Related papers: Demonstrating coherent control in 85Rb2 using ultr…
Recent quantum technologies have established precise quantum control of various microscopic systems using electromagnetic waves. Interfaces based on cryogenic cavity electro-optic systems are particularly promising, due to the direct…
Coherent single-electron control in a realistic semiconductor double quantum dot is studied theoretically. Using optimal-control theory we show that the energy spectrum of a two-dimensional double quantum dot has a fully controllable…
We study the interaction of a weak probe field, having two orthogonally polarized components, with an optically dense medium of four-level atoms in a tripod configuration. In the presence of a coherent driving laser, electromagnetically…
We report the experimental observation and control of space and time-resolved light-matter Rabi oscillations in a microcavity. Our setup precision and the system coherence are so high that coherent control can be implemented with…
We study the resonant control of two nonreactive polar molecules in an optical lattice site, focussing on the example of RbCs. Collisional control can be achieved by tuning bound states of the intermolecular dipolar potential, by varying…
We demonstrate the formation of a single RbCs molecule during the merging of two optical tweezers, one containing a single Rb atom and the other a single Cs atom. Both atoms are initially predominantly in the motional ground states of their…
Spin precession in Rubidium atoms is investigated through a pump-probe technique. The excited wave packet corresponds to a precession of spin and orbital angular momentum around the total angular momentum. We show that using shaped laser…
We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…
Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the…
We computationally demonstrate a new method for coherently controlling the rotation-axis direction in asymmetric top molecules with an optical centrifuge. Appropriately chosen electric-field strengths and the centrifuge's acceleration rate…
Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant $B\gets X$ transition of iodine $I_2$ is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has…
Optimal control experiments can readily identify effective shaped laser pulses, or "photonic reagents", that achieve a wide variety of objectives. For many practical applications, an important criterion is that a particular photonic reagent…
We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
We theoretically explore photoassociation by Adiabatic Passage of two colliding cold ^{85}Rb atoms in an atomic trap to form an ultracold Rb_2 molecule. We consider the incoherent thermal nature of the scattering process in a trap and show…
We demonstrate quantum entanglement of two trapped atomic ion qubits using a sequence of ultrafast laser pulses. Unlike previous demonstrations of entanglement mediated by the Coulomb interaction, this scheme does not require confinement to…
We explore coherent multi-photon processes in $^{87}$Rb$^{133}$Cs molecules using 3-level lambda and ladder configurations of rotational and hyperfine states, and discuss their relevance to future applications in quantum computation and…
Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…
The coherent superposition of two-atomic levels induced by coherent population trapping is employed in a standard $\Lambda$ type scheme to form a tripod-like system. A weak probe pulse scanning across the system is shown to experience a…
We explore the uses of ultracold molecules as a platform for future experiments in the field of quantum simulation, focusing on two molecular species, $^{40}$Ca$^{19}$F and $^{87}$Rb$^{133}$Cs. We report the development of coherent quantum…