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Related papers: Self-organized patterns of macroscopic quantum tun…

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We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 María José Santander , Alvaro S. Nunez , A. Roldán-Molina , Roberto E. Troncoso

The Coulomb phase, with its dipolar correlations and pinch-point-scattering patterns, is central to discussions of geometrically frustrated systems, from water ice to binary and mixed-valence alloys, as well as numerous examples of…

Multi-spins tunneling cross-relaxations in an ensemble of weakly-coupled Ho$^{3+}$ ions, mediated by weak anisotropic dipolar interactions, can be evidenced by ac-susceptibility measurements in a high temperature regime. Based on a…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 R. Giraud , A. M. Tkachuk , B. Barbara

It is proposed that nuclear (or electron) spins in a trapped molecule would be well isolated from the environment and the state of each spin can be measured by means of mechanical detection of magnetic resonance. Therefore molecular traps…

Quantum Physics · Physics 2007-05-23 Haiqing Wei , Xin Xue

The manipulation of single spins through spin-polarized tunneling opens new routes for quantum control at the atomic scale. We present a theoretical framework describing spin-transfer, spin torques and spin resonance in molecular quantum…

We report spin-pair tunneling observed in Mn$_3$ single-molecule magnet, which is a crystal with 2D network of identical exchange coupling. We observed a series of extra quantum tunnelings by the ac susceptibility measurements, and…

Mesoscale and Nanoscale Physics · Physics 2014-11-04 Yan-Rong Li , Rui-Yuan Liu , Yun-Ping Wang

The theory for the quantum tunneling of nano-magnets is developed within the intermediate spin framework. Periodic magnetic effects are seen to reflect that associated with a change of flux by a single flux quantum $\Phi_{0}$. Essential are…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 S. E. Barnes

The phenomenon of Quantum Tunneling of Mesoscopic Spins is reviewed in the light of the behavior of the archetype of these systems: the molecular complex Mn12-ac. Most observations can be understood in the framework of the reduced Hilbert…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 B. Barbara , I. Chiorescu , R. Giraud , A. G. M. Jansen , A. Caneschi

The control of spin-orbit coupling (SOC) at the microscopic level has become a major research quest within the magnetism and spintronics communities. Altering the interaction between the spin and orbital degrees of freedom can fundamentally…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 James H. Atkinson , Ross Inglis , Enrique del Barco , Euan K. Brechin

We demonstrate that transport spectroscopy of single molecular magnets shows signatures of quantum tunneling at low temperatures. We find current and noise oscillations as function of bias voltage due to a weak violation of spin selection…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , H. Schoeller

The swept-field experiments on magnetic molecular solids such as \Fe8 are studied using Monte Carlo simulations. A kinetic equation is developed to understand the phenomenon. It is found that the simulations provide a quantitatively…

Statistical Mechanics · Physics 2015-10-14 Erik Lenferink , Avinash Vijayaraghavan , Anupam Garg

Magnonic crystals with locally alternating properties and specific periodicities exhibit interesting effects, such as a multitude of different spin-wave states and large band gaps. This work aims for demonstrating and understanding the key…

Theory of magnetic deflagration taking into account dipolar-controlled spin tunneling has been applied to the realistic model of molecular magnet Mn_12 Ac. At small transverse field, the front speed v has tunneling maxima on the bias field…

Statistical Mechanics · Physics 2014-01-07 D. A. Garanin , Saaber Shoyeb

In a previous work (PRL 87, 140405), we have shown that a spinor condensate confined in a periodic or double-well potential exhibits ferromagnetic behavior due to the magnetic dipole-dipole interactions between different wells, and in the…

Soft Condensed Matter · Physics 2009-11-07 Han Pu , Weiping Zhang , Pierre Meystre

The nuclear spin-mediated quantum relaxation of ensembles of tunneling magnetic molecules causes a 'hole' to appear in the distribution of internal fields in the system. The form of this hole, and its time evolution, are studied using Monte…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 I. S. Tupitsyn , P. C. E. Stamp , N. V. Prokof'ev

The synthesis of molecular magnets has undergone rapid progress in recent years. Each of the identical molecular units can contain as few as two and up to several dozens of paramagnetic ions (spins). Although these materials appear as…

Strongly Correlated Electrons · Physics 2009-11-11 J. Schnack

We report on the Fe17 high-spin molecular cluster and show that this system is an exemplification of nanostructured dipolar magnetism. Each Fe17 molecule, with spin S=35/2 and axial anisotropy as small as D=-0.02K, is the magnetic unit that…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 M. Evangelisti , A. Candini , A. Ghirri , M. Affronte , G. W. Powell , I. A. Gass , P. A. Wood , S. Parsons , E. K. Brechin , D. Collison , S. L. Heath

We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation…

Condensed Matter · Physics 2009-10-30 Nikolai Prokof'ev , Philip Stamp

In this work, we explore the magnetic behavior of diluted spin-ice systems, where magnetic moments are randomly removed at various concentrations. We concentrate on features in which the effect of long range dipolar interactions (usually…

Statistical Mechanics · Physics 2024-11-08 M. Gorsd , S. A. Grigera , R. A. Borzi