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We use dynamical mean field theory to find an exact solution for inelastic light scattering in strongly correlated materials such as those near a quantum-critical metal-insulator transition. We evaluate the results for $\textbf{q}=0$…

Strongly Correlated Electrons · Physics 2009-11-10 A. M. Shvaika , O. Vorobyov , J. K. Freericks , T. P. Devereaux

We theoretically investigate several types of plasmonic slot waveguides for enhancing the measured signal in Raman spectroscopy, which is a consequence of electric field and Purcell factor enhancements, as well as an increase in…

Herein we report experimental evidence of directional SERS from molecules situated inside a single nanowire-nanoparticle junction cavity. The emission was confined to a narrow range of wavevectors perpendicular to the axis of the cavity. In…

Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…

Optics · Physics 2020-03-12 Xiaoqin Shen , Hyungwoo Choi , Dongyu Chen , Wei Zhao , Andrea M. Armani

Surface enhanced Raman scattering (SERS) effects on tin dioxide in the form of bulk material, nanostructured thin films and colloidal solutions were investigated. Raman spectra are characterized by the three Raman scattering peaks at 478,…

Materials Science · Physics 2015-06-03 Enza Fazio , Fortunato Neri , Salvatore Savasta , Salvatore Spadaro , Sebastiano Trusso

Resonant coupling of a vibration to a cavity mode has been reported to dramatically modify spontaneous Raman scattering, but subsequent studies have produced conflicting results. In this Letter, we develop a microscopic quantum framework…

Mesoscale and Nanoscale Physics · Physics 2025-11-04 Maxime Dherbécourt , Joël Bellessa , Clémentine Symonds , Guillaume Weick , David Hagenmüller

The Raman scattering of light by molecular vibrations offers a powerful technique to 'fingerprint' molecules via their internal bonds and symmetries. Since Raman scattering is weak, methods to enhance, direct and harness it are highly…

Vibrational Raman scattering -- a process where light exchanges energy with a molecular vibration through inelastic scattering -- is most fundamentally described in a quantum framework where both light and vibration are quantized. When the…

We explain quantitatively why resonant Raman scattering spectroscopy, an extensively used experimental tool in studying elementary electronic excitations in doped low dimensional semiconductor nanostructures, always produces an observable…

Strongly Correlated Electrons · Physics 2009-10-31 S. Das Sarma , Daw-Wei Wang

The optical properties of a concentric nanometer-sized spherical shell comprised of an (active) 3-level gain medium core and a surrounding plasmonic metal shell are investigated. Current research in optical metamaterials has demonstrated…

Optics · Physics 2009-11-13 Joshua A. Gordon , Richard W. Ziolkowski

Surface-Enhanced Raman Scattering (SERS) allows for detection and identification of molecular vibrational fingerprints in minute sample quantities. The SERS process can be also exploited for optical manipulation of molecular vibrations. We…

We suggest and theoretically study the local field enhancement in a metamaterial sample shaped as a pyramid and formed by plasmonic nanoplates alternating with dielectric ones in parallel to the pyramid base. Due to very small thickness of…

Optics · Physics 2010-03-10 Constantin Simovski , Jacek Pniewski

Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

We have investigated the effects of tuning the localized surface plasmon resonances (LSPRs) of silver nanoparticles on the fluorescence intensity, lifetime, and Raman signal from nearby fluorophores. The presence of a metallic structure can…

Other Condensed Matter · Physics 2009-11-13 N. I. Cade , T. Ritman-Meer , D. Richards

Generating a coherent optical frequency comb at an arbitrary wavelength is important for fields such as spectroscopy and optical communications. Dark solitons which are coherent states of optical frequency combs in normal dispersion…

Optics · Physics 2023-08-02 Gwangho Choi , Judith Su

We investigate light scattering by coated spheres composed of a dispersive plasmonic core and a dielectric shell. By writing the absorption cross-section in terms of the internal electromagnetic fields, we demonstrate it is an observable…

Optics · Physics 2015-06-15 Tiago J. Arruda , Alexandre S. Martinez , Felipe A. Pinheiro

We propose an integrated surface enhanced Raman scattering (SERS) chip based on liquid-core waveguide with total reflection, through which the depression of leaky mode enable a long propagating distance. An Raman enhancement factor for…

Optics · Physics 2015-12-08 Chunhong Lai , Gang Chen , Li Chen , Junhui Li , Qinghao Liu , Yi Xu

The scattering of lattice excitations (phonons) with the photoexcited charge carriers is of a major concern in optoelectronic devices. Here, the resonant Raman scattering will be utilized to study an exciton-phonon interaction in GaN…

We model Raman processes in silicene and germanene involving scattering of quasiparticles by, either, two phonons, or, one phonon and one point defect. We compute the resonance Raman intensities and lifetimes for laser excitations between 1…

Materials Science · Physics 2019-01-04 Gergő Kukucska , Viktor Zólyomi , János Koltai

We develop a generic theory for the resonant inelastic light (Raman) scattering by a conduction band quantum plasma taking into account the presence of the filled valence band in doped semiconductor nanostructures within a generalized…

Strongly Correlated Electrons · Physics 2009-11-07 Daw-Wei Wang , S. Das Sarma