English

Critical behavior in the Mn$_{5}$Ge$_{3}$ ferromagnet

Materials Science 2022-03-25 v1 Strongly Correlated Electrons

Abstract

High-Curie-temperature ferromagnets are promising candidates for designing new spintronic devices. Here we have successfully synthesized a single-crystal sample of the itinerant ferromagnet Mn5 _{5}Ge3_{3} used flux method and its critical properties were investigated by means of bulk dc-magnetization at the boundary between the ferromagnetic (FM) and paramagnetic (PM) phase. Critical exponents β=0.336±0.001 \beta=0.336 \pm 0.001 with a critical temperature Tc=300.29±0.01 T_{c}=300.29 \pm 0.01 K and γ=1.193±0.003 \gamma=1.193 \pm 0.003 with Tc=300.15±0.05 T_{c} = 300.15 \pm 0.05 K are obtained by the modified Arrott plot, whereas δ=4.61±0.03 \delta = 4.61 \pm 0.03 is deduced by a critical isotherm analysis at Tc=300 T_{c} = 300 K. The self-consistency and reliability of these critical exponents are verified by the Widom scaling law and the scaling equations. Further analysis reveals that the spin coupling in Mn5 _{5}Ge3_{3} exhibits three-dimensional Ising-like behavior. The magnetic exchange is found to decay as J(r)r4.855 J(r)\approx r^{-4.855} and the spin interactions are extended beyond the nearest neighbors, which may be related to different set of Mn--Mn interactions with unequal magnitude of exchange strengths. Additionally, the existence of noncollinear spin configurations in Mn5 _{5} Ge3 _{3} results in a small deviation of obtained critical exponents from those for standard 3D-Ising model.

Keywords

Cite

@article{arxiv.2203.12778,
  title  = {Critical behavior in the Mn$_{5}$Ge$_{3}$ ferromagnet},
  author = {Jun-Fa Lin and Huan Wang and Sheng Xu and Xiao-Yan Wang and Xiang-Yu Zeng and Zheng-Yi Dai and Jing Gong and Kun Han and Yi-Ting Wang and Xiao-Ping Ma and Tian-Long Xia},
  journal= {arXiv preprint arXiv:2203.12778},
  year   = {2022}
}

Comments

8 pages, 6 figures. arXiv admin note: substantial text overlap with arXiv:1803.05905 by other authors