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The long-time behavior of a reaction-diffusion front between one static (e.g. porous solid) reactant A and one initially separated diffusing reactant B is analyzed for the mean-field reaction-rate density R(\rho_A,\rho_B) =…

Chemical Physics · Physics 2009-10-31 Martin Z. Bazant , Howard A. Stone

The nonlinear theory of anomalous diffusion is based on particle interactions giving an explicit microscopic description of diffusive processes leading to sub-, normal, or super-diffusion as a result competitive effects between attractive…

Statistical Mechanics · Physics 2016-01-20 Jean Pierre Boon , James F. Lutsko

We present a theory for the kinetics of surfactant adsorption at the interface between an aqueous solution and another fluid (air, oil) phase. The model relies on a free-energy formulation. It describes both the diffusive transport of…

Condensed Matter · Physics 2007-05-23 H. Diamant , D. Andelman

The nonperturbative expressions for the free energy and force of interaction between a ground-state atom and a real-material surface at any temperature are presented. The transition to the Matsubara representation is performed, whereupon…

Quantum Physics · Physics 2018-01-23 M. Bordag , G. L. Klimchitskaya , V. M. Mostepanenko

Motivated by recent research of Nikitin et al. (J.Phys.D vol. 49, 055301(2009)), we examine the effects of interatomic interactions on adatom surface diffusion. By using a mean-field approach in the random walk problem, we derive a…

Statistical Mechanics · Physics 2011-05-17 Yuri B. Gaididei , Vadim M. Loktev , Anton G. Naumovets , Anatoly G. Zagorodny

The rate of diffusion of a Cu adatom on the Cu(100) surface is calculated using thermodynamic integration within the transition state theory. The results are found to be in excellent agreement with the essentially exact values from…

Materials Science · Physics 2009-10-31 Ghyslain Boisvert , Normand Mousseau , Laurent J. Lewis

Surface nanobubbles are nanoscopic spherical-cap shaped gaseous domains on immersed substrates which are stable, even for days. After the stability of a {\it single} surface nanobubble has been theoretically explained, i.e. contact line…

Fluid Dynamics · Physics 2020-02-06 Xiaojue Zhu , Roberto Verzicco , Xuehua Zhang , Detlef Lohse

We develop a version of the vacancy mediated tracer diffusion model, which follows the properties of the physical system of In atoms diffusing within the top layer of Cu(001) terraces. This model differs from the classical tracer diffusion…

Statistical Mechanics · Physics 2007-05-23 E. Somfai , R. van Gastel , S. B. van Albada , W. van Saarloos , J. W. M. Frenken

In this paper the percolation of monomers on a square lattice is studied as the particles interact with either repulsive or attractive energies. By means of a finite-size scaling analysis, the critical exponents and the scaling collapsing…

Statistical Mechanics · Physics 2009-11-13 M. Cecilia Gimenez , Felix Nieto , Antonio J. Ramirez-Pastor

A second order classical perturbation theory is developed and applied to elastic atom corrugated surface scattering. The resulting theory accounts for experimentally observed asymmetry in the final angular distributions. These include…

Materials Science · Physics 2014-01-16 Eli Pollak , S. Miret-Artes

Collective diffusion coefficient in a one dimensional lattice gas adsorbate is calculated using variational approach. Particles interact via either a long-range, or a long range electron-gas-mediated (for a metallic substrate), or a…

Materials Science · Physics 2009-05-26 Filip Krzyżewski , Magdalena A. Załuska-Kotur

Different approaches are presented to investigate diffusion from a point source in a slab delimited by two absorbing boundaries consisting of parallel infinite planes. These approaches enable to consider the effect of absorption at the…

General Physics · Physics 2007-05-23 Richard Taillet , Pierre Salati , David Maurin , Eric Pilon

At finite concentrations of reacting molecules, kinetics of diffusion-controlled reactions is affected by intra-reactant interactions. As a result, multi-particle reaction statistics cannot be deduced from single-particle results. Here we…

Statistical Mechanics · Physics 2019-08-23 Tal Agranov , Baruch Meerson

We review and complete the existing literature on the kinetic theory of spatially homogeneous systems with long-range interactions taking collective effects into account. The evolution of the system as a whole is described by the…

Statistical Mechanics · Physics 2012-02-20 Pierre-Henri Chavanis

Diffusion-induced Ramsey narrowing that appears when atoms can leave the interaction region and repeatedly return without lost of coherence is investigated using strong collisions approximation. The effective diffusion equation is obtained…

Quantum Physics · Physics 2008-01-23 Alexander Romanenko , Leonid Yatsenko

This paper is an electronic application to my set of lectures, subject:`Formal methods in solving differential equations and constructing models of physical phenomena'. Addressed, mainly: postgraduates and related readers. Content: a…

Mathematical Physics · Physics 2007-05-23 Sergej A. Choroszavin

Diffusion studies of adsorbates moving on a surface are often analyzed using 2D Langevin simulations. These simulations are computationally cheap and offer valuable insight into the dynamics, however, they simplify the complex interactions…

Materials Science · Physics 2015-05-28 Moshe Diamant , Saar Rahav , Riccardo Ferrando , Gil Alexandrowicz

We consider the effective surface motion of a particle that intermittently unbinds from a planar surface and performs bulk excursions. Based on a random walk approach we derive the diffusion equations for surface and bulk diffusion…

Statistical Mechanics · Physics 2015-06-05 Aleksei V. Chechkin , Irwin M. Zaid , Michael A. Lomholt , Igor M. Sokolov , Ralf Metzler

This chapter deals with various aspects related to the adsorption of long chain-like macromolecules (polymers) onto solid surfaces. Physical aspects of the adsorption mechanism are elaborated mainly at thermodynamical equilibrium. The basic…

Soft Condensed Matter · Physics 2007-05-23 David Andelman , Roland R. Netz

We consider reaction-diffusion equations on the planar square lattice that admit spectrally stable planar travelling wave solutions. We show that these solutions can be continued into a branch of travelling corners. As an example, we…

Dynamical Systems · Mathematics 2019-01-09 Hermen Jan Hupkes , Leonardo Morelli