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Magnetodielectric materials are characterized by a strong coupling of magnetic and dielectric properties and in rare cases simultaneously exhibit both, magnetic and polar order. Among other multiferroics, TbMnO3 and GdMnO3 reveal a strong…

Strongly Correlated Electrons · Physics 2015-06-25 A. Pimenov , A. A. Mukhin , V. Yu. Ivanov , V. D. Travkin , A. M. Balbashov , A. Loidl

The electronic valence state of Mn in Pb(Zr0.2Ti0.8)O3/La0.8Sr0.2MnO3 multiferroic heterostructures is probed by near edge x-ray absorption spectroscopy as a function of the ferroelectric polarization. We observe a temperature independent…

Materials Science · Physics 2010-04-13 C. A. F. Vaz , J. Hoffman , Y. Segal , J. W. Reiner , R. D. Grober , Z. Zhang , C. H. Ahn , F. J. Walker

We report inelastic neutron scattering results on the spin dynamics in the 50 % hole-doped manganites, Pr{1/2}Sr{1/2}MnO3 and Nd{1/2}Sr{1/2}MnO3. In the paramagnetic phase, these systems exhibit a ridge-type diffuse scattering, indicating a…

Strongly Correlated Electrons · Physics 2007-05-23 H. Kawano , R. Kajimoto , H. Yoshizawa , Y. Tomioka , H. Kuwahara , Y. Tokura

The crystal and magnetic structure of polycrystalline $La{}_{0.5-x}Nd{}_{x}Ca_{0.5}MnO{}_{3}$ (0.0 \ensuremath{\le} x \ensuremath{\le} 0.5) samples have been investigated using magnetization, resistivity, transmission electron microscope,…

Materials Science · Physics 2010-11-01 Indu Dhiman , A. Das , P. K. Mishra , N. P. Lalla , A. Kumar

We design a multiferroic metal that combines seemingly incompatible ferromagnetism, ferroelectricity, and metallicity by hole doping a two-dimensional (2D) ferroelectric with high density of states near the Fermi level. The strong…

Materials Science · Physics 2021-08-12 Xu Duan , Jiawei Huang , Bin Xu , Shi Liu

Collinear dipole orders such as ferroelectricity and antiferroelectricity have developed rapidly in last decades. While, the noncollinear dipole orders are rarely touched in solids. Noncollinear dipole orders can provide a route to realize…

Materials Science · Physics 2024-11-01 Xinyu Yang , Jun Chen , Shan-Shan Wang , Shuai Dong

By means of magnetic, specific heat and pyroelectric measurements, we report on magnetic ferroelectricity in the quadruple perovskite \namno, characterized by a canted antiferromagnetic (AFM) CE structure. Surprisingly, ferroelectricity is…

Based on ab initio density functional theory, we have investigated a microscopic mechanism that leads to Fe$^{2+}_{B}$/Fe$^{3+}_{B}$ dimerization and consequent ferroelectricity in charge ordered Fe$_{3}$O$_{4}$ with $P2$ symmetry. In…

Materials Science · Physics 2009-12-15 Tetsuya Fukushima , Kunihiko Yamauchi , Silvia Picozzi

In this letter, we report the structural, electronic and ferroelectric properties of the layered mixed-valent transition-metal compound, Sr$_{4}$Fe$_{6}$O$_{12}$ (SFO). We demonstrate how SFO undergoes a phase transition from a…

Strongly Correlated Electrons · Physics 2025-02-05 Arindam Sarkar , Hena Das , Prashant Singh , Aftab Alam

We report the remarkably robust ferroelectric state in the multiferroic compound Mn$_{1-x}$Zn$_x$WO$_4$. The substitution of the magnetic Mn$^{2+}$ with nonmagnetic Zn$^{2+}$ reduces the magnetic exchange and provides control of the various…

Strongly Correlated Electrons · Physics 2011-01-12 R. P. Chaudhury , F. Ye , J. A. Fernandez-Baca , B. Lorenz , Y. Q. Wang , Y. Y. Sun , H. A. Mook , C. W. Chu

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

Strongly Correlated Electrons · Physics 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

Spin, charge, and orbital structures in models for doped manganites are studied by a combination of analytic mean-field and numerical relaxation techniques. At realistic values for the electron-phonon and antiferromagnetic $t_{2g}$ spin…

Strongly Correlated Electrons · Physics 2009-10-31 Takashi Hotta , Elbio Dagotto

The electron spin polarization on half-metallic double-perovskites is usually conditioned to the ordered rock-salt arrangement of the transition-metal ions along the lattice. In this work, we investigate a polycrystalline sample of the…

We have investigated dielectric properties in a series of crystals of $R$MnO$_{3}$ ($R$ is a rare earth ion) under magnetic fields and quasihydrostatic pressure. We have found that ferroelectric phase appeared in GdMnO$_3$ crystal below…

Strongly Correlated Electrons · Physics 2009-11-10 H. Kuwahara , K. Noda , J. Nagayama , S. Nakamura

Using the first-principles density-functional theory plan-wave pseudopotential method, we investigate the structure and magnetism in 25% Mn substitutive and interstitial doped monoclinic, tetragonal and cubic ZrO2 systematically. Our…

Materials Science · Physics 2015-05-13 Xingtao Jia , Wei Yang , Minghui Qin , Jianping Li

Multiferroics are materials with coexisting electric and magnetic orders that are of central importance for fundamental research and technological applications. Unfortunately, intrinsic multiferroics that operate at room temperature remain…

Materials Science · Physics 2025-11-06 Ping Tang , Gerrit E. W. Bauer

We study an effective one-dimensional (1D) orbital t-J model derived for strongly correlated e_g electrons in doped manganites. The ferromagnetic spin order at half filling is supported by orbital superexchange prop. to J which stabilizes…

Strongly Correlated Electrons · Physics 2009-11-11 M. Daghofer , A. M. Oles , W. von der Linden

The coupling between magnetic order and ferroelectricity has been under intense investigation in a wide range of transition-metal oxides. The strongest coupling is obtained in so-called magnetically-induced multiferroics where…

Materials Science · Physics 2015-05-13 V. S. Zapf , M. Kenzelmann , F. Wolff-Fabris , F. Balakirev , Y. Chen

The low-temperature properties of the so-called ''charge ordered'' state in 50% doped perovskite manganites are described from the viewpoint of the magnetic spin ordering. In these systems, the zigzag antiferromagnetic ordering, combined…

Strongly Correlated Electrons · Physics 2007-05-23 I. V. Solovyev

We investigate the possibility of controlling the magnetic phase transition of the heterointerface between a half-doped manganite La$_{0.5}$Ca$_{0.5}$MnO$_{3}$ and a multiferroic BiFeO$_{3}$ through magnetoelectric coupling. Using…

Strongly Correlated Electrons · Physics 2015-06-17 Di Yi , Jian Liu , Satoshi Okamoto , Suresha Jagannatha , Yi-Chun Chen , Pu Yu , Ying-Hao Chu , Elke Arenholz , R. Ramesh