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The electric dipole moment of an electron (eEDM) is one of the sensitive probes of physics beyond the standard model. The possible existence of the eEDM gives rise to an experimentally observed energy shift, which is proportional to the…

Computational Physics · Physics 2017-01-18 A. Sunaga , M. Abe , M. Hada , B. P. Das

The hyperfine structure (hfs) of electron levels of $^{238}_{92}$U ions with the nucleus excited in the low-lying rotational $2^+$ state with an energy $E_{2^+} = 44.91$ keV is investigated. In hydrogenlike uranium, the hfs splitting for…

Quantum Physics · Physics 2009-10-31 L. N. Labzowsky , A. V. Nefiodov , G. Plunien , G. Soff , D. Liesen

The molecular ion ThF$^+$ is the species to be used in the next generation of search for the electron's Electric Dipole Moment (eEDM) at JILA. The measurement requires creating molecular ions in the eEDM sensitive state, the rovibronic…

Chemical Physics · Physics 2019-03-27 Yan Zhou , Kia Boon Ng , Lan Cheng , Daniel N. Gresh , Robert W. Field , Jun Ye , Eric A. Cornell

Recently an improved limits on the electron electric dipole moment, \eEDM, and dimensionless constant, $k_{T,P}$, characterizing the strength of the T,P-odd pseudoscalar$-$scalar electron$-$nucleus neutral current interaction in the…

Atomic Physics · Physics 2015-01-13 L. V. Skripnikov , A. V. Titov

We present an updated EDM effective electric field of $E_{\text{eff}} = 75.2\left[\frac{\rm GV}{\rm cm}\right]$ and the electron-nucleon scalar-pseudoscalar interaction constant $W_S=107.8$ [kHz] for the ${^3\Delta}_1$ science state of ThO.…

Atomic Physics · Physics 2016-05-11 Malika Denis , Timo Fleig

A recently implemented relativistic four-component configuration interaction approach to study ${\cal{P}}$- and ${\cal{T}}$-odd interaction constants in atoms and molecules is employed to determine the electron electric dipole moment…

Atomic Physics · Physics 2014-04-02 Timo Fleig , Malaya K. Nayak

Relativistic coupled-cluster calculations of the ionization potential, dissociation energy, and excited electronic states under 35,000 cm$^{-1}$ are presented for the actinium monofluoride (AcF) molecule. The ionization potential is…

Heavy polar diatomic molecules are currently among the most promising probes of fundamental physics. Constraining the electric dipole moment of the electron (eEDM), in order to explore physics beyond the Standard Model, requires a synergy…

Atomic Physics · Physics 2018-04-18 M Abe , V S Prasannaa , B P Das

Ab initio calculation of the hyperfine, P-odd, and P,T-odd constants for the YbF molecule was performed with the help of the recently developed technique, which allows to take into account correlations and polarization in the outercore…

Atomic Physics · Physics 2015-06-26 N. S. Mosyagin , M. G. Kozlov , A. V. Titov

We demonstrate the importance of electron correlation effects in the hyperfine structure constants of many low-lying states in $^{210}$Fr and $^{212}$Fr. This is achieved by calculating the magnetic dipole and electric quadrupole hyperfine…

Atomic Physics · Physics 2015-05-20 B. K. Sahoo , D. K. Nandy , B. P. Das , Y. Sakemi

HfF$^+$ cation is a very promising system to search for the electron electric dipole moment (EDM), and corresponding experiment is carried out by E. Cornell group. Here we theoretically investigate the cation to search for another T,P-odd…

Atomic Physics · Physics 2017-03-08 L. V. Skripnikov , A. V. Titov , V. V. Flambaum

A precise theoretical study of the electronic structure of heavy atom diatomic molecules is of key importance to interpret the experiments in the search for violation of time-reversal (T) and spatial-parity (P) symmetries of fundamental…

Atomic Physics · Physics 2016-12-02 L. V. Skripnikov

Recently the Eu$_{0.5}$Ba$_{0.5}$TiO$_{3}$ solid was suggested as a promising candidate for experimental search of the electron electric dipole moment. To interpret the results of this experiment one should calculate the effective electric…

Atomic Physics · Physics 2015-01-13 L V Skripnikov , A V Titov , A N Petrov , N S Mosyagin , O P Sushkov

We have completed a new precision measurement of the electron's electric dipole moment using trapped HfF$^+$ in rotating bias fields. We report on the accuracy evaluation of this measurement, describing the mechanisms behind our systematic…

The spectrum of electronic states at 30000--33000 cm$^{-1}$ in hafnium fluoride has been studied using (1+1) resonance-enhanced multi-photon ionization (REMPI) and (1+1$'$) REMPI. Six $\Omega' = 3/2$ and ten $\Pi_{1/2}$ vibronic bands have…

Efficient quantum-state detection is crucial for many precision control experiments, such as the ongoing effort to probe the electron's electric dipole moment using trapped molecular $^{232}\mathrm{ThF}^+$ ions at JILA. While quantum state…

We have investigated energies, magnetic dipole hyperfine structure constants ($A_{hyf}$) and electric dipole (E1) matrix elements of a number of low-lying states of the triply ionized tin (Sn$^{3+}$) by employing relativistic…

Atomic Physics · Physics 2020-04-22 Mandeep Kaur , Rishabh Nakra , Bindiya Arora , Cheng-Bin Li , B. K. Sahoo

Heavy polar diatomic molecules are currently one of the leading candidates for probing physics beyond the Standard Model via studies of time-reversal (T) and parity (P) violations. In this work, we analyze the effective electric field…

Atomic Physics · Physics 2018-11-14 A. Sunaga , V. S. Prasannaa , M. Abe , M. Hada , B. P. Das

The NL-eEDM collaboration is building an experimental setup to search for the permanent electric dipole moment of the electron in a slow beam of cold barium fluoride molecules [Eur. Phys. J. D, 72, 197 (2018)]. Knowledge of molecular…

The atomic states of the W IX (W8+) tungsten ion lying below the W9+ ionisation threshold have been studied theoretically, employing the multiconfiguration Dirac-Hartree-Fock method with configuration interaction. The level electronic…

Atomic Physics · Physics 2020-07-30 Karol Kozioł , Jacek Rzadkiewicz