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Plasmon-enhanced Raman scattering can push single-molecule vibrational spectroscopy beyond a regime addressable by classical electrodynamics. We employ a quantum electrodynamics (QED) description of the coherent interaction of plasmons and…

We present a systematic theoretical study of the Raman scattering effect for a two-level atomic system in near proximity of an ultrathin dielectric film with an embedded parallel array of periodically aligned single-wall semiconducting…

Mesoscale and Nanoscale Physics · Physics 2026-04-21 SK Firoz Islam , Michael Dean Pugh , Igor V. Bondarev

Raman spectroscopy is a powerful technique to characterize materials. It probes non-destructively chemical composition, crystallinity, defects, strain and coupling phenomena. However, the Raman response of surfaces or thin films is often…

We demonstrate cavity-enhanced Raman emission from a single atomic defect in a solid. Our platform is a single silicon-vacancy center in diamond coupled with a monolithic diamond photonic crystal cavity. The cavity enables an unprecedented…

The conventional explanation of plasmon-enhanced Raman scattering attributes the enhancement to the antenna effect focusing the electromagnetic field into sub-wavelength volumes. Here we introduce a new model that additionally accounts for…

Mesoscale and Nanoscale Physics · Physics 2016-02-10 Philippe Roelli , Christophe Galland , Nicolas Piro , Tobias J. Kippenberg

This article presents and discusses the general features and aspects regarding the electromagnetic scattering by a small core-shell plasmonic sphere. First, the thickness effects on the plasmonic resonances are presented in the…

Classical Physics · Physics 2018-02-14 Dimitrios C. Tzarouchis , Ari Sihvola

We investigate how proximity to a metal nanostructure, particularly to a flat mirror or a cavity confined between two mirrors, affects the vibronic structure of Raman scattering signals. We find that such proximity, particularly for the…

Optics · Physics 2026-05-28 Zeyu Zhou , Maxim Sukharev , Abraham Nitzan , Joseph Eli Subotnik

Strong coupling between cavity photons and molecular vibrations can lead to the formation of vibron-polaritons. In a recent experiment with PVAc molecules in a metal-metal microcavity [A.Shalabney et al., Ang.Chem.Int.Ed. 54 7971 (2015)],…

Optics · Physics 2016-08-31 Artem Strashko , Jonathan Keeling

We study Raman scattering in active media placed in proximity of different types of metal nanostructures, at wavelengths that display either Fabry-Perot or plasmonic resonances, or a combination of both. We use a semi-classical approach to…

Optics · Physics 2015-06-05 M. Scalora , M. A. Vincenti , D. de Ceglia , M. Grande , J. W. Haus

We present a scheme to obtain the coherently enhanced Raman scattering in atomic vapor which is induced by a spin wave initially written by a weak write laser. The enhancement of Raman scattering is dependent on the number and the spatial…

Quantum Physics · Physics 2015-05-19 Chun-Hua Yuan , L. Q. Chen , Jietai Jing , Z. Y. Ou , Weiping Zhang

We investigate the interplay of shape changes and localized surface plasmons in small metal particles with the potential of a large enhancement of the Raman signal from the particles own vibrations. The framework is a geometrical one where…

Optics · Physics 2016-01-26 S. P. Apell , G. Mukhopadhyay , Tomasz Antosiewicz , J Aizpurua

The spectral relationships between surface enhanced resonant Raman scattering (SERRS) and plasmon resonance observed in far field scattering cross are investigated using single silver nanoparticle dimers with focusing on the lowest energy…

Optics · Physics 2023-04-07 Tamitake Itoh , Yuko S. Yamamoto

We study light scattering by spherical nanoshells consistent of metal/dielectric composites. We consider two geometries of metallic nanoshell with dielectric core, and dielectric coated metallic nanoparticle. We demonstrate that for both…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 A. E. Miroshnichenko

Light scattering limits the penetration depth of non-invasive Raman spectroscopy in biological media. While safe levels of irradiation may be adequate to analyze superficial tissue, scattering of the pump beam reduces the Raman signal to…

Photonics caught world attention since channel capacity limit of metallic interconnects approached due to research and design in high speed digital processors. Use of dielectrics, instead, suitable for light propagation was more attractive…

Optics · Physics 2024-12-04 Abdurrahman Javid Shaikh , Othman Sidek

Surface-enhanced coherent anti-Stokes Raman scattering (SE-CARS) takes advantage of surface plasmon resonances supported on metallic nanostructures to amplify the coherent Raman response of target molecules. While these metallic antennas…

Optics · Physics 2022-09-07 Shamsul Abedin , Yong Li , Abid Anjum Sifat , Khokan Roy , Eric Olaf Potma

The resonant scattering of surface plasmon-polariton waves by embedded semiconductor quantum dots above the dielectric/metal interface is explored in the strong-coupling regime. In contrast to non-resonant scattering by a localized…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Danhong Huang , Michelle Easter , Godfrey Gumbs , A. A. Maradudin , Shawn-Yu Lin , Dave Cardimona , Xiang Zhang

Nanofibers functionalized by metal nanostructures and particles are exploited as effective flexible substrates for SERS analysis. Their complex three-dimensional structure may provide Raman signals enhanced by orders of magnitude compared…

Materials Science · Physics 2016-03-16 A. Camposeo , D. Spadaro , D. Magrì , M. Moffa , P. G. Gucciardi , L. Persano , O. M. Maragò , D. Pisignano

Based on the concept of complementary media, we propose a novel design which can enhance the electromagnetic wave scattering cross section of an object so that it looks like a scatterer bigger than the scale of the device. Such a…

Optics · Physics 2009-11-13 Tao Yang , Huanyang Chen , Xudong Luo , Hongru Ma

The paper analyzes some experiments on Raman scattering by molecules adsorbed on the face (111) of silver monocrystals performed by A. Campion et al. From the existence of the forbidden line of benzene, the conclusion about existence of the…

Optics · Physics 2015-06-15 A. M. Polubotko