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The formation energies and electronic structure of europium doped zinc oxide has been determined using DFT and many-body $GW$ methods. In the absence of intrisic defects we find that the europium-$f$ states are located in the ZnO band gap…

Materials Science · Physics 2016-03-23 M. Lorke , T. Frauenheim , A. L. da Rosa

First-principles, density-functional based electronic structure calculations are carried out for MgC(Ni_{1-x}Co_{x})_{3} alloys over the concentration range 0\leq x\leq1, using Korringa-Kohn-Rostoker coherent-potential approximation (KKR…

Materials Science · Physics 2009-11-11 P. Jiji Thomas Joseph , Prabhakar P. Singh

Electronic structure calculations are carried out to estimate the heats of formation of rare-earth orthophosphates from their oxides. The calculated heats of formation are systematically about 40 kJ/mol less exothermic than the measured…

Materials Science · Physics 2011-07-22 James R. Rustad

Tricobalt tetraoxide (Co3O4) is an important catalyst and Co3O4(110) is a frequently exposed surface in Co3O4 nanomaterials. We employed Density-functional theory with on-site Coulomb repulsion U term to study the atomic structures,…

Materials Science · Physics 2015-06-04 Jia Chen , Annabella Selloni

We present a systematic study of the atomic and electronic structure of the Si(111)-(5x2)-Au reconstruction using first-principles electronic structure calculations based on the density functional theory. We analyze the structural models…

Materials Science · Physics 2009-11-11 Sampsa Riikonen , Daniel Sanchez-Portal

Ab initio calculations using the APW+lo method as implemented in the WIEN2k code have been used to describe the electronic structure of the quasi-one-dimensional system BaCoO3. Both, GGA and LDA+U approximations were employed to study…

Strongly Correlated Electrons · Physics 2009-11-10 V. Pardo , P. Blaha , M. Iglesias , K. Schwarz , D. Baldomir , J. E. Arias

The electronic structure and properties of PuO$_{2}$ and Pu$_{2}$O$_{3}$ have been studied from first principles by the all-electron projector-augmented-wave (PAW) method. The local density approximation (LDA)+$U$ and the generalized…

Materials Science · Physics 2007-12-24 Bo Sun , Ping Zhang , Xian-Geng Zhao

We study the stability and universal behaviour of the ionization energy of N-electron atoms with nuclear charge Z in the anionic domain (Z<N), considering the nuclear charge Z as an arbitrary (non-integral) parameter. HF and CISD ground…

Atomic Physics · Physics 2013-09-16 G. Gil , A. Gonzalez

Near or less than 10% Nb substitution on the Ti site in perovskite SrTiO$_3$ results in metallic behavior, in contrast to what is seen in BaTiO$_3$. Given the nearly identical structure and electron counts of the two materials, the distinct…

Materials Science · Physics 2008-12-14 Katharine Page , Taras Kolodiazhnyi , Thomas Proffen , Anthony K. Cheetham , Ram Seshadri

In order to assist the search of new superconductors in iron selenide materials by intercalation, we calculate the crystal and electronic structures of MgOFeSe using the first-principles density functional theory. MgOFeSe is isotructural to…

Superconductivity · Physics 2013-10-01 Kai Liu , Miao Gao , Zhong-Yi LU , Tao Xiang

By systematic first-principles calculations, we study the electronic structure and magnetic property of SrCrO$_3$. Our results suggest that SrCrO$_3$ is a weakly correlated antiferromagnetic (AF) metal, a very rare situation in…

Materials Science · Physics 2010-07-20 Guangtao Wang , Zhi Li , C. Q. Jin , Zhong Fang

Given increasing energy storage demands and limited natural resources of Li, K-ion batteries (KIBs) could be promising next-generation systems having natural abundance, similar chemistry and energy density. Here, we have investigated the…

Materials Science · Physics 2024-06-21 Pawan Kumar Jha , Sanyam Nitin Totade , Prabeer Barpanda , Gopalakrishnan Sai Gautam

The $f$-electron materials have many unique properties under pressure, thus of great interest in high-pressure physics and related industrial fields. However, the $f$-electrons pose a substantial challenge to simulations since the electron…

Strongly Correlated Electrons · Physics 2024-10-15 Bei-Lei Liu , Yue-Chao Wang , Xing-Yu Gao , Hai-Feng Liu , Hai-Feng Song

The electronic structures of R2Fe3Si5 (where R = Lu, Tm, Er, Tb, Yb) intermetallics have been calculated from first principles in local-spin density (LSDA) and LSDA + U approaches. The majority of rare-earth iron silicides, except for the…

Superconductivity · Physics 2014-09-08 M. J. Winiarski , M. Samsel-Czekała

Recently, electrides have received increasing attention due to their multifunctional properties as superconducting, catalytic, insulating, and electrode materials, with potential to offer other performance and possess novel physical states.…

Superconductivity · Physics 2022-11-23 Zhongyu Wan , Chao Zhang , Tianyi Yang , Wenjun Xu , Ruiqin Zhang

Emergent magnetic states at oxide interfaces arise from the interplay of charge transfer, orbital reconstruction, and dimensional confinement, offering a route to engineered correlated-electron behavior in nanoscale spintronic materials.…

First-principles FLAPW-GGA calculations have been performed with the purpose to determine the peculiarities of the structural, electronic, magnetic properties and stability for a family of related ether carbides M3W3C and M6W6C (where M= Fe…

Materials Science · Physics 2015-05-13 D. V. Suetin , I. R. Shein , A. L. Ivanovskii

First principles calculations of rare earth (RE)-doped LaSi3N5 host lattice are performed to obtain the electronic structure, the band gap (BG), and the character of electronic transitions. Doping with both trivalent and bivalent RE cations…

Materials Science · Physics 2015-06-23 Ismail A. M. Ibrahim , Zoltan Lences , Pavol Sajgalik , Lubomir Benco , Martijn Marsman

Actinide and lanthanide-based materials display exotic properties that originate from the presence of itinerant or localized f-electrons and include unconventional superconductivity and magnetism, hidden order; and heavy fermion behavior.…

Materials Science · Physics 2021-02-26 Ayana Ghosh , Filip Ronning , Serge Nakhmanson , Jian-Xin Zhu

The ground-state 4f fine-structure levels in the intrinsic optical transition gaps between the 2p and 5d orbitals of lanthanide sesquioxides (Ln2O3, Ln=La...Lu) were calculated by a two-way crossover search for the U parameters for DFT+U…

Strongly Correlated Electrons · Physics 2015-11-17 Bolong Huang