laser pulses (ALP) with under-dense plasma is shown experimentally to be different from the interaction of conventional Gaussian pulses.…
We theoretically demonstrate the possibility to tune the temporal waveform of optical unipolar pulses upon their coherent interaction with a multi-level resonant medium. This is achieved through the coherent control of the response of a…
We demonstrate that the current laser technology used for field-free molecular alignment via a cascade of Raman rotational transitions allows for observing long-discussed non-linear quantum phenomena in the dynamics of the periodically…
Since the advent of chirped pulse amplification1 the peak power of lasers has grown dramatically and opened the new branch of high field science, delivering the focused irradiance, electric fields of which drive electrons into the…
The rotational echo response of molecules is found to strongly depend on the delay between the two ultrashort laser pulses, as opposed to two-level systems. We study this dependence experimentally and theoretically and show that by…
Abstract We report the experimental observation of molecular unidirectional rotation (UDR) echoes, and analyze their origin and behavior both classically and quantum mechanically. The molecules are excited by two time-delayed…
Using the Dirac-Heisenberg-Wigner (DHW) formalism, e?ects of asymmetric pulse shape on the generation of electron-positron pairs in three typical polarized fields, i.e., the linear, middle elliptical and circular ones, are investigated. Two…
We propose a system that exploits the fundamental features of topological photonics and synthetic dimensions to force many semiconductor laser resonators to synchronize, mutually lock, and under suitable modulation emit a train of…
An all-optical method of ultrafast spin rotation is put forward to precisely manipulate the polarization of relativistic charged particle beams of leptons or ions. In particular, laser-driven dense ultrashort beams are manipulated via…
We study nonperturbative pair production driven by alternating-sign electric field pulse trains. Using a quantum kinetic approach, we analyze both the longitudinal momentum spectrum and the particle yield for pulse sequences with either…
In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…
SABRE (Signal Amplification by Reversible Exchange) methods provide a simple, fast, and cost-effective method to hyperpolarize a wide variety of molecules in solution, and have been demonstrated with protons and, more recently, with…