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We have combined ab initio molecular dynamics with the intrinsic reaction coordinate in order to investigate the mechanisms of stability and pyrolysis of N$_{4}$-- N$_{120}$ fullerene-like nitrogen cages. The stability of the cages was…

Materials Science · Physics 2020-11-03 Konstantin Katin , Valeriy Merinov , Alexey Kochaev , Savas Kaya , Mikhail Maslov

We studied the temperature stability of the endohedral fullerene molecule, N@C60, inside single-wall carbon nanotubes using electron spin resonance spectroscopy. We found that the nitrogen escapes at higher temperatures in the encapsulated…

Materials Science · Physics 2010-07-14 S. Toth , D. Quintavalle , B. Nafradi , L. Korecz , L. Forro , F. Simon

Since the discovery of the fullerene C60, many very interesting structures have been proposed, such as Ti8C12, Au20, Au32, Au42, TM@Sin, Eu@Si20, B80, and B_{40}^{-/0}. Here, an exceptionally stable hollow cage containing 20 scandiums and…

Materials Science · Physics 2016-06-08 Jing Wang , Hong-Man Ma , Ying Liu

Investigations of clathrate structures have gained a new impetus with the recent discovery of room-temperature superconductivity in metal hydrides. Here we report the finding, through density functional theory calculations, of a clathrate…

Materials Science · Physics 2021-08-02 Jorge Laranjeira , Leonel Marques , Manuel Melle-Franco , Karol Strutynski , Manuel Barroso

In this study, based on density functional theory (DFT), we propose a new branch of pseudo-fullerenes which contain triple bonds with sp hybridization. We should call these new nanostructures fullerynes, according to IUPAC. We present four…

Materials Science · Physics 2020-03-24 Mohammad Qasemnazhand , Farhad Khoeini , Farah Marsusi

Based on the third allotropic form of carbon (Fullerenes) through theoretical study have been predicted structures described as non-classical fullerenes. We have studied novel allotropic carbon structures with a closed cage configuration…

Materials Science · Physics 2017-05-24 Christian A. Celaya , Jesús Muñiz , Luis Enrique Sansores

A family of unusually stable boron cages was identified and examined using first-principles local density functional method. The structure of the fullerenes is similar to that of the B12 icosahedron and consists of six crossing…

Materials Science · Physics 2021-09-21 Nevill Gonzalez Szwacki

The electron-conduction properties of fullerene chains are examined by first-principles calculations based on the density functional theory. The conductivity of the C$_{60}$ dimer is low owing to the constraint of the junction of the…

Materials Science · Physics 2015-06-25 Tomoya Ono , Kikuji Hirose

Sequential ionization of fullerene cluster ions (C$_{60}$)$_{n}^{+}$ within multiply-charged helium nanodroplets leads to the intriguing phenomenon of forming and stabilizing doubly- and triply-charged fullerene oligomers. Surprisingly, we…

Atomic and Molecular Clusters · Physics 2023-12-11 Lisa Ganner , Stefan Bergmeister , Lucas Lorenz , Milan Ončák , Paul Scheier , Elisabeth Gruber

Two-dimensional alloys of carbon and nitrogen represent an urgent interest due to prospective applications in nanomechanical and optoelectronic devices. Stability of these chemical structures must be understood as a function of their…

Materials Science · Physics 2015-02-09 Vitaly V. Chaban , Oleg V. Prezhdo

We investigate the stability of boron fullerene sets B76, B78 and B82. We evaluate the ground state energies, nucleus-independent chemical shift (NICS), the binding energies per atom and the band gap values by means of first-principles…

Materials Science · Physics 2017-09-13 Serkan Polad , Mete Ozay

The recent experimental fabrication of monolayer and few-layer C60 polymers paves the way for synthesizing two-dimensional cluster-assembled materials. Compared to atoms with the SO(3) symmetry, clusters as superatoms (e.g., C60) have an…

Materials Science · Physics 2023-05-08 Xueao Li , Fan Zhang , Xuefei Wang , Weiwei Gao , Jijun Zhao

A class of highly symmetric silicon carbide fullerene-like cage nanoclusters with carbon atoms inside the Si_20 cage and with high stability are presented. The Generalized Gradient Approximation of Density Functional Theory (GGA-DFT) is…

Condensed Matter · Physics 2007-05-23 M. N. Huda , A. K. Ray

Superconductivity in the new polymerized C60 fullerite clathrate doped with simple metals was investigated through density functional theory methods. The phonon dispersion curves were systematically computed for the clathrate structures…

We report a computational study of the stability and infrared (IR) vibrational spectra of neutral and singly ionised fullerene cages containing between 44 and 70 carbon atoms. The stability is characterised in terms of the standard enthalpy…

Astrophysics of Galaxies · Physics 2019-02-20 Alessandra Candian , Marina Gomes Rachid , Heather MacIsaac , Viktor N. Staroverov , Els Peeters , Jan Cami

Energy generation and storage are at the center of modern civilization. Energetic materials constitute quite a large class of compounds with a high amount of stored chemical energy that can be released. We hereby use a combination of…

Materials Science · Physics 2018-03-14 Vitaly V. Chaban , Nadezhda A. Andreeva

The stability of metallic clusters of sodium (Na) in the octahedral cages of Na-doped fullerites Na6C60 and Na11C60 is discussed within a Thomas-Fermi model. It is shown that the tetrahedral Na4-cluster in Na6C60 has an electric charge of…

mtrl-th · Physics 2008-02-03 M. Apostol

We report density functional study of alternate fullerene-like cage structures and finite closed capped single-wall nanotubes of aluminum nitride. The cages and nanotubes studied are modeled as Al24N24, Al28N28, Al32N32, Al36N36, Al48N48,…

Materials Science · Physics 2009-11-11 Rajendra R. Zope , Brett I. Dunlap

High-pressure polymeric structures of nitrogen have attracted great attention owing to their potential application as high-energy-density materials. We report the density functional structural prediction of the unexpected stabilization of a…

Materials Science · Physics 2012-06-26 Xiaoli Wang , Yanchao Wang , Maosheng Miao , Xin Zhong , Jian Lv , Jianfu Li , Li Chen , Chris J. Pickard , Yanming Ma

In this work we investigated the encapsulation of C$_20$ and C$_30$ fullerenes into semiconducting carbon nanotubes to study the possibility of bandgap engineering in such systems. Classical molecular dynamics simulations coupled to…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 K. S. Troche , V. R. Coluci , R. Rurali , D. S. Galvão
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