Related papers: Demonstrating coherent control in 85Rb2 using ultr…
Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…
We demonstrate high resolution coherent control of cold atomic Rubidium utilizing spectral phase manipulation of a femtosecond optical frequency comb. Transient coherent accumulation is directly manifested by the enhancement of signal…
We demonstrate the use of the ultrafast spatial coherent-control method to resolve the fine-structure two-photon transitions of atomic rubidium. Counter-propagating ultrafast optical pulses with spectral phase and amplitude programmed with…
The double laser pulse approach to relativistic electron beam (REB) collimation has been investigated at the LULI-ELFIE facility. In this scheme, the magnetic field generated by the first laser-driven REB is used to guide a second delayed…
We explore the effects of ultrafast shaped pulses for two-level systems that do not have a single photon resonance by developing a multiphoton density-matrix approach. We take advantage of the fact that the dynamics of the intermediate…
The controlled transfer of nuclear state population using two x-ray laser pulses is investigated theoretically. The laser pulses drive two nuclear transitions in a nuclear three-level system facilitating coherent population transfer via the…
Experimental realizations of two qubit entangling gates with trapped ions typically rely on addressing spectroscopically resolved motional sidebands, limiting gate speed to the secular frequency. Fast entangling gates using ultrafast pulsed…
We describe an experiment to produce 87Rb Bose-Einstein condensates in an optically plugged magnetic quadrupole trap, using a blue-detuned laser. Due to the large detuning of the plug laser with respect to the atomic transition, the…
We demonstrate optical control of magnons using femtosecond laser pulses by performing ab-initio real-time time-dependent density functional theory (TDDFT) simulations. We predict that the spin-wave dynamics in Fe$_{50}$Ni$_{50}$ can be…
Achieving high-fidelity control of quantum systems is of fundamental importance in physics, chemistry and quantum information sciences. However, the successful implementation of a high-fidelity quantum control scheme also requires…
We investigate computationally a method for ultrafast preparation of alkali metal atoms in their Rydberg states using a three-dimensional model potential in the single active electron approximation. By optimizing laser pulse shapes that can…
Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two…
The ability to control and exploit quantum coherence and entanglement drives research across many fields ranging from ultra-cold quantum gases to spin systems in condensed matter. Transcending different physical systems, optical approaches…
Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…
We investigate the interaction of femtosecond laser pulses with spins including relativistic corrections. The time-ordered magneto-optical signals corresponding to a pump-probe configuration are calculated in the case of one electron…
The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…
In this paper we develop a unified framework to study the coherent control of trapped ions subject to state-dependent forces. Taking different limits in our theory, we can reproduce two different designs of a two-qubit quantum gate --the…
Femtosecond magneto-optical pump-probe measurements of ultrafast demagnetization show an intriguing difference in the first 100 fs of the magneto-optical Kerr response depending on whether the polarization of the pump and probe beams are in…
We present new results on the quantum control of systems with infinitely large Hilbert spaces. A control-theoretic analysis of the control of trapped ion quantum states via optical pulses is performed. We demonstrate how resonant…
We have studied the formation of ultracold RbSr molecules with laser pulses. After discussing the advantages of the Mott insulator phase for the control with pulses, we present two classes of strategies. The first class involves two…