English

NMR study of the high-field magnetic phase of LiCuVO$_4$

Materials Science 2010-02-12 v1 Strongly Correlated Electrons

Abstract

We report on NMR studies of the quasi--1D antiferromagnetic S=1/2S=1/2 chain cuprate LiCuVO4_4, focusing on the high--field spin--modulated phase observed recently in applied magnetic fields H>Hc2H > H_{\rm c2} (μ0Hc27.5\mu_0H_{\rm c2} \approx 7.5 T). The NMR spectra of 7^7Li and 51^{51}V around the transition from the ordered to the paramagnetic state were measured. It is shown that the spin--modulated magnetic structure forms with ferromagnetic interactions between spins of neighboring chains within the {\bf ab}--plane at low temperatures 0.6 K <T<TN < T < T_{\rm N}. The best fit provides evidence that the mutual orientation between spins of neighboring {\bf ab}--planes is random. For elevated temperatures TN<T15T_{\rm N} < T \lesssim 15 K, short--range magnetic order occurs at least on the characteristic time scale of the NMR experiment.

Keywords

Cite

@article{arxiv.0912.4376,
  title  = {NMR study of the high-field magnetic phase of LiCuVO$_4$},
  author = {N. Buttgen and W. Kraetschmer and L. E. Svistov and L. A. Prozorova and A. Prokofiev},
  journal= {arXiv preprint arXiv:0912.4376},
  year   = {2010}
}

Comments

5 pages, 5 figures