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We explore the magnetic properties of isolated a-b planes of trinuclear organometallic crystals, Mo3S7(dmit)3, in which an interplay of strong electronic correlations and spin molecular-orbital coupling (SMOC) occurs. The magnetic…

Strongly Correlated Electrons · Physics 2018-11-01 J. Merino , A. C. Jacko , A. L. Khosla , A. Ralko , B. J. Powell

We report the structural and magnetic properties of the 4}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Rh) based and 5}\textit{\textcolor{black}{d }}\textcolor{black}{(M = Ir) based systems Ba$_{3}$M$_{x}$Ti$_{3-x}$O$_{9}$…

Strongly Correlated Electrons · Physics 2017-08-03 R. Kumar , D. Sheptyakov , P. Khuntia , K. Rolfs , P. G. Freeman , H. M. Rønnow , Tusharkanti Dey , M. Baenitz , A. V. Mahajan

We have performed high-field magnetization and ESR measurements on Ba$_3$CoSb$_2$O$_9$ single crystals, as a representative two-dimensional spin-1/2 Heisenberg antiferromagnet on a uniform triangular lattice, and have determined all the…

Strongly Correlated Electrons · Physics 2015-06-15 Takuya Susuki , Nobuyuki Kurita , Takuya Tanaka , Hiroyuki Nojiri , Akira Matsuo , Koichi Kindo , Hidekazu Tanaka

Low-temperature magnetization (M) measurements down to 0.1 K have been performed in magnetic fields up to 14.5 T for a single piece of a tiny single-crystalline sample (0.2 mg weight) of the spin-gap system YbAl3C3. At the base temperature…

Strongly Correlated Electrons · Physics 2013-07-15 Shunichiro Kittaka , Tomoyoshi Sugiyama , Yasuyuki Shimura , Toshiro Sakakibara , Saori Matsuda , Akira Ochiai

The quantum dimer magnet (QDM) is the canonical example of quantum magnetism. The QDM state consists of entangled nearest-neighbor spin dimers and often exhibits a field-induced triplon Bose-Einstein condensate (BEC) phase. We report on a…

Strongly Correlated Electrons · Physics 2019-07-11 Gavin Hester , H. S. Nair , T. Reeder , D. R. Yahne , T. N. DeLazzer , L. Berges , D. Ziat , J. R. Neilson , A. A. Aczel , G. Sala , J. A. Quilliam , K. A. Ross

The metallic kagome compound Sc$_3$Mn$_3$Al$_7$Si$_5$ has attracted attention as a candidate platform where geometric frustration and itinerant electrons may cooperate to stabilize a quantum-disordered magnetic ground state. Here, we…

Strongly Correlated Electrons · Physics 2025-12-03 R. Guehne , A. K. Sharma , P. Yanda , J. Noky , J. Sichelschmidt , R. Koban , W. Schnelle , C. Shekhar , M. Baenitz , C. Felser

We use NMR techniques to investigate the magnetic properties of BaCo2As2 single crystals, the non-superconducting end member of the Co-substituted iron-pnictide high Tc superconductor Ba(Fe1-xCox)2As2 with x = 1. We present 75As NMR…

Superconductivity · Physics 2015-06-22 K. Ahilan , T. Imai , A. S. Sefat , F. L. Ning

Recently a new class of quantum magnets, the so-called breathing pyrochlore spin systems, have attracted much attention due to their potential to host exotic emergent phenomena. Here, we present magnetometry, heat capacity, thermal…

Magnetic behavior of a spin-1 Heisenberg dimer is analysed in dependence on both uniaxial single-ion anisotropy and XXZ exchange anisotropy in a zero- as well as non-zero longitudinal magnetic field. A complete set of eigenfunctions and…

Materials Science · Physics 2007-05-23 J. Strecka , M. Jascur , M. Hagiwara , Y. Narumi , J. Kuchar , S. Kimura , K. Kindo

The structure and magnetic interactions of the triplon Bose-Einstein condensation candidates Ba$_3$Cr$_2$O$_8$ and Sr$_3$Cr$_2$O$_8$ have been studied thoroughly in the literature, but little is known about a possible triplon condensation…

Strongly Correlated Electrons · Physics 2016-03-23 Henrik Grundmann , Alsu Gazizulina , Fabian von Rohr , Laurens Peters , Tobias Förster , Andreas Schilling

The dimerized S=1/2 spins of the Cu ions in TlCuCl3 are ordered antiferromagnetically in the presence of a field larger than about 54 kOe in the zero-temperature limit. Within the mean-field approximation all thermal effects are frozen out…

Strongly Correlated Electrons · Physics 2015-05-13 Jens Jensen , Henrik Smith

Magnetic anisotropy (MA) is one of the most important material properties for modern spintronic devices. Conventional manipulation of the intrinsic MA, i.e. magnetocrystalline anisotropy (MCA), typically depends upon crystal symmetry.…

High-Curie-temperature ferromagnets are promising candidates for designing new spintronic devices. Here we have successfully synthesized a single-crystal sample of the itinerant ferromagnet Mn$ _{5}$Ge$_{3}$ used flux method and its…

Single crystals of the spin dimer system Sr3Cr2O8 have been grown for the first time. Magnetization, heat capacity, and magnetocaloric effect data up to 65 T reveal magnetic order between applied fields of Hc1 ~ 30.4 T and Hc2 ~ 62 T. This…

CsFeBr$_3$ is an $S\,{=}\,1$ hexagonal antiferromagnet that has a singlet ground state owing to its large easy-plane single-ion anisotropy. The critical behavior of the magnetic-field-induced phase transition for a magnetic field parallel…

Strongly Correlated Electrons · Physics 2017-10-11 Kazuki Shirasawa , Nobuyuki Kurita , Hidekazu Tanaka

Measurements of proton NMR and the spin lattice relaxation rate 1/T1 in the octanuclear iron (III) cluster [Fe8(N3C6H15)6O2(OH)12][Br8 9H2O], in short Fe8, have been performed at 1.5 K in a powder sample aligned along the main anisotropy z…

Materials Science · Physics 2009-11-10 Y. Furukawa , K. Aizawa , K. Kumagai , R. Ullu , A. Lascialfari , F. Borsa

The heterobimetallic metallacrown (MC), (TMA)$_2${Mn(OAc)$_2$[12-MC$_{Mn(III)Cu(II)N(shi)}$-4](CH$_3$OH)}$\cdot$2.90CH$_3$OH, 1, where TMA$^+$ is tetramethylammonium, $^-$OAc is acetate, and shi$^{3-}$ is salicylhydroximate, consists of a…

Mesoscale and Nanoscale Physics · Physics 2022-03-04 A. J. Lewis , E. Garlatti , F. Cugini , M. Solzi , M. Zeller , S. Carretta , C. M. Zaleski

The minerals A2Cu3O(SO4)3 (A2=Na2, NaK, K2) constitute quantum spin systems with copper hexamers as basic structural units. Strong intra-hexamer spin couplings give rise to an effective triplet ground-state. Weak inter-hexamer spin…

Strongly Correlated Electrons · Physics 2021-12-06 A. Furrer , A. Podlesnyak , E. Pomjakushina , V. Pomjakushin

The spin-3/2 Heisenberg antiferromagnet on the bilayer honeycomb lattice is a minimal model to describe the magnetic behavior of Bi$_3$Mn$_4$O$_{12}$(NO$_3$). We study this model with frustrating inter-layer second-neighbor couplings,…

Strongly Correlated Electrons · Physics 2021-12-15 S. Acevedo , C. A. Lamas , P. Pujol

The structure of K2Ni2(MoO4)3 consists of S=1 tetramers formed by Ni^{2+} ions. The magnetic susceptibility chi(T) and specific heat Cp(T) data on a single crystal show a broad maximum due to the low-dimensionality of the system with…

Strongly Correlated Electrons · Physics 2017-06-28 B. Koteswararao , P. Khuntia , R. Kumar , A. V. Mahajan , Arvind Yogi , M. Baenitz , Y. Skourski , F. C. Chou
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