English

Sc20C60: A Volleyballene

Materials Science 2016-06-08 v2

Abstract

Since the discovery of the fullerene C60, many very interesting structures have been proposed, such as Ti8C12, Au20, Au32, Au42, TM@Sin, Eu@Si20, B80, and B_{40}^{-/0}. Here, an exceptionally stable hollow cage containing 20 scandiums and 60 carbons was identified. This Sc20C60 molecular cluster has a Th point group symmetry and a volleyball-like shape, that we refer to below as Volleyballene. Electronic structure analysis shows that the formation of delocalized {\pi} bonds between Sc atoms and neighboring five-membered carbon rings is crucial for stabilizing the cage structure. A relatively large HOMO-LUMO gap was found. The results of vibrational frequency analysis and molecular dynamics simulations also demonstrate that this Volleyballene molecule is exceptionally stable.

Cite

@article{arxiv.1502.03507,
  title  = {Sc20C60: A Volleyballene},
  author = {Jing Wang and Hong-Man Ma and Ying Liu},
  journal= {arXiv preprint arXiv:1502.03507},
  year   = {2016}
}
R2 v1 2026-06-22T08:28:06.084Z