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We present local probe results on the honeycomb lattice antiferromagnet Ba3CuSb2O9. Muon spin relaxation measurements in zero field down to 20 mK show unequivocally that there is a total absence of spin freezing in the ground state. Sb NMR…

Strongly Correlated Electrons · Physics 2015-06-05 J. A. Quilliam , F. Bert , E. Kermarrec , C. Payen , C. Guillot-Deudon , P. Bonville , C. Baines , H. Luetkens , P. Mendels

We determined the crystal structure of Ba$_2$CoSi$_2$O$_6$Cl$_2$, which was synthesized in this work, and investigated its quantum magnetic properties using single crystals. This compound should be described as a two-dimensionally coupled…

The compounds A$_2$Cu$_3$O(SO$_4$)$_3$ (A=Na, K) are characterized by copper hexamers which are weakly coupled to realize antiferromagnetic order below TN=3 K. They constitute novel quantum spin systems with S=1 triplet ground-states. We…

Strongly Correlated Electrons · Physics 2020-06-16 A. Furrer , A. Podlesnyak , J. M. Clemente-Juan , E. Pomjakushina , H. U. Guedel

In this article, we consider the heterodinuclear complex [Ni(dpt)(H2O)Cu(pba)].2H2O [pba =1,3-propylenebis(oxamato) and dpt = bis-(3-aminopropyl)amine] realized through the theoretical model of mixed spin-(1/2,1) coupled via Heisenberg…

Quantum Physics · Physics 2022-11-30 S. Bhuvaneswari , R. Radha , R. Muthuganesan

Single crystals of Ba_{1-x}Rb_{x}Fe_2As_2 with x=0.05-0.1 have been grown from Sn flux and are bulk superconductors with T_c up to 23 K. The crystal structure was determined by X-ray diffraction analysis, and Sn is found to be incorporated…

Superconductivity · Physics 2009-04-07 Z. Bukowski , S. Weyeneth , R. Puzniak , P. Moll , S. Katrych , N. D. Zhigadlo , J. Karpinski , H. Keller , B. Batlogg

We report on the magnetic properties of HoCo dimers as a model system for the smallest intermetallic transition metal-lanthanide compound. The dimers are adsorbed on ultrathin MgO(100) films grown on Ag(100). New for $4f$ elements, we…

Atomic and Molecular Clusters · Physics 2018-12-26 A. Singha , F. Donati , F. D. Natterer , C. Wäckerlin , S. Stavrić , Z. S. Popović , {Ž}. {Š}ljivan{č}anin , F. Patthey , H. Brune

We present the results of muon-spin spectroscopy ($\mu^{+}$SR) measurements on the molecular spin ladder system (Hpip)$_{2}$CuBr$_{4(1-x)}$Cl$_{4x}$, [Hpip=(C$_{5}$H$_{12}$N)]. Using transverse field $\mu^{+}$SR we are able to identify…

We devise a formalism to investigate in a systematic way the spectroscopic magnetic excitations in molecular magnets. This consists in introducing a bilinear spin Hamiltonian that allows for discrete coupling parameters accounting for…

Strongly Correlated Electrons · Physics 2018-05-04 M. Georgiev , H. Chamati

Dimers are the smallest chemical objects that show magnetic anisotropy. We focus on 3$d$ and 4$d$ transition metal dimers that have magnetic ground states in most cases. Some of these magnetic dimers have a considerable barrier against…

Atomic and Molecular Clusters · Physics 2008-04-09 Daniel Fritsch , Klaus Koepernik , Manuel Richter , Helmut Eschrig

Using the exact solution in terms of the generalized classical transfer matrix method we presented a detailed analysis of the magnetic properties and ground state structure of the simplified model of the single-chain magnet, trimetallic…

Statistical Mechanics · Physics 2014-03-12 Stefano Bellucci , Vadim Ohanyan , Onofre Rojas

We report on an extended fluctuation regime in the spin dimer system Sr3Cr2O8 based on anomalies in Raman active phonons and magnetic scattering. The compound has two characteristic temperatures, TS = 275 K, related to a Jahn-Teller…

Hexagonal RMnO3 is a multiferroic compound with a giant spin-lattice coupling at an antiferromagnetic transition temperature [1]. Despite extensive studies over the past two decades, however, the origin and underlying microscopic mechanism…

Strongly Correlated Electrons · Physics 2017-03-08 Seongil Choi , Hasung Sim , Sunmin Kang , Ki-Young Choi , Je-Geun Park

First-principles calculations are used to gauge different levels of approximation to calculate the magnetocrystalline anisotropy energies (MAE) of five $L1_0$ FeMe alloys (Me=Co, Cu, Pd, Pt, Au). We find that a second-order perturbation…

Materials Science · Physics 2020-12-14 M. Blanco-Rey , J. I. Cerda , A. Arnau

The recent breakthrough discovery of twisted bilayer $CrI_3$ system, where both ferromagnetic and antiferromagnetic order coexist and act as a main motivation for simulating simple magnetic systems where this type of mixed-phase arises.…

Statistical Mechanics · Physics 2023-12-27 Nepal Banerjee

The magnetic interactions in La{0.70}Ca{0.30}Mn{1-x}Cr{x}O{3} (x = 0.15, 0.50 and 0.70) are investigated by x-ray absorption spectroscopy (XAS), x-ray magnetic circular dichroism (XMCD), high-resolution x-ray powder diffraction, and bulk…

Materials Science · Physics 2012-04-27 H. Terashita , J. C. Cezar , F. M. Ardito , L. F. Bufaical , E. Granado

Ba4NbIr3O12, a previously unreported material with a triangular planar geometry of Ir3O12 trimers, is described. Magnetic susceptibility measurements show no magnetic ordering down to 1.8 K despite the Curie-Weiss temperature of -13 K. The…

Strongly Correlated Electrons · Physics 2019-01-30 Loi T. Nguyen , R. J. Cava

Spin-1/2 compounds A3Cu3AlO2(SO4)4 (A=K, Rb, and Cs) have one-dimensional (1D) inequilateral diamond chains. We analyze the temperature dependence of the magnetic susceptibility and determine the magnetic exchange interactions. In contrast…

Nuclear magnetic resonance (NMR) study of the high magnetic field (H) part of the Bose-Einstein condensed (BEC) phase of the quasi-onedimensional (quasi-1D) antiferromagnetic quantum spin-chain compound NiCl2-4SC(NH2)2 (DTN) was performed.…

The magnetic behaviour of the low-dimensional Vanadium-oxides Sr2V3O9 and Ba2V3O9 was investigated by means of magnetic susceptibility and specific heat measurements. In both compounds, the results can be very well described by an S=1/2…

Condensed Matter · Physics 2009-11-07 E. E. Kaul , H. Rosner , V. Yushankhai , J. Sichelschmidt , R. V. Shpanchenko , C. Geibel

The recently discovered superconductivity in MgB2 has captured world attention due to its simple crystal structure and relatively high superconducting transition temperature Tc=39K. It appears to be generally accepted that it is…

Superconductivity · Physics 2009-11-07 A. I. Posazhennikova , T. Dahm , K. Maki