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We report the observation of quantized translational and rotational motion of molecular hydrogen inside the cages of C60. Narrow infrared absorption lines at the temperature of 6K correspond to vibrational excitations in combination with…

The capacity of carbon atomic chains with different terminations for hydrogen storage is studied using first-principles density functional theory calculations. Unlike the physisorption of H2 on the H-terminated chain, we show that two Li…

Mesoscale and Nanoscale Physics · Physics 2010-07-23 Chun-Sheng Liu , Hui An , Zhi Zeng

Transition metal clusters have a broad spectrum of potential applications in electronic and magnetic devices owing to their unique properties. Protective shells such as fullerene C$_{80}$ can be introduced to improve their stability. In…

Materials Science · Physics 2023-09-12 Yixin Li , Hongrong Qiu , Maolin Bo

Using density functional theory calculations, we study doping of a Cr, Mo, and W atom in boron clusters in the size range of 18-24 atoms and report the finding of metal atom encapsulated fullerene-like cage structures with 20 to 24 boron…

Atomic and Molecular Clusters · Physics 2019-07-31 Amol B. Rahane , Pinaki Saha , N. Sukumar , Vijay Kumar

Fullerene coalescence experimentally found in fullerene-embedded single-wall nanotubes under electron-beam irradiation or heat treatment is simulated by minimizing the classical action for many atom systems. The dynamical trajectory for…

Materials Science · Physics 2009-11-07 Yong-Hyun Kim , In-Ho Lee , K. J. Chang , Sangsan Lee

In order to understand the first stages of the nucleation of carbon nanotubes in catalytic processes, we present a tight-binding Monte Carlo study of the stability and cohesive mechanisms of different carbon structures deposited on nickel…

Materials Science · Physics 2009-11-13 Hakim Amara , Christophe Bichara , François Ducastelle

The current paper presents the second part of the study devoted to composites formed by fullerene C60 and single-walled carbon nanotube ([C60-(4,4)] carbon nanobud). The formation of composites is considered from the basic points related to…

Materials Science · Physics 2011-06-06 E. F. Sheka , L. Kh. Shaymardanova

We present all-electron density functional study of the geometry, electronic structure, vibrational modes, polarizabilities as well as the infrared and Raman spectra of fullerene-like arsenic cages. The stability of As$_n$ cages for sizes…

Atomic and Molecular Clusters · Physics 2009-11-10 Tunna Baruah , Mark R. Pederson , Rajendra R. Zope , M. R. Beltran

Recent experimental reports on the realizations of two-dimensional (2D) networks of the C60-based fullerenes with anisotropic and nanoporous lattices represent a significant advance, and create exciting prospects for the development of a…

Materials Science · Physics 2023-07-13 Bohayra Mortazavi

We present novel structural motifs for boron-carbon nano-cages of the stochiometries B12C48 and B12C50, based on first principle calculations. These configurations are distinct from those proposed so far by the fact that the boron atoms are…

Methods for creating endofullerenes have been steadily improving since their discovery, allowing for new types of endofullerenes to be created in larger numbers. When a molecule is trapped in a fullerene, the fullerene creates a harmonic…

Chemical Physics · Physics 2025-01-27 Jonathan Smucker , Jesus Perez-Rios

We study numerically nonlinear dynamics of several types of molecular systems composed of hydrogen-bonded chains placed inside carbon nanotubes with open edges. We demonstrate that carbon nanotubes provide a stabilization mechanism for…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Alexander V. Savin , Yuri S. Kivshar

We study the electronic states of giant single-shell and the recently discovered nested multi-shell carbon fullerenes within the tight-binding approximation. We use two different approaches, one based on iterations and the other on…

Materials Science · Physics 2009-10-22 Yeong-Lieh Lin , Franco Nori

The infrared bar-spectrum of a single ammonia molecule encapsulated in nano-cage C$_{60}$ fullerene molecule is modelled using the site inclusion model successfully applied to analyze spectra of CO$_2$ isotopologues isolated in rare gas…

Chemical Physics · Physics 2011-03-30 Azzedine Lakhlifi , Pierre-Richard Dahoo

Several dimerization products of fullerene C60 are presented and thoroughly characterized with a quantum chemical DFT model augmented by dispersion. We reanalyze and expand significantly the number of known dimers from 12 to 41. Many of the…

On the basis of a topological discussion as well as an {\it ab initio} calculation, we show that it is possible to construct a fullerene-like Si cage by doping of a transition metal atom. The cage is a simple 3-polytope which maximizes the…

Materials Science · Physics 2009-11-07 Takehide Miyazaki , Hidefumi Hiura , Toshihiko Kanayama

Density functional theory is applied to study the mechanism of the Stone-Wales defect formation in pure and nitrogen-doped dodecahedral C$_{20}$ fullerenes. The molecular structures of initial and defected cages as well as transition states…

Mesoscale and Nanoscale Physics · Physics 2016-12-01 Konstantin Katin , Mikhail Maslov

The quasi-hexagonal phase of the two-dimensional fullerene network (qHPC$_{60}$), recently synthesized, has emerged as a stable carbon-based material with distinct structural and electronic features. In this work, we employed density…

To understand the phenomenon of fullerene growth during its synthesis, an attempt is made to model a minimum energy growth route using a semi-empirical quantum mechanics code. C2 addition leading to C60 was modelled and three main routes,…

Chemical Physics · Physics 2016-09-21 Sabih D Khan , Shoaib Ahmad

Li4C60, one of the best representatives of lithium intercalated fullerides, features a novel type of 2D polymerization. Extensive investigations, including laboratory x-ray and synchrotron radiation diffraction, 13C NMR, MAS and Raman…

Materials Science · Physics 2007-05-23 M. Ricco , T. Shiroka , M. Belli , D. Pontiroli , M. Pagliari , G. Ruani , D. Palles , S. Margadonna , M. Tomaselli