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Related papers: Cavity-enhanced dual-comb spectroscopy

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Frequency comb assisted diode laser spectroscopy, employing both the accuracy of an optical frequency comb and the broad wavelength tuning range of a tunable diode laser, has been widely used in many applications. In this letter we present…

Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…

Breath analysis enables rapid, non-invasive diagnostics, as well as long-term monitoring, of human health through the identification and quantification of exhaled biomarkers. Here, for the first time, we demonstrate the remarkable…

Chemical Physics · Physics 2022-06-07 Qizhong Liang , Ya-Chu Chan , P. Bryan Changala , David J. Nesbitt , Jun Ye , Jutta Toscano

Accurate time transfer has become a crucial issue for future space experiments which require increasing resolution over large distances. In 2008, a scheme combining homodyne detection and mode-locked femtosecond lasers was proposed that…

Quantum Physics · Physics 2018-11-21 Shaofeng Wang , Xiao Xiang , Nicolas Treps , Claude Fabre , Ruifang Dong , Tao Liu , Shougang Zhang

Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

Dual THz comb spectroscopy has the potential to be used as universal THz spectroscopy with high spectral resolution, high spectral accuracy, and broad spectral coverage; however, the requirement for dual stabilized femtosecond lasers…

Instrumentation and Detectors · Physics 2019-08-06 Guoqing Hu , Tatsuya Mizuguchi , Ryo Oe , Kazuki Nitta , Xin Zhao , Takeo Minamikawa , Ting Li , Zheng Zheng , Takeshi Yasui

Optical frequency combs have revolutionised time and frequency metrology [1, 2]. The advent of microresonator-based frequency combs ('microcombs' [3-5]) is set to lead to the miniaturisation of devices that are ideally suited to a wide…

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

Non-perturbative and phase-sensitive light-matter interactions have led to the generation of attosecond pulses of light and the control electrical currents on the same timescale. Traditionally, probing these effects via high harmonic…

Optics · Physics 2022-05-17 Daniel M. B. Lesko , Kristina F. Chang , Scott A. Diddams

Providing an accurate, representative sample of mass flux across large open areas for atmospheric studies or the extreme conditions of a hypersonic engine is challenging for traditional intrusive or point-based sensors. Here, we demonstrate…

Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the…

Optics · Physics 2022-02-10 Tobias Pfeiffer , Jens Klier , Georg von Freymann , Daniel Molter

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Dual-comb spectroscopy enables broadband, high-resolution measurements with microsecond temporal resolution, but extending this capability to the 10~12.5 $\mu$m molecular fingerprint region remains technically challenging, particularly for…

Optics · Physics 2026-04-30 Pei-Ling Luo , I-Yun Chen

Mid-infrared (MIR) spectral imaging enables precise target identification and analysis by capturing rich chemical fingerprints, which calls for high-sensitivity broadband MIR imagers at room temperature. Here, we devise and implement a…

Optics · Physics 2026-05-26 Yue Song , Jianan Fang , Wen Zhang , Yijing Li , Ben Sun , Zhiwei Jia , Kun Huang , Heping Zeng

We demonstrate a 13-fold speed improvement in broadband cantilever-enhanced photoacoustic spectroscopy (CEPAS) by combining it with phase-controlled Fourier-transform spectroscopy (PC-FTS) instead of traditional Fourier-transform infrared…

Optics · Physics 2022-12-21 Santeri Larnimaa , Mikhail Roiz , Markku Vainio

The achievable instrument sensitivity is a critical parameter for the continued development of THz applications. Techniques such as Cavity-Enhanced Techniques and Cavity Ring Down Spectroscopy have not yet been employed at THz frequency due…

Dual-comb spectroscopy (DCS) is a powerful Fourier-transform spectroscopic technique that provides high-speed, high-resolution, and broadband measurements without moving parts. However, the high peak power of mode-locked pulses limits the…

Optics · Physics 2025-09-30 Wei Long , Xinru Cao , Xiangze Ma , Jiaqi Zhou , Wenbin He , Dijun Chen

Single-cavity dual-comb lasers are a new class of ultrafast lasers which have a wide possible application space including pump-probe sampling, optical ranging, and gas absorption spectroscopy. However, to this date laser cavity multiplexing…

We extend the technique of multiplex coherent Raman spectroscopy with two femtosecond mode-locked lasers to oscillators of a pulse repetition frequency of 1 GHz. We demonstrate spectra of liquids, which span 1100 cm$^{-1}$ of Raman shifts.…

A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

Optics · Physics 2021-07-21 Brad C. Smith , Bachana Lomsadze , Steven T. Cundiff
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