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Related papers: Field-free molecular alignment induced by elliptic…

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We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

We experimentally investigate generation of molecular nitrogen-ion lasers with two femtosecond laser pulses at different wavelengths. The first pulse serves as the pump which ionizes the nitrogen molecules and excites the molecular ions to…

A recent paper reported elliptically polarized high-order harmonics from aligned N$_2$ using a linearly polarized driving field [X. Zhou \emph{et al.}, Phys. Rev. Lett. \textbf{102}, 073902 (2009)]. This observation cannot be explained in…

Atomic Physics · Physics 2010-03-29 Adam Etches , Christian Bruun Madsen , Lars Bojer Madsen

We report the observation of a novel nonlinear optical response from the prototypical three-dimensional topological insulator Bi$_2$Se$_3$ through the process of high-order harmonic generation. We find that the generation efficiency…

We consider the formation of RbCs by an elliptically polarized laser pulse. By varying the ellipticity of the laser for sufficiently large laser intensity, we see that the formation probability presents a strong dependence, especially…

Atomic Physics · Physics 2019-02-06 J. Pablo Salas , Cristel Chandre , J Salas

We theoretically analyze the effectiveness of multiple-pulse laser alignment methods for asymmetric-top molecules. As an example, we choose SO_2 and investigate the alignment dynamics induced by two different sequences, each consisting of…

Atomic Physics · Physics 2010-10-01 Stefan Pabst , Robin Santra

The recent PVLAS experiment observed the rotation of polarization and the ellipticity when a linearly polarized laser beam passes through a transverse magnetic field. The phenomenon cannot be explained in the conventional QED. We attempt to…

High Energy Physics - Phenomenology · Physics 2008-11-26 Xue-Peng Hu , Yi Liao

Free-electron lasers (FELs) have been built ranging in wavelength from long-wavelength oscillators using partial wave guiding through ultraviolet through hard x-ray that are either seeded or start from noise (SASE). In addition, FELs that…

Accelerator Physics · Physics 2017-03-08 H. P. Freund , P. J. M. van der Slot , D. L. A. G. Grimminck , I. D. Setija , P. Falgari

We predict new end-of-pulse behavior in high-field atomic double ionization. Calculations of atomic electron trajectories in short intense laser pulses confirm our analysis of elliptical polarization. We exhibit a four-band structure in ion…

Atomic Physics · Physics 2010-08-20 Xu Wang , J. H. Eberly

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

Short laser pulses are widely used for controlling molecular rotational degrees of freedom and inducing molecular alignment, orientation, unidirectional rotation and other types of coherent rotational motion. To follow the ultra-fast…

We present a theoretical study of the impact of an electrostatic field combined with nonresonant linearly polarized laser pulses on the rotational dynamics of a thermal ensemble of linear molecules. We solve the time-dependent Schr\"odinger…

Quantum Physics · Physics 2015-06-16 Juan J. Omiste , Rosario González Férez

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

Ultrashort laser pulses are widely used for transient field-free molecular orientation -- a phenomenon important in chemical reaction dynamics, ultrafast molecular imaging, high harmonics generation, and attosecond science. However,…

Chemical Physics · Physics 2022-12-21 Ilia Tutunnikov , Long Xu , Yehiam Prior , Ilya Sh. Averbukh

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

We study the higher-harmonic generation (HHG) using elliptically polarized two-color driving fields. The HHG via bi-chromatic counter-rotating laser fields is a promising source of circularly polarized ultrashort XUV radiation at the…

Atomic Physics · Physics 2022-01-12 Rambabu Rajpoot , Amol R. Holkundkar , Jayendra N. Bandyopadhyay

We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…

Chemical Physics · Physics 2015-06-12 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

The below-threshold harmonic generation in the multiphoton ionization regime for a helium atom driven by the elliptically polarized laser field is studied numerically within the framework of two-dimensional (2D) and three-dimensional (3D)…

Optics · Physics 2024-12-11 Mikhail Yu. Emelin , Mikhail Yu. Ryabikin

We present a novel method for probing the alignment of the molecular axis of an ultracold, nonpolar dimer. These results are obtained using diatomic $^{87}\textrm{Rb}_2$ molecules in the vibrational ground state of the lowest triplet…

Atomic Physics · Physics 2015-01-15 Markus Deiß , Björn Drews , Benjamin Deissler , Johannes Hecker Denschlag

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…