Related papers: Cavity-enhanced dual-comb spectroscopy
Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex and fast, and existing…
Optical frequency combs were developed nearly two decades ago to support the world's most precise atomic clocks. Acting as precision optical synthesizers, frequency combs enable the precise transfer of phase and frequency information from a…
Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…
Recent advancements in silicon photonics are enabling the development of chip-scale photonics devices for sensing and signal processing applications, among which on-chip spectrometers are of particular interest for precision wavelength…
Electro-optic frequency combs with tooth spacings as low as 100 Hz were employed to probe electromagnetically induced transparency (EIT) and hyperfine pumping in rubidium and potassium vapor cells. From the potassium EIT transition we were…
Improving spectral acquisition rate of broadband mid-infrared spectroscopy promises further advancements of molecular science and technology. Unlike the pump-probe spectroscopy that requires repeated measurements with different pump-probe…
We present a versatile mid-infrared frequency comb spectroscopy system based on a doubly resonant optical parametric oscillator tunable in the 3-5.4 {\mu}m range and two detection methods, a Fourier transform spectrometer (FTS) and a…
Optical detection of ultrasound for photoacoustic imaging provides large bandwidth and high sensitivity at high acoustic frequencies. Higher spatial resolutions can therefore be achieved using Fabry-P\'erot cavity sensors, as compared to…
Dual-comb spectroscopy is a promising method for precise optical spectrum analysis with fast data acquisition speed. However, its implementation and applications are often hindered by the complexity of optical comb systems. Here, as a…
Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…
Dual-comb spectroscopy is a rapidly developing technique enabling ultraprecise broadband optical diagnostics of atoms and molecules. This powerful tool typically requires two phase-locked femtosecond lasers, yet it has been shown that it…
Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…
Optical frequency combs have the potential to improve the precision of the radial velocity measurement of celestial bodies, leading to breakthroughs in such fields as exoplanet exploration. For these purposes, the comb must have a broad…
Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…
It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…
Direct frequency comb spectroscopy of trapped ions is demonstated for the first time. It is shown that the 4s^2S_(1/2)-4p^2P_(3/2) transition in calcium ions can be excited directly with a frequency comb laser that is upconverted to 393 nm.…
Extreme ultraviolet frequency combs are a versatile tool with applications including precision measurement, strong-field physics, and solid-state physics. Here we report on an application of extreme ultraviolet frequency combs and their…
Frequency-stabilized mid-infrared lasers are valuable tools for precision molecular spectroscopy. However, their implementation remains limited by complicated stabilization schemes. Here we achieve optical self-locking of a quantum cascade…
We measure the fluorescence spectrum of broadband emitters in an open optical microcavity with radius of curvature R = 17.7(3) um and finesse F ~= 1000. This geometry enables a combined measurement of emission spectra versus cavity length,…
We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines…