We argue that to explain recent resonant tunneling experiments on crystals of Mn12 and Fe8, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-T, short-time relaxation will then have a t/τ form, where τ depends on the nuclear T2, on the tunneling matrix element Δ10 between the two lowest levels, and on the initial distribution of internal fields in the sample, which depends very strongly on sample shape. The results are directly applicable to the Fe8 system. We also give some results for the long-time relaxation.
@article{arxiv.cond-mat/9710246,
title = {Low-Temperature Quantum Relaxation in a System of Magnetic Nanomolecules},
author = {Nikolai Prokof'ev and Philip Stamp},
journal= {arXiv preprint arXiv:cond-mat/9710246},
year = {2009}
}