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Related papers: Hydrogen/nitrogen/oxygen defect complexes in silic…

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Defects in crystalline silicon consisting of a silicon self-interstitial atom and one, two, three, or four hydrogen atoms are studied within density-functional theory (DFT). We search for low-energy defects by starting from an ensemble of…

Materials Science · Physics 2010-02-11 Andrew J. Morris , Chris J. Pickard , R. J. Needs

An extensive search for low-energy lithium defects in crystalline silicon using density-functional-theory methods and the ab initio random structure searching (AIRSS) method shows that the four-lithium-atom substitutional point defect is…

Materials Science · Physics 2013-05-28 Andrew J. Morris , R. J. Needs , Elodie Salager , C. P. Grey , Chris J. Pickard

We have studied hydrogen/lithium complexes in crystalline silicon using density-functional-theory methods and the ab initio random structure searching (AIRSS) method for predicting structures. A method based on the Maxwell construction and…

Materials Science · Physics 2012-01-25 Andrew J. Morris , C. P. Grey , R. J. Needs , Chris J. Pickard

This work presents an in-depth investigation of the properties of complexes composed of hydrogen, silicon or oxygen with carbon, which are major unintentional impurities in undoped GaN. This manuscript is a complement to our previous work…

Materials Science · Physics 2017-06-20 Masahiko Matsubara , Enrico Bellotti

The structural and electronic properties of amorphous silicon ($a$-Si) are investigated by first-principles calculations based on the density-functional theory (DFT), focusing on the intrinsic structural defects. By simulated melting and…

Materials Science · Physics 2017-10-11 Yoritaka Furukawa , Yu-ichiro Matsushita

It is essential to know the arrangement of the atoms in a material in order to compute and understand its properties. Searching for stable structures of materials using first-principles electronic structure methods, such as density…

Materials Science · Physics 2015-03-17 Chris J. Pickard , R. J. Needs

We investigate the behavior of oxygen vacancies in three different metal-oxide semiconductors (rutile and anatase TiO2, monoclinic WO3, and tetragonal ZrO2) using a recently proposed hybrid density-functional method in which the fraction of…

We have studied intrinsic defect complexes in In$_2$O$_3$ using ab initio random structure searching (AIRSS). Our first-principles density-functional-theory calculations predict the thermodynamic stability of several novel defect…

Materials Science · Physics 2016-09-16 Jamie M. Wynn , Richard J. Needs , Andrew J. Morris

Point defects in the binary group-IV monochalcogenide monolayers of SnS, SnSe, GeS, GeSe are investigated using density-functional-theory calculations. Several stable configurations are found for oxygen defects, however we give evidence…

Mesoscale and Nanoscale Physics · Physics 2016-08-17 Lídia C. Gomes , A. Carvalho , A. H. Castro Neto

Standard density functional approximations often give questionable results for odd-electron radical complexes, with the error typically attributed to self-interaction. In density corrected density functional theory (DC-DFT), certain classes…

Chemical Physics · Physics 2015-06-19 Min-Cheol Kim , Eunji Sim , Kieron Burke

Due to their technological importance, point defects in silicon are among the best studied physical systems. The experimental examination of point defects buried in bulk is difficult and evidence for the various defects usually indirect.…

Materials Science · Physics 2009-11-07 Stefan Goedecker , Luc Billard , Thierry Deutsch

The influence of oxygen and carbon impurities on the concentrations of defects in silicon for detector uses, in complex fields of radiation, characteristic to high energy physics experiments, is investigated in the frame of the quantitative…

High Energy Physics - Phenomenology · Physics 2009-11-10 Sorina Lazanu , Ionel Lazanu

Point defects in diamond are of high interest as candidates for realizing solid state quantum bits, bioimaging agents, or ultrasensitive electric or magnetic field sensors. Various artificial diamond synthesis methods should introduce…

Materials Science · Physics 2016-09-14 Gergő Thiering , Adam Gali

We have made a systematic theoretical study to determine which are the most stable structures for substitutional nitrogen defects in carbon nanotubes, by making total energy calculations via DFT. These calculations were made for a (5,5) and…

Other Condensed Matter · Physics 2007-05-23 Mariana Rossi , Adalberto Fazzio , Antonio J. R. da Silva

Recent experiments on hydrogenated amorphous silicon using infrared absorption spectroscopy have indicated the presence of mono- and divacancy in samples for concentration of up to 14\% hydrogen. Motivated by this observation, we study the…

Materials Science · Physics 2015-05-19 Parthapratim Biswas , Rajendra Timilsina

Cubic hafnia (HfO$_2$) is of great interest for a number of applications in electronics because of its high dielectric constant. However, common defects in such applications degrade the properties of hafina. We have investigated the…

Materials Science · Physics 2019-07-31 Raghuveer Chimata , Hyeondeok Shin , Anouar Benali , Olle Heinonen

Properties of point defects resulting from the incorporation of inert-gas atoms in bcc tungsten are investigated systematically using first-principles density functional theory (DFT) calculations. The most stable configuration for the…

Materials Science · Physics 2015-10-29 Duc Nguyen-Manh , S. L. Dudarev

Zirconolite, CaZrTi2O7, is a proposed ceramic for the use in disposal of highly active nuclear waste. Density functional theory (DFT) has been used, in conjunction with a random search technique, to identify the stable interstitial sites…

Materials Science · Physics 2012-01-27 Jack Mulroue , Andrew J. Morris , Dorothy M. Duffy

Defect energy formation, lattice distortions and electronic structure of cubic In2O3 with Sn, Ga and O impurities were theoretically investigated using density functional theory. Different types of point defects, consisting of 1 to 4 atoms…

Mesoscale and Nanoscale Physics · Physics 2020-02-06 Alexandr I. Cocemasov , Vladimir I. Brinzari , Denis L. Nika

Quantum technologies would benefit from the development of high performance quantum defects acting as single-photon emitters or spin-photon interface. Finding such a quantum defect in silicon is especially appealing in view of its favorable…

Materials Science · Physics 2024-05-09 Yihuang Xiong , Jiongzhi Zheng , Shay McBride , Xueyue Zhang , Sinéad M. Griffin , Geoffroy Hautier
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