Related papers: Cavity-enhanced dual-comb spectroscopy
Broadband and high-resolution spectroscopy in the visible and ultraviolet is central to advances in multiple fields, including fundamental quantum physics, biology, atmospheric science and astronomy. Traditionally, these measurements are…
The broad and equidistant spectrum of frequency combs has had a profound impact on spectroscopic studies. Particularly, experiments involving the coupling of frequency combs to cavities have already enabled unprecedented broadband and…
We have developed an extreme ultraviolet (XUV) frequency comb for performing ultra-high precision spectroscopy on the many XUV transitions found in highly charged ions (HCI). Femtosecond pulses from a 100 MHz phase-stabilized near-infrared…
A fieldable dual-comb spectrometer is described based on a "bootstrapped" frequency referencing scheme in which short-term optical phase coherence between combs is attained by referencing each to a free-running diode laser, whilst high…
Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…
Mid-infrared dual-comb spectroscopy has the potential to supplant conventional high-resolution Fourier transform spectroscopy in applications that require high resolution, accuracy, signal-to-noise ratio, and speed. Until now, dual-comb…
Two-photon excitation spectroscopy with broad spectral span is demonstrated at Doppler-limited resolution. We describe first Fourier transform two-photon spectroscopy of an atomic sample with two mode-locked laser oscillators in a dual-comb…
Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…
Dual-comb interferometry is a measurement technique that uses two laser frequency combs to retrieve complex spectra in a line-by-line basis. This technique can be implemented with electro-optic frequency combs, offering intrinsic mutual…
Harnessing the quantum interference of photon-pair generation processes, infrared quantum absorption spectroscopy (IRQAS) can extract the infrared optical properties of a sample through visible or near-infrared photon detection without the…
Photo-acoustic spectroscopy (PAS) is one of the most sensitive non-destructive analysis techniques for gases, fluids and solids. It can operate background-free at any wavelength and is applicable to microscopic and even non-transparent…
We present gapless, high-resolution absorption and dispersion spectra obtained with quantum cascade laser frequency combs covering 55 cm$^{-1}$. Using phase-sensitive dual comb design, the comb lines are gradually swept over 10 GHz,…
Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…
We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…
A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…
An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…
The advent of optical frequency standards with ultimate uncertainties in the low 1x10$^{-18}$ requires femtosecond frequency combs to support a similar level of resolution in the spectral transfer and the computation of optical frequency…
High-speed measurement confronts the extreme speed limit when the signal becomes comparable to the noise level. In the context of broadband mid-infrared spectroscopy, state-of-the-art ultrafast Fourier-transform infrared spectrometers, in…
We demonstrate incoherent broadband cavity enhanced absorption spectroscopy in the mid-infrared wave- length range from 3000 to 3450 nm using an all-fiber based supercontinuum source. Multi-components gas detection is performed and…
Here, ultra-low relative phase jitters over a wide optical spectrum were achieved for dual Ti:Sapphire optical frequency combs. The two optical frequency combs were independently phase-locked to a Sr optical lattice clock laser delivered…