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Related papers: Field-free molecular alignment induced by elliptic…

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The mixed-field orientation of an asymmetric-rotor molecule with its permanent dipole moment non-parallel to the principal axes of polarizability is investigated experimentally and theoretically. We find that for the typical case of a…

We investigate experimentally and numerically the field-free orientation of the symmetric top molecule of methyl-iodide at high temperature using a terahertz radiation generated by a plasma induced by a two-color laser beam. The degree of…

Quantum Physics · Physics 2016-11-03 P. Babilotte , K. Hamraoui , F. Billard , E. Hertz , B. Lavorel , O. Faucher , D. Sugny

We review on the theoretical status of intense laser orientation and alignment. The evolution of the rotational wave packet and its dynamics leading to orientation and alignment is the topic of the present discussion. The major part of the…

Atomic Physics · Physics 2021-04-14 Vijit V. Nautiyal , Sumana Devi , Ashish Tyagi , Bhawna Vidhani , Anjali Maan , Vinod Prasad

We have investigated non-dipole effects in the interaction of a hydrogen atom with elliptically polarized laser pulses of intensity 10$^{14}$ W/cm$^2$ with about 8 fs duration. The study was performed within the framework of a hybrid…

Atomic Physics · Physics 2025-09-03 Vladimir S. Melezhik , Sara Shadmehri

We discuss the existence of elliptical polarisation in rotational spectral lines of CO and other molecules within the context of the Anisotropic Resonant Scattering (ARS) model. We show that the effect of ARS on the radiation field can lead…

Astrophysics of Galaxies · Physics 2022-01-12 Martin Houde , Boy Lankhaar , Fereshteh Rajabi , Mohammed A. Chamma

Recently, we have used, pulsar polarisation datasets, on circular polarisation degree & linear polarisation position angle, to relate with well established theories, on ellipticity parameter and linear polarisation position angles, accrued…

High Energy Astrophysical Phenomena · Physics 2020-01-22 Karam Chand , Subhayan Mandal

We show that a 450 fs nonresonant, moderately intense, linearly polarized laser pulse can induce field-free molecular axis alignment of methyliodide molecules dissolved in a helium nanodroplet. Time-resolved measurements reveal rotational…

Chemical Physics · Physics 2015-06-12 Dominik Pentlehner , Jens H. Nielsen , Alkwin Slenczka , Klaus Mølmer , Henrik Stapelfeldt

We develop a general method allowing one to construct the consistent theory of light pulse propagation through an atomic medium in arbitrary nonlinear regime with respect to the field strength, taking into account the light polarization,…

Optics · Physics 2015-06-16 V. I. Yudin , M. Yu. Basalaev , D. V. Brazhnikov , A. V. Taichenachev

We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…

Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While…

Atomic Physics · Physics 2012-09-14 Michael Spanner , Serguei Patchkovskii , Eugene Frumker , Paul Corkum

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

Optics · Physics 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu

We predict theoretically and demonstrate experimentally an ellipticity-dependent nonlinear magneto-optic rotation of elliptically-polarized light propagating in a coherent atomic medium. We show that this effect results from a hexadecapole…

Atomic Physics · Physics 2009-11-07 A. B. Matsko , I. Novikova , M. S. Zubairy , G. R. Welch

Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…

The impact of nonadiabatic laser-induced molecular alignment on filamentation is numerically studied. Weak and strong field model of impulsive molecular alignment are compared in the context of nonlinear pulse propagation. It is shown that…

Optics · Physics 2014-12-03 N. Berti , P. Béjot , J. -P. Wolf , O. Faucher

Two types of room temperature detectors of terahertz laser radiation have been developed which allow in an all-electric manner to determine the plane of polarization of linearly polarized radiation and the Stokes parameters of elliptically…

Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…

Atomic Physics · Physics 2018-01-17 Nehzat Safaei

A pump-probe polarimetric technique is demonstrated, which provides a complete, temporally and spatially-resolved mapping of the megagauss magnetic fields generated in intense short-pulse laser-plasma interactions. A normally-incident…

Focusing optics for neutral molecules finds application in shaping and steering molecular beams. Here we present an electrostatic elliptical mirror for polar molecules consisting of an array of microstructured gold electrodes deposited on a…

We explore the possibility of forming a oriented polar molecule directly from a pair of colliding atoms. The process comprises the photoassociation and vibrational stabilization along with the molecular orientation. These processes are…

Quantum Physics · Physics 2026-01-14 Murilo D. Forlevesi , Edson Denis Leonel , Emanuel F. de Lima

We present a study of Mott scattering of polarized electrons in the presence of a laser field with circular polarization using the helicity formalism and the introduction of the well known concept of non flip differential cross section as…

Atomic Physics · Physics 2009-07-28 B. Manaut , Y. Attaourti , S. Taj , S. Elhandi