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We report a structural/magnetic investigation by X-ray absorption spectroscopy (XAS), neutron diffraction, dc-susceptibility ($\chi_{\mbox{dc}}$) and electron spin resonance (ESR) of the 12R-type perovskite BaTi$_{1/2}$Mn$_{1/2}$O$_{3}$.…

We synthesized single crystals of composition Ba$_2$CuSi$_2$O$_6$Cl$_2$ and investigated its quantum magnetic properties. The crystal structure is closely related to that of the quasi-two-dimensional (2D) dimerized magnet BaCuSi$_2$O$_6$…

Nb$_3$Cl$_8$, a cluster Mott insulator with a distinctive magnetic molecular orbital structure organized into a breathing kagome lattice, showcases critical phase transitions under specialized conditions. By transitioning from paramagnetic…

Materials Science · Physics 2024-09-10 Yuya Haraguchi , Kazuyoshi Yoshimura

We study the N\'eel to dimer transition driven by interlayer exchange coupling in spin-S Heisenberg antiferromagnets on bilayer square and honeycomb lattices for S=1/2, 1, 3/2. Using exact stochastic series expansion quantum Monte Carlo…

Other Condensed Matter · Physics 2013-05-29 R. Ganesh , Sergei V. Isakov , Arun Paramekanti

We report on the magnetocrystalline anisotropy energy (MAE) and spin reorientation in antiferromagnetic state of spin $S=1/2$ tetramer system SeCuO$_3$ observed in torque magnetometry measurements in magnetic fields $H<5$~T and simulated…

X-ray diffraction, thermodynamic measurements, and density-functional band-structure calculations are used to study the magnetic behavior of BaCuTe$_{2}$O$_{6}$, a member of the $A$CuTe$_2$O$_6$ structural family that hosts complex…

Materials Science · Physics 2021-04-21 P. Bag , N. Ahmed , Vikram Singh , M. Sahoo , A. A. Tsirlin , R. Nath

The crystal structure of hexagonal-Sr0.6Ba0.4MnO3 allows various competing superexchange interactions, leading to intriguing magnetic properties. Local structural changes modify overlapping between Mn and oxygen ions with temperature.…

We report the results of measurements of the dc-susceptibility and the 23Na-NMR response of Na2V2O7, a recently synthesized, non metallic low dimensional spin system. Our results indicate that upon reducing the temperature to below 100 K,…

Strongly Correlated Electrons · Physics 2009-11-07 J. L. Gavilano , D. Rau , S. Mushkolaj , H. R. Ott , P. Millet , F. Mila

Optimally-doped La1.85Sr0.15CuO4 single crystals have been investigated by dc and ac magnetic measurements. These crystals have rectangular needle-like shapes with the long needle axis parallel to the crystallographic c axis (c-crystal) or…

Superconductivity · Physics 2015-06-05 I. Felner , M. I. Tsindlekht , G. Drachuck , A. Keren

Dimerized quantum magnets provide a unique possibility to investigate Bose-Einstein condensation of magnetic excitations in crystalline systems at low temperature. Here, we model the low-temperature magnetic properties of the recently…

Strongly Correlated Electrons · Physics 2022-12-14 B. Lenz , B. Koteswararao , S. Biermann , P. Khuntia , M. Baenitz , S. K. Panda

An argument that relaxor ferroelectricity in the isovalent alloy $\mathrm {Ba(Zr}_{1-x}\mathrm{Ti}_{x})\mathrm{O}_3$ can be understood as an induced moment soft pseudo-spin glass on the B-ions of the $\mathrm{ABO}_{3}$ matrix is extended to…

Materials Science · Physics 2015-06-17 David Sherrington

Low-dimensional quantum magnets, due to the existence of abundant exotic quantum phases therein and experimental feasibilities in laboratories, continues intriguing people in condensed matter physics. In this work, a comprehensive study of…

Strongly Correlated Electrons · Physics 2016-07-15 Junsen Xiang , Cong Chen , Wei Li , Xianlei Sheng , Na Su , Zhaohua Cheng , Qiang Chen , Ziyu Chen

We discuss low-temperature properties of magnets with integer spin and large single-ion easy-plane anisotropy $D$ in transverse magnetic field $h$. Considering the exchange interaction between spins as a perturbation and using the diagram…

Strongly Correlated Electrons · Physics 2011-12-30 A. V. Sizanov , A. V. Syromyatnikov

The polycrystalline form of the compound, Tb5Si3, crystallizing in Mn5Si3-type hexagonal structure, which was earlier believe to order antiferromagnetically below 69 K, has been recently reported by us to exhibit interesting…

Materials Science · Physics 2015-06-05 Kartik K. Iyer , K. Mukherjee , P. L. Paulose , E. V. Sampathkumaran , Y. Xu , W. Löser

We carried out AC magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ~1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type…

Strongly Correlated Electrons · Physics 2013-06-03 M. A. de Vries , J. O. Piatek , M. Misek , J. S. Lord , H. M. Ronnow , J. -W. G. Bos

The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based…

Strongly Correlated Electrons · Physics 2025-09-10 A. Brassington , Q. Ma , G. Duan , S. Calder , A. I. Kolesnikov , K. M. Taddei , G. Sala , E. S. Choi , H. Wang , W. Xie , B. A. Frandsen , N. Li , X. F. Sun , C. Liu , R. Yu , H. D. Zhou , A. A. Aczel

The magnetic behavior of the low-dimensional phosphates (Sr,Ba)_2 Cu(PO_4)_2 and BaCuP_2O_7 was investigated by means of magnetic susceptibility and ^{31}P nuclear magnetic resonance (NMR) measurements. We present here the NMR shift K(T),…

Strongly Correlated Electrons · Physics 2009-11-10 R. Nath , A. V. Mahajan , N. Buttgen , C. Kegler , A. Loidl

Heisenberg spin-1/2 chain materials are known to substantially alter their static and dynamic properties when experiencing an effective transverse staggered field originating from the varying local environment of the individual spins. We…

Strongly Correlated Electrons · Physics 2016-11-26 F. Casola , T. Shiroka , V. Glazkov , A. Feiguin , G. Dhalenne , A. Revcolevschi , A. Zheludev , H. -R. Ott , J. Mesot

We present a combined computational and experimental study of Nb$_3$Cl$_8$, a correlated layered material containing Nb trimers, through the lens of competing intra- and intercluster interactions. Different proposed explanations for its…

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

Strongly Correlated Electrons · Physics 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee