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Probing the axis alignment of an ultracold spin-polarized $\textrm{Rb}_2$ molecule

Atomic Physics 2015-01-15 v3 Quantum Gases

Abstract

We present a novel method for probing the alignment of the molecular axis of an ultracold, nonpolar dimer. These results are obtained using diatomic 87Rb2^{87}\textrm{Rb}_2 molecules in the vibrational ground state of the lowest triplet potential a3Σu+a^3\Sigma_u^+ trapped in a 3D optical lattice. We measure the molecular polarizabilities, which are directly linked to the alignment, along each of the xx, yy, and zz directions of the lab coordinate system. By preparing the molecules in various, precisely defined rotational quantum states we can control the degree of alignment of the molecular axis with high precision over a large range. Furthermore, we derive the dynamical polarizabilities for a laser wavelength of 1064.5nm1064.5\:\textrm{nm} parallel and orthogonal to the molecular axis of the dimer, α=(8.9±0.9)×103a.u.\alpha_\parallel=(8.9 \pm 0.9)\times10^3\:\textrm{a.u.} and α=(0.9±0.4)×103a.u.\alpha_\perp=(0.9 \pm 0.4)\times10^3\:\textrm{a.u.}, respectively. Our findings highlight that the depth of an optical lattice strongly depends on the rotational state of the molecule which has to be considered in collision experiments. The present work paves the way for reaction studies between aligned molecules in the ultracold temperature regime.

Keywords

Cite

@article{arxiv.1404.1255,
  title  = {Probing the axis alignment of an ultracold spin-polarized $\textrm{Rb}_2$ molecule},
  author = {Markus Deiß and Björn Drews and Benjamin Deissler and Johannes Hecker Denschlag},
  journal= {arXiv preprint arXiv:1404.1255},
  year   = {2015}
}

Comments

6 pages and 4 figures including supplemental material