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Transport and non-equilibrium magnetization in monolayers of magnetic molecules subject to a bias voltage are considered. We apply a master-equation approach going beyond the sequential-tunneling approximation to study the Coulomb-blockade…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Florian Elste , Carsten Timm

We have shown that the size of the magnetization step due to resonant spin tunneling in a molecular magnet can be strongly affected by sound. The transverse acoustic wave can also generate macroscopic quantum beats of the magnetization…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Gwang-Hee Kim , E. M. Chudnovsky

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Florian Elste , Carsten Timm

We show that resonant quantum tunneling of the magnetization, until now observed only in zero-dimensional (0D) cluster systems, occurs in the molecular Ising spin chain $[(CH_3)_3NH]CoCl_3\cdot 2H_2O$, which orders as a canted…

Materials Science · Physics 2007-05-23 E. Lhotel , E. N. Khatsko , C. Paulsen

We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic…

Statistical Mechanics · Physics 2007-05-23 J. F. Fernandez , J. J. Alonso

We have mapped out a detailed phase diagram that shows the ground state structure of a spin-1 condensate with magnetic dipole-dipole interactions. We show that the interplay between the dipolar and the spin-exchange interactions induces a…

Other Condensed Matter · Physics 2009-11-11 S. Yi , H. Pu

We have developed a quantitative theory of resonant tunneling of magnetic flux between discrete macroscopically distinct quantum states in SQUID systems. The theory is based on the standard density-matrix approach. Its new elements include…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 D. V. Averin , Jonathan R. Friedman , J. E. Lukens

We report experimental studies of crystals of Mn12 molecular magnetic clusters in pulsed magnetic fields with sweep rates up to 4x10^3 T/s. The steps in the magnetization curve are observed at fields that are shifted with respect to the…

Other Condensed Matter · Physics 2009-11-10 J. Vanacken , S. Stroobants , M. Malfait , V. V. Moshchalkov , M. Jordi , J. Tejada , R. Amigo , E. M. Chudnovsky , D. A. Garanin

Current theories still fail to give a satisfactory explanation of the observed quantum phenomena in the relaxation of the magnetisation of the molecular cluster Mn12 acetate. In the very low temperature regime, Prokof'ev and Stamp recently…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 W. Wernsdorfer , R. Sessoli , D. Gatteschi

Decay of metastable states in molecular magnets (MM) leads to energy release that results in temperature increase that, in turn, positively affects the decay rate. This is the mechanism of recently discovered magnetic deflagration that is…

Mesoscale and Nanoscale Physics · Physics 2014-01-07 D. A. Garanin

The quantum tunneling of the magnetization vector between excited levels are studied theoretically in single-domain ferromagnetic nanoparticles with biaxial crystal symmetry placed in an external magnetic field at an arbitarily directed…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Rong Lu , Su-Peng Kou , Jia-Lin Zhu , Lee Chang , Bing-Lin Gu

Spin tunneling in molecular magnets has attracted much attention, however theoretical considerations of this phenomenon up to now have not taken into account the many-spin nature of molecular magnets. We present, to our knowledge, the first…

Materials Science · Physics 2009-10-31 M. Al-Saqer , V. V. Dobrovitski , B. N. Harmon , M. I. Katsnelson

We study the self-assembly of magnetic colloids using the Stockmayer (SM) model characterized by short-range Lennard-Jones interactions and long-range dipole-dipole interactions. Using molecular dynamics simulations, we design cooling…

Soft Condensed Matter · Physics 2025-06-30 Anuj Kumar Singh , Sanjay Puri , Varsha Banerjee

We study the semiclassical dynamics of a spinor condensate with the magnetic dipole-dipole interaction included. The time evolution of the population imbalance and the relative phase among different spin components depends greatly on the…

Other Condensed Matter · Physics 2009-11-11 Rong Cheng , J. -Q. Liang , Yunbo Zhang

We report results from Monte Carlo simulations of systems of magnetic dipoles that relax through quantum tunneling, much as Fe_8 crystals at very low temperature.For short times, a hole develops in suitably defined magnetic field…

Condensed Matter · Physics 2007-05-23 J. J. Alonso , J. F. Fernandez

This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…

Mesoscale and Nanoscale Physics · Physics 2013-03-04 Junjie Liu , Enrique del Barco , Stephen Hill

At low densities, electrons confined to two dimensions in a delta-doped heterostructure can arrange themselves into self-consistent droplets due to disorder and screening effects. We use this observation to show that at low temperatures,…

Strongly Correlated Electrons · Physics 2007-10-10 V. Tripathi , M. P. Kennett

Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Hui Hu , Jia-Lin Zhu , Rong Lu , Jia-Jiong Xiong

Ensembles of gold nanoparticles present a magnetic behavior which is at odds with the weakly diamagnetic response of bulk gold. In particular, an unusual ferromagnetic order has been unveiled by several experiments. Here we investigate if…

Mesoscale and Nanoscale Physics · Physics 2022-02-08 Gaëtan J. Percebois , Dietmar Weinmann , Rodolfo A. Jalabert , Guillaume Weick

At high densities fluids of strongly dipolar spherical particles exhibit spontaneous long-ranged orientational order. Typically, due to demagnetization effects induced by the long range of the dipolar interactions, the magnetization…

Soft Condensed Matter · Physics 2009-10-30 B. Groh , S. Dietrich