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Low-dimensional magnetic materials with spin-$\frac{1}{2}$ moments can host a range of exotic magnetic phenomena due to the intrinsic importance of quantum fluctuations to their behavior. Here, we report the structure, magnetic structure…

We consider the effect of doping on the magnetic order in quasi one-dimensional (1D) antiferromagnets. First the detailed magnetic response of finite spin-1/2 chains in the presence of a staggered field is determined, which by itself shows…

Strongly Correlated Electrons · Physics 2015-06-25 Sebastian Eggert , Ian Affleck

The structure and the magnetic properties of layered Li3Cu2SbO6 are investigated by powder X-ray diffraction, static susceptibility, and electron spin resonance studies up to 330 GHz. The XRD data experimentally verify the space group C2/m…

We investigate the structural and magnetic properties of two molecule-based magnets synthesized from the same starting components. Their different structural motifs promote contrasting exchange pathways and consequently lead to markedly…

We report $^{139}$La nuclear magnetic resonance (NMR) measurements on La$_{2-x}$Sr$_x$CuO$_4$ ($0.07\leq x \leq 0.15$) and La$_{2-x}$Ba$_x$CuO$_4$ ($x=1/8$) single crystals, focusing on the spin freezing observed in 1/8-doped lanthanum…

Superconductivity · Physics 2014-06-13 S. -H. Baek , M. Hücker , A. Erb , G. D. Gu , B. Büchner , H. -J. Grafe

We present neutron scattering measurements on powder samples of the spinel FeSc2S4 that reveal a previously unobserved magnetic ordering transition occurring at 11.8(2)~K. Magnetic ordering occurs subsequent to a subtle cubic-to-tetragonal…

Strongly Correlated Electrons · Physics 2016-12-21 K. W. Plumb , Jennifer Morey , J. A. Rodriguez-Rivera , Hui Wu , A. A. Podlesnyak , T. M. McQueen , C. L. Broholm

Neutron diffraction measurements on multiferroic LuFe2O4 show changes in the antiferromagnetic (AFM) structure characterized by wavevector q = (1/3 1/3 1/2) as a function of electric field cooling procedures. The increase of intensity from…

Strongly Correlated Electrons · Physics 2011-11-09 A. M. Mulders , M. Bartkowiak , J. R. Hester , E. Pomjakushina , K. Conder

We have analyzed the magnetic interactions of a five orbital model for iron superconductors treated both within Hartree-Fock and Heisenberg approximations. We have found that the exchange constants depend non-trivially on the Fe-As-Fe angle…

Strongly Correlated Electrons · Physics 2012-10-08 M. J. Calderon , G. Leon , B. Valenzuela , E. Bascones

Here we report a resonant x-ray diffraction (RXD) study at the Cu L3 edge on the multi-chiral system CsCuCl3, exhibiting helical magnetic order in a chiral crystal structure. RXD is a powerful technique to disentangle electronic degrees of…

On the triangular lattice, for $J_2/J_1$ between $1/8$ and $1$, the classical Heisenberg model with first and second neighbor interactions presents four-sublattice ordered ground-states. Spin-wave calculations of Chubukov and…

Condensed Matter · Physics 2009-10-28 P. Lecheminant , B. Bernu , C. Lhuillier , L. Pierre

Density functional calculations are performed to study the magnetic order of the severely distorted square planar cupric oxide (CuO) and local spin disorder in it in the presence of the transition metal impurities M (= Cr, Mn, Fe, Co and…

Strongly Correlated Electrons · Physics 2017-04-05 B. G. Ganga , P. N. Santhosh , B. R. K. Nanda

Several Cu$^{2+}$ hydroxide minerals have recently been identified as candidate realizations of the $S=1/2$ kagome Heisenberg model. In this context, we have studied the distorted system KCu$_3$As$_2$O$_7$(OD)$_3$ using neutron scattering…

The temperature dependence of the optical and magnetic properties of CuO were examined by means of hybrid density functional theory calculations. Our work shows that the spin exchange interactions in CuO are neither fully one-dimensional…

Materials Science · Physics 2015-05-13 X. Rocquefelte , M. -H. Whangbo , A. Villesuzanne , S. Jobic , F. Tran , K. Schwarz , P. Blaha

Contrary to prior calculations, the Ni-rich ordered structures of the Cr-Ni alloy system are found to be antiferromagnetic under semi-local density-functional theory. The optimization of local magnetic moments significantly increases the…

Materials Science · Physics 2023-08-23 Flynn Walsh , Robert O. Ritchie , Mark Asta

Hexagonal LuFe2O4 is a promising charge-order (CO) driven multiferroic material with high charge and spin ordering temperatures. The coexisting charge and spin orders on Fe3+/Fe2+ sites result in novel magnetoelectric behaviors, but the…

Motivated by the co-existing charge and spin order found in strongly correlated ladder systems, we study an effective pseudospin model on a coupled two-leg ladder. A bosonisation analysis yields a rich phase diagram showing Wigner/Peierls…

Strongly Correlated Electrons · Physics 2007-05-23 Siddhartha Lal , Mukul S. Laad

We explore the effects of noncommuting applied fields on the ground-state ordering of the quasi-one-dimensional spin-1/2 XY-like antiferromagnet Cs2CoCl4 using single-crystal neutron diffraction. In zero field interchain couplings cause…

Strongly Correlated Electrons · Physics 2009-11-07 M. Kenzelmann , R. Coldea , D. A. Tennant , D. Visser , M. Hofmann , P. Smeibidl , Z. Tylczynski

We investigate the spin $S=1/2$ Heisenberg model on the body centered cubic lattice in the presence of ferromagnetic and antiferromagnetic nearest-neighbor $J_{1}$, second-neighbor $J_{2}$, and third-neighbor $J_{3}$ exchange interactions.…

Starting from the Mott insulator picture for cubic vanadates, we derive and investigate the model of superexchange interactions between V$^{3+}$ ions, with nearly degenerate $t_{2g}$ orbitals occupied by two electrons each. The…

Strongly Correlated Electrons · Physics 2007-06-19 Andrzej M. Oles , Peter Horsch , Giniyat Khaliullin

The exchange interactions in insulators depend on the orbital state of magnetic ions, obeying certain phenomenological principles, known as Goodenough-Kanamori-Anderson rules. Particularly, the ferro order of alike orbitals tends to…

Strongly Correlated Electrons · Physics 2024-11-11 I. V. Solovyev , R. Ono , S. A. Nikolaev
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