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A series of manganites Tb1-xHoxMnO3 (0<=x<=0.6) with orthorhombic structure are synthesized and detailed investigations on their multiferroicity are performed. Successive magnetic transitions upon temperature variation are evidenced for all…

Strongly Correlated Electrons · Physics 2010-04-19 C. L. Lu , S. Dong , K. F. Wang , J. -M. Liu

In multiferroic TbMn$_2$O$_5$, the behavior of the terbium ions forms a crucial part of the magneto-electric coupling. The result is a magnetically induced reversal of the electric polarization at 2 T. In this article we present the first…

Strongly Correlated Electrons · Physics 2011-06-27 R. D. Johnson , C. Mazzoli , S. R. Bland , C-H. Du , P. D. Hatton

Obtaining strong magnetoelectric couplings in bulk materials and heterostructures is an ongoing challenge. We demonstrate that manganite heterostructures of the form ${\rm (Insulator)/(LaMnO_3)_n/(CaMnO_3)_n/(Insulator)}$ show strong…

Strongly Correlated Electrons · Physics 2017-02-22 Sanjukta Paul , Ravindra Pankaj , Sudhakar Yarlagadda , Pinaki Majumdar , Peter B. Littlewood

Obtaining strong magnetoelectric couplings in bulk materials and heterostructures is an ongoing challenge. We demonstrate that manganite heterostructures of the form ${\rm (Insulator)/(LaMnO_3)_n/(CaMnO_3)_n/(Insulator)}$ show strong…

Strongly Correlated Electrons · Physics 2017-11-22 Sanjukta Paul , Ravindra Pankaj , Sudhakar Yarlagadda , Pinaki Majumdar , Peter B. Littlewood

Density functional theory calculations have been performed for the structural, electronic, magnetic and ferroelectric properties of a mixed-valence Fe(II)-Fe(III) formate framework [NH$_2$(CH$_3$)$_2$][Fe$^{\rm III}$Fe$^{\rm II}$(HCOO)$_6$]…

Materials Science · Physics 2019-10-15 Gang Tang , Wei Ren , Jiawang Hong , Alessandro Stroppa

We consider theoretically the possibility of coexisting ferroelectric and metallic altermagnetic order, which has recently been predicted in insulating and semiconducting systems via ab initio calculations. Solving self-consistently a…

Materials Science · Physics 2025-10-31 Chi Sun , Jacob Linder

A mechanism for charge-ordered ferromagnetic phase in manganites is proposed. The mechanism is based on the double exchange in the presence of diagonal disorder. It is modeled by a combination of the Ising double-exchange and the…

Strongly Correlated Electrons · Physics 2009-11-10 Tran Minh-Tien

Multiferroics are compounds in which at least two ferroic orders coexist - typically (anti)ferromagnetism and ferroelectricity. While magnetic order can arise in both insulating and conducting compounds, ferroelectricity is in principle not…

Self-interaction corrected local spin density approximation calculations were performed for La$_{(1-x)}$Sr$_x$MnO$_3$ (LSMO) ($0.0<x<0.5$). The influence and inter-relationship of Sr doping, magnetic structure, O displacements and phase…

Strongly Correlated Electrons · Physics 2009-11-10 G. Banach , W. M. Temmerman

We put forward double perovskites of the R$_2$NiMnO$_6$ family (with $R$ a rare-earth atom) as a new class of multiferroics on the basis of {\it ab initio} density functional calculations. We show that changing $R$ from La to Y drives the…

Strongly Correlated Electrons · Physics 2015-05-14 Sanjeev Kumar , Gianluca Giovannetti , Jeroen van den Brink , Silvia Picozzi

Using the degenerate double exchange Hamiltonian with on-site Coulomb interactions we show that there is an instability towards the displacement of the manganese ion in La_{1-x}Ca_{x}MnO_{3}. The result is a dipole moment due to the charge…

Strongly Correlated Electrons · Physics 2007-05-23 E. R. Sanchez Guajardo

Recently, we predicted based on symmetry considerations that KMnFeF$_{6}$ and Ba$_{2}$Ni$_{7}$F$_{18}$ are likely magnetoelectric multiferroic materials. In this contribution, we investigate with Landau theory and crystal structure…

Materials Science · Physics 2009-11-13 G. Nénert

The coupling between ferroelectrics and magnetism presents a promising avenue for low-dissipation spintronic devices. However, such couplings remain rare, and the direct realization of magnetic order driven by ferroelectric switching in…

We show that electronic correlations decimate the intrinsic ferroelectric polarization of the recently discovered class of multiferroic manganites RMn$_2$O$_5$, where R is a rare earth element. Such is manifest from {\it ab initio}…

Materials Science · Physics 2009-11-13 Gianluca Giovannetti , Jeroen van den Brink

The future of spintronic and semiconductor applications demands materials with tailored electronic and magnetic properties. This study uses density functional theory to investigate the electronic structure of the half-metallic compound…

Materials Science · Physics 2025-07-08 Sujoy Datta , Prashant Singh

The number of magnetoelectric multiferroic materials reported to date is scarce, as magnetic structures that break inversion symmetry and induce an improper ferroelectric polarization typically arise through subtle competition between…

We have carried out a first-principles theoretical study of the magnetically induced polarization in orthorhombic TbMnO3, a prototypical material in which a cycloidal spin structure generates an electric polarization via the spin-orbit…

Materials Science · Physics 2009-12-16 Andrei Malashevich , David Vanderbilt

Optically-induced phase transitions of the manganite $\rm Pr_{1/3}Ca_{2/3}MnO_3$ have been simulated using a model Hamiltonian, that captures the dynamics of strongly correlated charge, orbital, lattice, and spin degrees of freedom. Its…

Strongly Correlated Electrons · Physics 2020-12-01 Sangeeta Rajpurohit , Liang Z. Tan , Christian Jooss , P. E. Blöchl

Using a combination of Density Functional Theory, mean-field analysis and exact diagonalization calculations we reveal the emergence of a dimerized charge ordered state in TMTTF$_2$-PF$_6$ organic crystal. The interplay between charge and…

Strongly Correlated Electrons · Physics 2015-03-19 Gianluca Giovannetti , Sanjeev Kumar , Jean-Paul Pouget , Massimo Capone

Based on a two-dimensional extended Hubbard model with electron-phonon interaction, we have studied the effect of polaron formation on the charge ordering (CO) transition. It is found that for fully ferromagnetically ordered spins the CO…

Strongly Correlated Electrons · Physics 2009-10-31 Qingshan Yuan , Peter Thalmeier
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