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A detailed electronic phase diagram of perovskite-type oxides Sr$_{1-x}$La$_x$FeO$_3$ $(0\leq x \leq 0.5)$ was established by synchrotron X-ray diffraction, magnetization, and transport measurements for polycrystalline samples synthesized…

Strongly Correlated Electrons · Physics 2022-09-15 Masaho Onose , Hidefumi Takahashi , Hajime Sagayama , Yuichi Yamasaki , Shintaro Ishiwata

In this paper, we explore magneteoelectricity of rare earth orthochromites from the symmetry point of view. We determine the principal structural order parameters and find their couplings with ferroelectric and magnetic orderings. Our…

Materials Science · Physics 2021-08-11 A. K. Zvezdin , Z. V. Gareeva , X. M. Chen

First principles density functional calculations for Fe$_{2}$O$_{3}$ has been performed over a wide range of pressures. The ground state is corundum-type hematite and is an antiferromagnetic insulator. This is in good agreement with…

Materials Science · Physics 2009-03-13 Dipta Bhanu Ghosh , Stefano de Gironcoli

In this study, we report a tetragonal perovskite structure of SrIrO$_3$ (P4/mmm, a = 3.9362(9) \r{A}, c = 7.880(3) \r{A}) synthesized at 6 GPa and 1400 $\deg$C, employing the ambient pressure monoclinic SrIrO$_3$ with distorted 6H structure…

We report on the electronic ground state of a layered perovskite vanadium oxide Sr$_2$VO$_4$ studied by the combined use of synchrotron radiation x-ray diffraction (SR-XRD) and muon spin rotation/relaxation ($\mu$SR) techniques, where…

The perovskite oxides are known to be susceptible to structural distortions over a long wavelength when compared to their parent cubic structures. From an ab initio simulation perspective, this requires accurate calculations including many…

Computational Physics · Physics 2022-02-16 Jack S. Baker , Tsuyoshi Miyazki , David R. Bowler

Recently, the perovskite BiCoO$_3$ has been shown experimentally to be isostructural with PbTiO$_3$, while simultaneously the $d^6$ Co$^{3+}$ ion has a high spin ground state with $C$-type antiferromagnetic ordering. Using hybrid density…

Materials Science · Physics 2016-05-04 Leigh Weston , Xiangyuan Cui , Simon P. Ringer , Catherine Stampfl

There has been a rapidly growing interest on the interplay between spin-orbit coupling (SOC) and Hubbard interaction U in correlated materials. A current consensus is that the stronger the SOC, the smaller is the critical interaction Uc…

Strongly Correlated Electrons · Physics 2013-05-30 M. Ahsan Zeb , Hae-Young Kee

Helimagnetic materials are identified as promising for novel spintronic applications. Since helical spin order is manifested as a compromise of competing magnetic exchange interactions, its emergence is limited by unique constraints imposed…

Strongly Correlated Electrons · Physics 2018-08-29 H. Sakai , S. Yokoyama , A. Kuwabara , J. S. White , E. Canévet , H. M. Rønnow , T. Koretsune , R. Arita , A. Miyake , M. Tokunaga , Y. Tokura , S. Ishiwata

We report x-ray diffraction, resistivity, thermopower, and magnetization of Sr3ErMn4-xGaxO10.5-d, in which A-site ordered tetragonal phase appears above x=1, and reveal that the system exhibits typical properties seen in the…

Materials Science · Physics 2015-05-27 W. Kobayashi , T. Ishibashi

The electronic, magnetic and orbital structures of KCrF_3 are determined in all its recently identified crystallographic phases (cubic, tetragonal, and monoclinic) with a set of {\it ab initio} LSDA and LSDA+U calculations. The…

Strongly Correlated Electrons · Physics 2009-11-13 Gianluca Giovannetti , Serena Margadonna , Jeroen van den Brink

The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…

Strongly Correlated Electrons · Physics 2016-08-31 Arata Tanaka

The origin of successive phase transitions observed in the layered perovskite $\alpha$-Sr$_2$CrO$_4$ is studied by the density-functional-theory-based electronic structure calculation and mean-field analysis of the proposed low-energy…

Strongly Correlated Electrons · Physics 2017-02-08 T. Ishikawa , T. Toriyama , T. Konishi , H. Sakurai , Y. Ohta

The electronic, magnetic and optical properties of the double perovskite Sr$_2$CoIrO$_6$ (SCIO) under biaxial strain are explored in the framework of density functional theory (DFT) including a Hubbard $U$ term and spin-orbit coupling (SOC)…

Strongly Correlated Electrons · Physics 2021-11-24 Jiongyao Wu , Marcel Ney , Sebastian Esser , Vijaya Begum , Günther Prinz , Axel Lorke , Philipp Gegenwart , Rossitza Pentcheva

We investigate the electronic and magnetic structures and the character and direction of spin and orbital moments of the recently synthesized quadruple perovskite cobaltovanadate CaCo3V4O12 using a selection of methods from density…

Strongly Correlated Electrons · Physics 2014-11-19 H. B. Rhee , W. E. Pickett

The synthesis and physical properties of the double perovskite (DP) compound Ba2CdReO6 with the 5d1 electronic configuration are reported. Three successive phases originating from a spin-orbit-entangled Jeff = 3/2 state, confirmed by the…

Strongly Correlated Electrons · Physics 2021-04-06 Daigorou Hirai , Zenji Hiroi

We attribute the structural phase transition (SPT) in the parent compounds of the iron pnictides to orbital ordering. Due to the anisotropy of the $d_{xz}$ and $d_{yz}$ orbitals in the $xy$ plane, a ferro-orbital ordering makes the…

Strongly Correlated Electrons · Physics 2013-05-29 Weicheng Lv , Jiansheng Wu , Philip Phillips

The 5d pyrochlore oxide superconductor Cd2Re2O7 (CRO) has attracted significant interest as a spin-orbit-coupled metal (SOCM) that spontaneously undergoes a phase transition to an odd-parity multipole phase by breaking the spatial inversion…

Strongly Correlated Electrons · Physics 2023-09-18 Daigorou Hirai , Atsuhito Fukui , Hajime Sagayama , Takumi Hasegawa , Zenji Hiroi

The crystallographic and magnetic properties of La{0.5+delta}A{0.5-delta}Mn{0.5+epsilon}Ru{0.5-epsilon}O{3} (A= Ca, Sr, Ba) were investigated by means of neutron powder diffraction. All studied samples show the orthorhombic perovskite…

Strongly Correlated Electrons · Physics 2007-05-23 Eduardo Granado , Qingzhen Huang , Jeff W. Lynn , J. Gopalakrishnan , K. Ramesha

Motivated by the unusual features observed in the transport properties of the ferromagnetic "bad metal" $SrRuO_{3}$, we construct a model incorporating essential features of the realistic structure of this nearly cubic material. In…

Strongly Correlated Electrons · Physics 2009-11-07 M. S. Laad , E. Müller-Hartmann