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Large-scale $\textit{ab initio}$ calculations of the electric field gradient, which constitutes the electronic contribution to the electric quadrupole hyperfine constant $B$, were performed for the $5s^25p6s$ $^{1,3}\!P^{\rm o}_1$ excited…

The electronic excitation spectrum of a material characterises the response to external electromagnetic perturbations through its energy loss function (ELF), which is obtained from several experimental sources that usually do not completely…

Materials Science · Physics 2024-12-20 Fan Cheng , Pablo de Vera , Rafael Garcia-Molina

In conjunction with ab initio potential energy and dipole moment surfaces for the electronic ground state, we have made a theoretical study of the radiative lifetimes for the hydronium ion H$_3$O$^{+}$ and its deuterated isotopologues. We…

Chemical Physics · Physics 2016-11-03 Vladlen V. Melnikov , Sergei N. Yurchenko , Jonathan Tennyson , Per Jensen

The ground state hyperfine splitting values and the transition probabilities between the hyperfine structure components of high Z lithiumlike ions are calculated in the range $Z=49-83$. The relativistic, nuclear, QED and interelectronic…

We report on high-resolution laser spectroscopy of $^{255}$Fm ($T_{1/2} = 20$h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4~nm and…

\'Eliashberg theory, being generalized to the electron-phonon (EP) systems with not constant density of electronic states, as well as to the frequency behavior of the renormalization of both the electron mass and the chemical potential, is…

Superconductivity · Physics 2016-07-11 Nikolay Kudryashov , Alexander Kutukov , Evgeny Mazur

The thorium nucleus with mass number $A=229$ has attracted much interest because its extremely low lying first excited isomeric state at about $8$eV opens the possibility for the development of a nuclear clock. However, neither the exact…

A measurement of hafnium foil using a modified ultra-low-background high purity detector with optimized sample-to-detector geometry was performed at Laboratori Nazionale del Gran Sasso. Radiopurity of the stock Hf foil was studied in…

Nuclear Experiment · Physics 2021-06-02 B. Broerman , M. Laubenstein , S. Nagorny , N. Song , A. C. Vincent

<001> oriented 0.7Pb(Mg1/3Nb2/3)O3-0.3PbTiO3 single crystals were poled under different electric fields, i.e. Epoling=4 kV/cm and Epoling=13 kV/cm. In addition to the temperature-dependent dielectric constant measurement, X-ray diffraction…

Materials Science · Physics 2009-11-07 Ke-Pi Chen , Xiao-Wen Zhang , Hao-Su Luo

We present state-of-the-art configuration interaction and coupled cluster calculations of the electron electric dipole moment, the nucleon-electron scalar-pseudoscalar, and the magnetic hyperfine interaction constants ($\alpha_{d_e},…

Atomic Physics · Physics 2019-10-28 Timo Fleig , Leonid V. Skripnikov

To support efforts on cooling and trapping of alkaline-earth atoms and designs of atomic clocks, we performed ab initio relativistic many-body calculations of electric-dipole transition amplitudes between low-lying states of Mg, Ca, and Sr.…

Atomic Physics · Physics 2009-11-07 S. G. Porsev , M. G. Kozlov , Yu. G. Rakhlina , A. Derevianko

The most sensitive measurements of the electron electric dipole moment d_e have previously been made using heavy atoms. Heavy polar molecules offer a greater sensitivity to d_e because the interaction energy to be measured is typically 10^3…

High Energy Physics - Experiment · Physics 2011-08-11 J. J. Hudson , B. E. Sauer , M. R. Tarbutt , E. A. Hinds

Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals).…

Atomic Physics · Physics 2016-06-01 V. A. Dzuba , V. V. Flambaum

We consider the ground state of the homogeneous electron gas and we prove that a Hartree-Fock solution, motivated by previous simulations, has lower energy than the Fermi gas in the large density limit. This solution is a metallic phase :…

Strongly Correlated Electrons · Physics 2008-07-08 F. Delyon , M. Duneau , B. Bernu , M. Holzmann

We calculate the ground state phase diagram of the homogeneous electron gas in three dimensions within the Hartree-Fock approximation and show that broken symmetry states are energetically favored at any density against the homogeneous…

Strongly Correlated Electrons · Physics 2014-03-04 Lucas Baguet , François Delyon , Bernard Bernu , Markus Holzmann

The relativistic multiconfiguration Dirac-Hartree-Fock (MCDHF) and the non-relativistic multiconfiguration Hartree-Fock (MCHF) methods have been employed to calculate the magnetic dipole and electric quadrupole hyperfine structure constants…

The electronic structures of element cerium under high pressure remain unclear all the time. We tried to calculate the electronic structures of $\alpha'$, $\alpha"$, and $\epsilon$-Ce which only exist in the presence of pressure, by using…

Strongly Correlated Electrons · Physics 2018-11-02 Haiyan Lu , Li Huang

We perform a high-throughput screening on phonon-mediated superconductivity in ternary metal diboride structure with alkali, alkaline earth, and transition metals. We find 17 ground states and 78 low-energy metastable phases. From fast…

Condensed matter systems offer the opportunity to maximize the number of spins, probed in magnetic resonance experiments that search for physics beyond the standard model. EuCl$_3\cdot 6$H$_2$O is a promising solid-state platform for such…

Other Condensed Matter · Physics 2023-04-25 Alexander O. Sushkov

Within the finite-field Kohn-Sham framework, static electric response properties of diatomic molecules are presented. The electronic energy, dipole moment ({\boldmath$\mu$}), static dipole polarizability ({\boldmath$\alpha$}) and…

Chemical Physics · Physics 2019-04-26 Abhisek Ghosal , Tanmay Mandal , Amlan K. ~Roy
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