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The recently observed multiferroic behavior in the s=1/2 chain cuprate LiVCuO_4 (LiCuVO_4) with edge-shared CuO_4 plaquettes and helical spin ordering does not agree with the existing theories such as a spin-current scenario. We argue that…

Strongly Correlated Electrons · Physics 2009-11-13 A. S. Moskvin , S. -L. Drechsler

We argue for a recently observed puzzling multiferroic behavior in s=1/2 1D chain cuprate LiCu2O2 with edge-shared arrangement of CuO4 plaquettes and incommensurate spiral spin ordering can be consistently explained if one takes into…

Strongly Correlated Electrons · Physics 2009-11-13 A. S. Moskvin , Yu. D. Panov , S. -L. Drechsler

A ferroelectric transition occurring simultaneously with helical spin order has been found in both the polycrystalline and single crystal samples of LiCuVO4. The system has Cu2+ spins (s=1/2) of the CuO2 chains formed of edge-sharing CuO4…

Strongly Correlated Electrons · Physics 2015-06-25 Yutaka Naito , Kenji Sato , Yukio Yasui , Yusuke Kobayashi , Yoshiaki Kobayashi , Masatoshi Sato

The microscopic origin of the recently observed helical structure in LiCu2O2 [1] is considered. It is shown that the frustrated antiferromagnetic double chain scenario adopted in Ref.1 is unrealistic. It should be replaced by a frustrated…

Strongly Correlated Electrons · Physics 2009-11-10 S. -L. Drechsler , J. Malek , J. Richter , A. S. Moskvin , A. A. Gippius , H. Rosner

Neutron diffraction and 7Li-NMR have been applied to determine the multiferroic system LiCu2O2, which has four chains (ribbon chains) of edge-sharing CuO4 square planes in a unit cell. We have confirmed that there are successive magnetic…

Materials Science · Physics 2015-05-13 Yoshiaki Kobayashi , Kenji Sato , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Kazuhisa Kakurai

The magnetic structure of the edge sharing cuprate compound Li2CuO2 has been investigated by means of ab initio electronic structure calculations. The first and second neighbor in-chain magnetic interactions are calculated to be -142 K and…

Materials Science · Physics 2007-05-23 Coen de Graaf , Iberio de P. R. Moreira , Francesc Illas , Oscar Iglesias , Amilcar Labarta

We report on NMR studies of the quasi--1D antiferromagnetic $S=1/2$ chain cuprate LiCuVO$_4$, focusing on the high--field spin--modulated phase observed recently in applied magnetic fields $H > H_{\rm c2}$ ($\mu_0H_{\rm c2} \approx 7.5$ T).…

Materials Science · Physics 2010-02-12 N. Buttgen , W. Kraetschmer , L. E. Svistov , L. A. Prozorova , A. Prokofiev

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

We present an inelastic neutron scattering investigation of Li2CuO2 detecting the long sought quasi-1D magnetic excitations with a large dispersion along the CuO2-chains studied up to 25 meV. The total dispersion is governed by a…

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

A spin model of quasi-one dimensional LiCu$_{2}$O$_{2}$ compound with ground state of ellipsoidal helical structure in which the helical axis is along the diagonal of CuO$_{4}$ squares has been adopted. By taking into account the interchain…

Materials Science · Physics 2015-06-18 Yan Qi , An Du

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

Strongly Correlated Electrons · Physics 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

Neutron diffraction and bulk measurements are used to determine the nature of the low-temperature ordered state in LiCu$_2$O$_2$, a $S=1/2$ spin-chain compound with competing interactions. The magnetic structure is found to be helimagnetic,…

Strongly Correlated Electrons · Physics 2007-05-23 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

Exchanged interactions in recently observed helical structure in LiCu2O2 is probed by inelastic neutron scattering. The main conlusions of Refs. [1,2] are confirmed: nn interactions in single chains are ferromagnetic and frustrated by nnn…

Strongly Correlated Electrons · Physics 2009-11-10 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

We report susceptibility, specific heat, and neutron diffraction measurements on NaCu$_2$O$_2$, a spin-1/2 chain compound isostructural to LiCu$_2$O$_2$, which has been extensively investigated. Below 13 K, we find a long-range ordered,…

Strongly Correlated Electrons · Physics 2013-05-29 L. Capogna , M. Mayr , P. Horsch , M. Raichle , R. K. Kremer , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

We study the one-dimensional spin-1/2 Heisenberg chain with competing ferromagnetic nearest-neighbor J_1 and antiferromagnetic next-nearest-neighbor J_2 exchange couplings in the presence of magnetic field. We use both numerical approaches…

Strongly Correlated Electrons · Physics 2008-10-07 Toshiya Hikihara , Lars Kecke , Tsutomu Momoi , Akira Furusaki

A new spin-1/2 quasi-one-dimensional antiferromagnet KCuMoO_4(OH) is prepared by the hydrothermal method. The crystal structures of KCuMoO_4(OH) and the already-known Na-analogue, NaCuMoO_4(OH), are isotypic, comprising chains of Cu^{2+}…

Strongly Correlated Electrons · Physics 2015-05-21 Kazuhiro Nawa , Takeshi Yajima , Yoshihiko Okamoto , Zenji Hiroi

We present a SU(2) gauge theory of fluctuating magnetic order in the two-dimensional Hubbard model. The theory is based on a fractionalization of electrons in fermionic chargons and bosonic spinons. The chargons undergo N\'eel or spiral…

Strongly Correlated Electrons · Physics 2022-12-08 Pietro M. Bonetti , Walter Metzner

A complete phase diagram of Zn substituted quantum quasi-two-dimensional helimagnet LiCu2O2 has been presented. Helical ordering transition temperature (T_h) of the original LiCu2O2 follows finite size scaling for less than ~ 5.5% Zn…

Strongly Correlated Electrons · Physics 2013-05-29 H. C. Hsu , J. -Y. Lin , W. L. Lee , M. -W. Chu , T. Imai , Y. J. Kao , C. D. Hu , H. L. Liu , F. C. Chou

The spin dynamics of the geometrically frustrated triangular antiferromagnet multiferroic CuCrO2 have been mapped out using inelastic neutron scattering. The relevant spin Hamiltonian parameters modelling the incommensurate modulated…

Strongly Correlated Electrons · Physics 2015-05-14 M. Poienar , F. Damay , C. Martin , J. Robert , S. Petit
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